重丰中子核237Th半衰期的测量

通过60MeV/u的¹⁸O离子束轰击天然铀靶,利用多核子转移反应并由放射化学分离方法准备了²³⁷Th的存在,测得它的半衰期为(4.69±0.60)min.这个新的值不仅与我们较早获得的(5.0±0.9)min值一致,而且提高了实验精度.     

关于重丰中子远离核研究的实验方法

简单地介绍了重丰中子远离核研究的科学意义,报告了重丰中子新核素的产生、分离和鉴别方法。     

液-液萃取从Th中分离Ac

用234Th、228Ac和139Ce 3做示踪剂,二(2-乙基己基)磷酸做萃取剂,研究了初始HNO3浓度对234Th、228Ac和139Ce 3萃取效率的影响。发现在广泛的酸度范围内,234Th均能被定量地萃取;当HNO3浓度大于2.0mol/L时,228Ac和139Ce3 的萃取效率下降到2%以下。研究了震荡时间对234Th萃取效率的影响,数据显示,1min便可达到萃取平衡。从含大量钍的溶液中分离痕量Ac的实验结果显示,用二(2-乙基己基)磷酸-苯的萃取流程,可使Ac与大量的钍分离,同时Ac的损失又较小。     

Dependence of the cross sections for Ir isotopes on the values of Qgg in the heavy ion collision

¹⁹⁷Au were irradiated with 47 MeV/u ¹²C ions. Iridium was produced via the multinucleon transfer reactions in bombardments of ¹⁹⁷Au with ¹²C. and was separated radiochemically from Au and the mixture of the reaction products. The γ radioactivities of Ir isotopes were measured by using a HPGe detector. The production cross sections of Ir isotopes were determined from activities of Ir isotopes at the end of bombardment and the other relative data. It has been found that the cross sections for neutron-rich isotopes of iridium show an exponential dependence on the values of Q_gg. Our experimental results also demonstrate lack of correlation between the cross sections and Q_gg in the case of neutron-deficient isotopes of iridium. The fact can be explained from that neutron-rich isotopes of iridium were produced in the deep inelastic transfer reactions.     

丰中子同位素189W β－衰变的新γ线

本文报告了用快中子轰击天然Os靶,化学分离后,通过对W样品的γ单谱和时间序列谱的分析,发现了11条以前未知的¹⁸⁹W的新γ射线     

新重丰中子同位素175Er的合成和γ衰变

用14MeV中子轰击天然镜靶,通过¹⁷⁶Yb(n,2p)¹⁷⁵Er反应,首次合成了新同位素¹⁷⁵Er.利用γ(X)谱学方法,对¹⁷⁵Er的活性进行了观测,发现了能量为76.5,120.9,123.7,128.5,227.3,234.0,281.4,1167.5keV半衰期为1.2±0.3min的八条新γ射线,并指定为¹⁷⁵Er的β-衰变.建立了¹⁷⁵Er的部分衰变纲图.     

用二-2-乙基己基磷酸和P2O5混合物从硝酸溶液中萃取Am（Ⅲ）

用二-2-乙基己基磷酸（HDEHP）和P2O5混合物做萃取剂^241 Am^3＋为示踪剂,做了从硝酸溶液中液-液萃取Am的实验研究。完成了硝酸浓度和震荡时间的变化影响^241 Am^3＋萃取效率的条件实验。发现P20,的浓度≥0．0125mol／L时,^241 Am^3＋ 的萃取效率大干98％;震荡时间≥30s,两相便可达到萃取平衡。分别用二乙撑三胺五乙酸（DTPA）-乳酸以及N％CO3溶液对^241 Am^3＋进行反萃取。结果显示N％CO,溶液能给出很高的反萃效率。而且,在很短的震荡时间内,两相都能达到反萃平衡。     

266Bh的α衰变性质研究(英文)

报道了利用兰州重离子研究装置提供的26Mg重离子束流轰击243Am靶产生和鉴别已知超重核素266Bh的实验结果。利用转轮收集探测装置依靠母子核遗传关系通过观测Bh同位素与其子核Db和Lr之间的α-α关联事件来鉴别266Bh。实验中观测到266Bh的α能量为（9.03 ± 0.08）MeV, 与日本理化学研究所在合成113号元素中第一个衰变链中观测到266Bh的α能量为9.07 MeV相近。 266Bh的半衰期为0.66+0.59-0.26 s, 从实验得到的Qα也符合Z=107的Qα随中子数变化的系统性。The isotope of 266Bh was produced and identified definitely in bombardments of 243Am target with 162 MeV 26Mg ions at HIRFL. Identification was made by observation of correlated α particle decays between the Bh isotopes and their Db and Lr daughters using a rotating wheel system. The measured α energy for 266Bh is (9.03±0.08) MeV, and this value close to the 9.07 MeV for 266Bh observed in the first chain of element 113 at RIKEN. The half life of 266Bh is 0.66+0.59 -0.26 s. The Qα value derived from this experiment fits well into the general trend in a “Qα N systematics” for the isotopes with Z = 107.     

新核素238Th的鉴别

利用60MeV/u的¹⁸O离子束轰击天然铀靶,通过多核子转移反应生成重丰中子新核素²³⁸Th.观测到了²³⁸Th的子体²³⁸Paγ活性的生长、衰变行为,鉴别了²³⁸Th的存在,并测得它的半衰期为(9.4±2.0)min.同时,发现了一条能量为(89.0±0.3)keV、半衰期为(8.9±1.5)min的新γ射线,指定为²³⁸Th的衰变γ射线.     

208Hg鉴别

本文较详细地描述了新丰中子核素²⁰⁸Hg的鉴别及半衰期测定程序.²⁰⁸Hg的鉴别采用了二步离线化学分离:第一步是基于热色谱原理的高效、高选择性的Hg产物收集,第二步是周期性地提取生长起来的T1.在提取的T1样品中观察到半衰期约3min的2614.6keVγ活性.该γ活性可归结为由²⁰⁸Hg β^－衰变而生长起来的²⁰⁸T1的衰变γ.