紧耦合方法研究离子原子碰撞的单俘获过程

介绍了双中心原子轨道紧耦合方法计算离子原子碰撞的单俘获截面的基本原理，对于双中心 原子轨道紧耦合方法，找到一种系统化计算模型参数的方法，并根据该方法得到有关模型参 数，计算了O⁶⁺离子与H碰撞系统，所得计算结果在实验误差范围内与实验值很 好符合． 关键词： 双中心原子轨道紧耦合 单俘获截面 模型势 半经典碰撞参数模型 Numer ov算法     

Measurement of ^16O^5＋ Induced L X-Ray Production Cross Sections for Gold

The characteristic L1, Lα, Lβ and Lγ x-rays of Au and energy shifts produced by 20-50 MeV ^16O^5＋ beams on a thick Au film are measured with a Si （Li） detector. Cross-section ratios of σ（Ll）/σ（Lα）, σ（Lβ）/σ（Lβ） and σ（Lγ）/σ（Lα） versus O^5＋ energy show that consistent calculations yield considerably better agreements. Energy shifts L1, Lα, Lβ and Lγ x-rays of Au target increase with more incidence energy. The main application for these measurements is multi-element trace analysis through particle induced x-ray emission.     

Multi-Electron Processes in ^13C^6＋ Ions with Neon Collisions in Energy Region 4.15-11.08 keV/u

The cross-section ratios of double-, triple-, quadruple-, and the total multi-electron processes to the single electron capture process （σ^DE/σ^SC, σ^TE/σ^SC, σ^QE/σ^SC and σ^ME/σ^SC） as well as the relative ratios among reaction channels in double-electron active, triple-electron active and quadruple-electron active are measured in ^13C^6＋_Ne collision in the energy region of 4.15-11.08keV/u by employing position-sensitive and time-of-flight coincident techniques. It is determined that the cross-section ratios σ^DE /σ^SC, σ^TE /σ^SC, σ^QE /σ^SC and σ^ME /σ^SC are approximately the constants of 0.20 ± 0.03, 0.16 ± 0.04, 0.06 ± 0.02 and 0.42 ± 0.05. These values are obviously smaller than the predictions of the molecular Coulomb over-the-barrier model （MCBM） [J. Phys. B 23 （1990） 4293], the extended classical over-the-barrier model （ECBM） [J. Phys. B 19 （1986） 2925] and the semiempirical scaling laws （SL） [Phys. Rev. A 54 （1996） 4127]. However, the relative ratios among partial processes of DE, TE and QE are found to depend on collision energy, which suggests that the collision dynamics depends on the collision velocity. The limitation of velocity-independent character of ECBM, MCBM and SL is undoubtedly shown.     

Two Electron Transfer and Stabilization in Slow O^6＋ and Rare-Gas Collisions

The stabilization ratios R for double-electron transfer, i.e., the cross section ratios of true double capture to total double-electron transfer, are measured in O^6＋ ＋He, Ne and Ar collisions at 6 keV/u. A high R value about 68% is obtained for the He target, while for the Ar target, the R value is only 8%. The high R value for the He target is due to the significant direct population of the （2l, nl′ ） configurations with high n. For the Ar target, the （quasi）symmetric configurations （3l, nl′） lead to the much lower R value. Neglecting the core effects, the O^6＋ ion can be taken as a bare ion C^6＋ except the occupied ls shell, and then the measured R values are compared with previous experimental results of C^6＋ projectile ions at Ne and Ar target, while the occupied ls shell for the C^6＋ ＋He collisions. similar impact velocity. It yields good agreement with the O^6＋ ＋He system results in a higher R value than that in     

高电荷态离子Ar~(q+)与Nb作用产生的X射线谱

利用光谱技术在超导离子源SECRAL上研究了10~20keV·q的Arq+(q=16,17)离子入射在金属Nb表面产生的X射线谱.实验结果表明,高电荷态Ar16+离子在金属表面中性化过程中存在着多电子激发,Ar16+的K壳层电子被激发产生空穴,级联退激发射Ar的Kα特征X射线.Ar空心原子的K层发射X射线的强度随入射离子的动能减弱,靶原子Nb的L层发射X射线强度随入射离子动能的增加而增强.Ar17+单离子的Kα-X射线产额比Ar16+单离子的Kα-X射线产额大3个数量级.     

非全裸氟离子与氦原子碰撞中的转移电离过程

采用位置灵敏探测和散射离子 反冲离子飞行时间测量技术 ,测量了强相互作用区氟离子与氦原子碰撞中的转移电离截面与单电子俘获截面之比 .实验发现 ,该比值随作用强度的增加而减小 .在本工作能区 ,转移电离现象可视作一个电子被俘获、另一个电子被电离的两步过程 ;He原子二重电离的主要机制为两步机制. The cross-section ratios of the transfer ionization to the single electron capture of helium induced by fluorine ions in the strong-interaction region were measured by means of the position-sensitive-detecting and the time-of -flight (TOF) technologies. Is is found that the cross section ratios decrease with the increasing of the interaction-strength κ in this work. In the energy range of this work, the transfer ionization can be considered as a two-step process that one electron is captured by projectile...     

Ar16+和Ar17+离子与Zr作用产生的X射线谱

将超导离子源提供的10—20keV/q Ar¹⁶⁺和Ar¹⁷⁺离子入射到Zr金属表面,在相互作用中产生的X射线谱表明,高电荷态Ar¹⁶⁺离子在金属表面中性化过程中有可能存在多电子激发,使Ar¹⁶⁺的K壳层电子被激发形成空穴,在退激过程中发射特征Kα-X射线.空心原子Ar的K层发射X射线强度随入射离子的动能而减弱,靶原子Zr的L壳层发射X射线强度随入射离子动能的增加而增强.Ar¹⁷⁺的单离子的Kα- 关键词： 高电荷态离子 空心原子 X射线     

Ar16+和Ar17+离子与Zr作用产生的X射线谱

将超导离子源提供的10—20keV/q Ar¹⁶⁺和Ar¹⁷⁺离子入射到Zr金属表面，在相互作用中产生的X射线谱表明，高电荷态Ar¹⁶⁺离子在金属表面中性化过程中有可能存在多电子激发，使Ar¹⁶⁺的K壳层电子被激发形成空穴，在退激过程中发射特征Kα-X射线.空心原子Ar的K层发射X射线强度随入射离子的动能而减弱，靶原子Zr的L壳层发射X射线强度随入射离子动能的增加而增强.Ar¹⁷⁺的单离子的Kα-     

高电荷态Xe离子与He原子碰撞中的电子转移过程研究

采用位置灵敏探测和飞行时间技术研究了高电荷态Xe离子（q=15，17，19，21，23）与He原子碰撞中双电子转移截面与单电子转移截面比随入射离子电荷态的变化规律.提出一步过程假定，对扩展的经典过垒（ECB）模型进行了修正，利用修正模型计算得到的单、双电子转移绝对截面与Andersson等人和Selberg等人的实验结果很好符合，所得截面比与本实验得到的双电子转移截面与单电子俘获截面比较好符合. 关键词： 离子 原子碰撞 电荷转移 一步过程     

Transfer ionization of the isocharge sequence ion and Ar collisions

The ratios of transfer ionization to single capture for isocharge C^{q+}, N^{q+}, O^{q+}, Ne^{q+} ions on Ar atoms are measured by using position-sensitive and time-of-flight techniques. It is found that the ratio R_{1} increases with nuclear charge Z in a q=4 sequence, and the ratio R_{1} sequences have the minimum values at Z=7 and Z=8 in q=5 and q=6 sequences, respectively, and the ratio R_{1} decreases with the increase in the nuclear charge Z in a q=7 sequence. The results may be explained within the frame of the statistical model. It may be concluded that the transfer ionization depends remarkably upon the electronic structure of the projectile. The projectiles used in this study have the same charge state and velocity, but different electronic structures. The dependence of the ratio R_{1} on q is studied for Ne^{q+}-Ar collisions. The ratio R_{1} is found to increase as q increases for Ne^{q+}－Ar collisions. The measured dependence of the ratio R_{1} on q is compared with the calculation using the molecular Coulomb over-barrier model.