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31.
Ran Chen Dr. Nikoloz Nioradze Dr. Padmanabhan Santhosh Dr. Zhiting Li Dr. Sumedh P. Surwade Ganesh J. Shenoy David G. Parobek Min A. Kim Prof. Haitao Liu Prof. Shigeru Amemiya 《Angewandte Chemie (International ed. in English)》2015,54(50):15134-15137
High electrochemical reactivity is required for various energy and sensing applications of graphene grown by chemical vapor deposition (CVD). Herein, we report that heterogeneous electron transfer can be remarkably fast at CVD‐grown graphene electrodes that are fabricated without using the conventional poly(methyl methacrylate) (PMMA) for graphene transfer from a growth substrate. We use nanogap voltammetry based on scanning electrochemical microscopy to obtain very high standard rate constants k0≥25 cm s?1 for ferrocenemethanol oxidation at polystyrene‐supported graphene. The rate constants are at least 2–3 orders of magnitude higher than those at PMMA‐transferred graphene, which demonstrates an anomalously weak dependence of electron‐transfer rates on the potential. Slow kinetics at PMMA‐transferred graphene is attributed to the presence of residual PMMA. This unprecedentedly high reactivity of PMMA‐free CVD‐grown graphene electrodes is fundamentally and practically important. 相似文献
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Dr. A. Shine J. Shenoy Parvathy Jayan Dr. A. C. Jiji Dr. Vinesh Vijayan 《Chemphyschem》2020,21(9):888-894
Although the conformation of the polymer chain of Ubiquitin (Ub) mainly depends on the type of isopeptide linkage connecting two Ub molecules, the non-covalent (noncovalent) interaction between two Ub molecules within the chain could also tune their conformational preference. Here, we studied the conformation of noncovalently formed Ub dimers in solution using residual dipolar couplings (RDCs). Comparing the RDC derived alignment tensor of the noncovalently formed dimer with the two most abundant (K11 and K48) covalent linked Ub dimers revealed that the conformation of K11 linked and noncovalent Ub dimers were similar. Between the various NMR and crystal structures of K11 linked Ub dimers, RDC tensor analysis showed that the structure of K11 linked dimer crystalized at neutral pH is similar to noncovalent dimer. Analogous to the experimental study, the comparison of predicted order matrix of various covalent Ub dimers with that of the experimentally determined order matrix of noncovalent Ub dimer also suggests that the conformation of K11 linked dimers crystalized at neutral pH is similar to the noncovalent dimer. 相似文献
35.
Raunak M. Shenoy P. Goyal P. Ramamritham K. Kulkarni P. 《Selected Areas in Communications, IEEE Journal on》2002,20(7):1276-1289
In this paper, we examine the potential benefits of Web proxy caches in improving the effective capacity of servers and networks. Since networks and servers are typically provisioned based on a high percentile of the load, we focus on the effects of proxy caching on the tail of the load distribution. We find that, unlike their substantial impact on the average load, proxies have a diminished impact on the tail of the load distribution. The exact reduction in the tail and the corresponding capacity savings depend on the nature of the workload and the percentile of the load distribution chosen for provisioning networks and servers-the higher the percentile, the smaller the savings. For workloads considered in this study, compared with over a 50% reduction in the average load, the savings in network and server capacity was only 20%-35% for the 99th percentile of the load distribution. We also find that while proxies can be somewhat useful in smoothing out some of the burstiness in Web workloads; the resulting workload continues, however, to exhibit substantial burstiness and a heavy-tailed nature. We identify one-time requests for large objects to be the limiting factor that diminishes the impact of proxies on the tail of load distribution. We conclude that, while proxies are immensely useful to users due to the reduction in the average response time, they are less effective in improving the capacities of networks and servers. 相似文献
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P.P. Vaishnava C.W. Kimball A.M. Umarji S.K. Malik G.K. Shenoy 《Journal of magnetism and magnetic materials》1985,49(3):286-290
Magnetic and Mössbauer studies have been carried out on a series of ternary borides RFe4B (R = Er, Tm, Lu) which have the hexagonal CeCo4B type structure. These compounds are found to be magnetically ordered at room temperature. Magnetization studies in the temperature range from 5 to 300 K reveal the presence of compensation temperatures in Er and Tm compounds and indicate antiferromagnetic coupling between the rare earth and Fe moments. Room temperature 57Fe Mössbauer studies yield values of hyperfine fields at the two Fe sites as 246 and 185 kOe in ErFe4B and TmFe4B, and 204 and 145 kOe in LuFe4B. The 166Er Mössbauer studies give nearly free-ion hyperfine field at the Er sites which indicates that the exchange interaction in ErFe4B is much stronger than crystal field interaction. 相似文献
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A. V. Shenoy 《Colloid and polymer science》1984,262(4):319-337
A state-of-the-art review on drag reduction has been presented in order to bring out some important aspects of the drag reduction phenomenon and its potential for practical use. The review is biased towards micellar systems and discusses in detail the morphological differences between drag reducing polymeric and micellar systems. Work relating to polymeric systems has not been dealt in detail as it has been the subject of earlier reviews. Studies relating to biological additives as well as suspensions have been briefly mentioned without detailed discussion as their potential for practical use presently appears] to be limited.NCL-Communication No. 3384 相似文献
39.
A dynamic solution concept for abstract games 总被引:1,自引:0,他引:1
P. P. Shenoy 《Journal of Optimization Theory and Applications》1980,32(2):151-169
Several solution concepts have been defined for abstract games. Some of these are the core, due to Gillies and Shapley, the Von Neumann-Morgenstern stable sets, and the subsolutions due to Roth. These solution concepts are rather static in nature. In this paper, we propose a new solution concept for abstract games, called the dynamic solution, that reflects the dynamic aspects of negotiation among the players. Some properties of the dynamic solution are studied. Also, the dynamic solution of abstract games arising fromn-person cooperative games in characteristic function form is investigated.This research was supported by the Office of Naval Research under Contract No. N00014-75-C-0678, by the National Science Foundation under Grants Nos. MPS-75-02024 and MCS-77-03984 at Cornell University, by the United States Army under Contract No. DAAG-29-75-C-0024, and by the National Science Foundation under Grant No. MCS-75-17385-A01 at the University of Wisconsin. The author is grateful to Professor W. F. Lucas under whose guidance the research was conducted. 相似文献
40.
The hyperfine structure of dilute 166Er impurities in Au has been investigated between 1.8 and 60 K by Mössbauer spectroscopy. The hyperfine spectrum of the Γ7 electronic ground state is clearly observed below 4.2 K while at higher temperatures there is an indication of the contribution from the excited CEF-states Γ(1)8 and Γ6. Using Hirst's relaxation theory for the Γ7 ground state the magnetic hyperfine coupling constant A=(247±3) MHz and the exchange coupling constant Jsf=(0.10±0.02)eV were derived. A quadruple coupling constant B of about 1 MHz was estimated from the hyperfine pattern of the Γ(1)8 quartet. 相似文献