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111.
Hui Zhang Yinkun Sun Junjie Yang Zhiyu Sun Yanxin Zhao Xin Li Wei Wang Dongwei Lu Jun Ma 《Advanced functional materials》2023,33(40):2302816
Precise adjustment of the pore size, damage repair, and efficient cleaning is all challenges for the wider application of inorganic membranes. This study reports a simple strategy of combining dry-wet spinning and electrosynthesis to fabricate stainless-steel metal–organic framework composite membranes characterized by customizable pore sizes, targeted reparability, and high catalytic activity for membrane cleaning. The membrane pore size can be precisely customized in the range of 14–212 nm at nanoscale, and damaged membranes can be repaired by targeted treatment in 120 s. In addition, advanced oxidation processes can be used to quickly clean the membrane and achieve 98% flux recovery. The synergistic actions of the membrane matrix and the selective layer increase the adsorption energy of active sites to oxidant, shorten the electron transfer cycle, and enhance the overall catalytic performance. This study can provide a new direction for the development of advanced membranes for water purification and high-efficiency membrane cleaning methods. 相似文献
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Jine Zhang Xiaobing Chen Mengqin Wang Qinghua Zhang Wenxiao Shi Xiaozhi Zhan Meng Zhao Zhe Li Jie Zheng Hui Zhang Furong Han Huaiwen Yang Tao Zhu Banggui Liu Fengxia Hu Baogen Shen Yuansha Chen Yue Zhang Yunzhong Chen Weisheng Zhao Jirong Sun 《Advanced functional materials》2023,33(41):2306434
Ferromagnetic materials with a strong spin-orbit coupling (SOC) have attracted much attention in recent years because of their exotic properties and potential applications in energy-efficient spintronics. However, such materials are scarce in nature. Here, a proximity-induced paramagnetic to ferromagnetic transition for the heavy transition metal oxide CaRuO3 in (001)-(LaMnO3/CaRuO3) superlattices is reported. Anomalous Hall effect is observed in the temperature range up to 180 K. Maximal anomalous Hall conductivity and anomalous Hall angle are as large as ∼15 Ω−1 cm−1 and ∼0.93%, respectively, by one to two orders of magnitude larger than those of the typical 3d ferromagnetic oxides such as La0.67Sr0.33MnO3. Density functional theory calculations indicate the existence of avoid band crossings in the electronic band structure of the ferromagnetic CRO layer, which enhances Berry curvature thus strong anomalous Hall effects. Further evidences from polarized neutron reflectometry show that the CaRuO3 layers are in a fully ferromagnetic state (∼0.8 μB/Ru), in sharp contrast to the proximity-induced canted antiferromagnetic state in 5d oxides SrIrO3 and CaIrO3 (∼0.1 μB/Ir). More than that, the magnetic anisotropy of the (001)-(LaMnO3/CaRuO3) superlattices is eightfold symmetric, showing potential applications in the technology of multistate data storage. 相似文献
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Wireless Personal Communications - With the rapid development of information technology, issues such as network security and privacy protection have attracted more and more attention. The... 相似文献
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A new self-assembled and highly oriented one-dimensional single-crystal nanostructure of WO3 with hexagonal form was successfully prepared by a mild, solution-based colloidal approach. 相似文献