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101.
Wei‐Ling Wang Jian‐Wei Xu Yee‐Hing Lai 《Journal of polymer science. Part A, Polymer chemistry》2006,44(13):4154-4164
Bipyridinophane–fluorene conjugated copolymers have been synthesized via Suzuki and Heck coupling reactions from 5,8‐dibromo‐2,11‐dithia[3]paracyclo[3](4,4′)‐2,2′‐bipyridinophane and suitable fluorene precursors. Poly[2,7‐(9,9‐dihexylfluorene)‐co‐alt‐5,8‐(2,11‐dithia[3]paracyclo[3](4,4′)‐2,2′‐bipyridinophane)] ( P7 ) exhibits large absorption and emission redshifts of 20 and 34 nm, respectively, with respect to its planar reference polymer Poly[2,7‐(9,9‐dihexylfluorene)‐co‐alt‐1,4‐(2,5‐dimethylbenzene)] ( P11 ), which bears the same polymer backbone as P7 . These spectral shifts originate from intramolecular aromatic C? H/π interactions, which are evidenced by ultraviolet–visible and 1H NMR spectra as well as X‐ray single‐crystal structural analysis. However, the effect of the intramolecular aromatic C? H/π interactions on the spectral shift in poly[9,9‐dihexylfluorene‐2,7‐yleneethynylene‐co‐alt‐5,8‐(2,11‐dithia[3]paracyclo[3](4,4′)‐2,2′‐bipyridinophane)] ( P10 ) is much weaker. Most interestingly, the quenching behaviors of these two conjugated polymers are largely dependent on the polymer backbone. For example, the fluorescence of P7 is efficiently quenched by Cu2+, Co2+, Ni2+, Zn2+, Mn2+, and Ag+ ions. In contrast, only Cu2+, Co2+, and Ni2+ ions can partially quench the fluorescence of P10 , but much less efficiently than the fluorescence of P7 . The static Stern–Volmer quenching constants of Cu2+, Co2+, and Ni2+ ions toward P7 are of the order of 106 M?1, being 1300, 2500, and 37,300 times larger than those of P10 , respectively. © 2006 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 44: 4154–4164, 2006 相似文献
102.
Mueller C. Sullivan C. Chang W. Hall D. Zino J. Rice R. 《Quantum Electronics, IEEE Journal of》1980,16(3):363-372
Calculated butt coupling efficiency between a GaAlAs double heterostructure laser and a single-mode LiNbO3 Ti-diffused optical waveguide is presented in this paper as a function of the transverse displacement, the angular alignment, the longitudinal separation between the laser and the waveguide end surfaces, the radiation field of the laser diode and its dependence on the laser diode structure, and the mode profile of the waveguide and its dependence on experimental diffusion parameters. The maximum efficiency is less than 40 percent because of the mismatch between the waveguide mode and the laser radiation, caused primarily by the experimental limitations in their structures. The effect of the reflection of the waveguide end surface on the laser oscillation has also been estimated. 相似文献
103.
In this paper, we give a recursive construction from an LTTS(v + 2) to an LTTS(16v + 2) for v 3. Furthermore, the existence of LTTS(2n + 2) is proved. Thereby, we completely solve the existence problem of LTTS)(v) (large set of pairwise disjoint transitive triple systems of order v). 相似文献
104.
Shu-Cheng Chang 《Mathematische Annalen》2002,324(3):465-490
In this paper, we consider the 2-dimensional local Calabi flow on a complete noncompact surface . Then, based on the Harnack-type estimate, we show the long-time existence and asymptotic convergence of a subsequence of
solutions of such a flow on with and bounded from above by a negative constant on a ball. For its applications, this will lead to the existence of extremal metrics
on a complete noncompact surface of finite topological type. In particular, there exists an extremal metric of nonconstant
Gaussian curvature on or
Received: 21 June 2001 / 18 January 2002 / Published online: 27 June 2002
Research supported in part by NSC and NCTS. 相似文献
105.
106.
107.
本文讨论了M序列的自相关性,并证明了:当0<|t-2^n-1|≤[n-1/2]时,|CM(t)|≤2^n-1。 相似文献
108.
天线方向图的复射线仿真 总被引:1,自引:0,他引:1
根据复射线理论,利用复源点高斯波束场来模拟天线的远场方向图。本文提出三种模拟方法,即主瓣匹配法,峰值匹配法和逐点匹配法,给出了多种方向图的仿真结果。数值分析和优化结果表明,复射线峰值匹配法是一种精确实用的天线方向图仿真技术。 相似文献
109.
Long-Wen Chang Shui-kung Chuag Shang-shung Yu 《Multidimensional Systems and Signal Processing》1994,5(3):319-330
The compression of Chinese characters is very important for Chinese office automation and desktop publishing. In this paper, various methods are used to compress 13,051 Chinese characters losslessly by coding their skeleton points. The skeleton points are composed of isolated points and curves. To trace every point in a curve once and consecutively is a NP problem. Therefore, we use contour path following and revisiting algorithms to trace skeleton curves with chain codes. The remaining isolated skeleton points are encoded by an Elias code. Our coding method has a better compression rate than that of conventional skeleton coding. 相似文献
110.
Yu-Zung Chiou Yan-Kuin Su Shoou-Jinn Chang Yi-Chao Lin Chia-Sheng Chang Chin-Hsiang Chen 《Solid-state electronics》2002,46(12):2227-2229
InGaN/GaN multiquantum well (MQW) p–n junction photodetectors with semi-transparent Ni/Au electrodes were fabricated and characterized. It was found that the fabricated InGaN/GaN MQW p–n junction photodetectors exhibit a 20 V breakdown voltage and a 3.5 V forward 20 mA turn on voltage. It was also found that the photocurrent to dark current contrast ratio is higher than 105 when a 0.4 V reverse bias was applied to the InGaN/GaN MQW p–n junction photodetectors. Furthermore, it was found that the maximum responsivity was 1.28 and 1.76 A/W with a 0.1 and 3 V applied reverse bias, respectively. 相似文献