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991.
The influence of nearest-neighbor diffusion on the decay of a metastable low-coverage phase (monolayer adsorption) in a square lattice-gas model of electrochemical metal deposition is investigated by kinetic Monte Carlo simulations. The phase-transformation dynamics are compared to the well-established Kolmogorov-Johnson-Mehl-Avrami theory. The phase transformation is accelerated by diffusion, but remains in accord with the theory for continuous nucleation up to moderate diffusion rates. At very high diffusion rates the phase-transformation kinetic shows a crossover to instantaneous nucleation. Then, the probability of medium-sized clusters is reduced in favor of large clusters. Upon reversal of the supersaturation, the adsorbate desorbs, but large clusters still tend to grow during the initial stages of desorption. Calculation of the free energy of subcritical clusters by enumeration of lattice animals yields a quasiequilibrium distribution which is in reasonable agreement with the simulation results. This is an improvement relative to classical droplet theory, which fails to describe the distributions, since the macroscopic surface tension is a bad approximation for small clusters. 相似文献
992.
Lindenberg AM Acremann Y Lowney DP Heimann PA Allison TK Matthews T Falcone RW 《The Journal of chemical physics》2005,122(20):204507
Dynamical changes in the structure factor of liquid water, S(Q,t), are measured using time-resolved x-ray diffraction techniques with 100 ps resolution. On short time scales following femtosecond optical excitation, we observe temperature-induced changes associated with rearrangements of the hydrogen-bonded structure at constant volume, before the system has had time to expand. We invert this data to extract transient changes in the pair correlation function associated with isochoric heating effects, and interpret these in terms of a decrease in the local tetrahedral ordering. 相似文献
993.
This paper describes the design and implementation of a system-on-chip digital pH meter, for use in a wireless capsule application. The system is organized around an 8-bit microcontroller, designed to be functionally identical to the Motorola 6805. The analog subsystem contains a floating-electrode ISFET, which is fully compatible with a commercial CMOS process. On-chip programmable voltage references and multiplexors permit flexibility with the minimum of external connections. The chip is designed in a modular fashion to facilitate verification and component re-use. The single-chip pH meter can be directly connected to a personal computer, and gives a response of 37 bits/pH, within an operating range of 7 pH units. 相似文献
994.
Single-trial dynamical estimation of event-related potentials: a Kalman filter-based approach 总被引:3,自引:0,他引:3
Georgiadis SD Ranta-aho PO Tarvainen MP Karjalainen PA 《IEEE transactions on bio-medical engineering》2005,52(8):1397-1406
A method for single-trial dynamical estimation of event-related potentials (ERPs) is presented. The method is based on recursive Bayesian mean square estimation and the estimators are obtained with a Kalman filtering procedure. We especially focus on the case that previous trials contain prior information of relevance to the trial being analyzed. The potentials are estimated sequentially using the previous estimates as prior information. The performance of the method is evaluated with simulations and with real P300 responses measured using auditory stimuli. Our approach is shown to have excellent capability of estimating dynamic changes form stimulus to stimulus present in the parameters of the ERPs, even in poor signal-to-noise ratio (SNR) conditions. 相似文献
995.
Gauthier PA Berry A Woszczyk W 《The Journal of the Acoustical Society of America》2005,117(2):662-678
This paper describes the simulations and results obtained when applying optimal control to progressive sound-field reproduction (mainly for audio applications) over an area using multiple monopole loudspeakers. The model simulates a reproduction system that operates either in free field or in a closed space approaching a typical listening room, and is based on optimal control in the frequency domain. This rather simple approach is chosen for the purpose of physical investigation, especially in terms of sensing microphones and reproduction loudspeakers configurations. Other issues of interest concern the comparison with wave-field synthesis and the control mechanisms. The results suggest that in-room reproduction of sound field using active control can be achieved with a residual normalized squared error significantly lower than open-loop wave-field synthesis in the same situation. Active reproduction techniques have the advantage of automatically compensating for the room's natural dynamics. For the considered cases, the simulations show that optimal control results are not sensitive (in terms of reproduction error) to wall absorption in the reproduction room. A special surrounding configuration of sensors is introduced for a sensor-free listening area in free field. 相似文献
996.
Popper AN Smith ME Cott PA Hanna BW MacGillivray AO Austin ME Mann DA 《The Journal of the Acoustical Society of America》2005,117(6):3958-3971
Seismic airguns produce considerable amounts of acoustic energy that have the potential to affect marine life. This study investigates the effects of exposure to a 730 in.3 airgun array on hearing of three fish species in the Mackenzie River Delta, the northern pike (Esox lucius), broad whitefish (Coregonus nasus), and lake chub (Couesius plumbeus). Fish were placed in cages in the 1.9 m of water and exposed to five or 20 airgun shots, while controls were placed in the same cage but without airgun exposure. Hearing in both exposed and control fish were then tested using the auditory brainstem response (ABR). Threshold shifts were found for exposed fish as compared to controls in the northern pike and lake chub, with recovery within 24 hours of exposure, while there was no threshold shift in the broad whitefish. It is concluded that these three species are not likely to be substantially impacted by exposure to an airgun array used in a river seismic survey. Care must be taken, however, in extrapolation to other species and to fishes exposed to airguns in deeper water or where the animals are exposed to a larger number of airgun shots over a longer period of time. 相似文献
997.
We have investigated azimuthal spin-wave modes in magnetic vortex structures using time-resolved Kerr microscopy. Spatially resolved phase and amplitude spectra of ferromagnetic disks with diameters from 5 microm down to 500 nm reveal that the lowest order azimuthal spin-wave mode splits into a doublet as the disk size decreases. We demonstrate that the splitting is due to the coupling between spin waves and the gyrotropic motion of the vortex core. 相似文献
998.
A catastrophe model for the onset of fast magnetic reconnection is presented that suggests why plasma systems with magnetic free energy remain apparently stable for long times and then suddenly release their energy. For a given set of plasma parameters there are generally two stable reconnection solutions: a slow (Sweet-Parker) solution and a fast (Alfvénic) Hall reconnection solution. Below a critical resistivity the slow solution disappears and fast reconnection dominates. Scaling arguments predicting the two solutions and the critical resistivity are confirmed with two-fluid simulations. 相似文献
999.
Lisowski M Loukakos PA Melnikov A Radu I Ungureanu L Wolf M Bovensiepen U 《Physical review letters》2005,95(13):137402
Femtosecond electron and spin dynamics of the Gd(0001) surface are investigated by time-resolved photoemission and second harmonic generation. Upon optical excitation the spin polarization of the surface state is reduced by half while its exchange splitting remains nearly unchanged. Electron-magnon interaction is proposed to facilitate electron-spin-flip scattering among spin-mixed surface and bulk states, which provides a mechanism for ultrafast demagnetization. 相似文献
1000.
The question of whether or not DNA is intrinsically conducting is still a challenge. The ongoing debate on DNA molecules as an electronic material has so far underestimated a key distinction of the system: the role of base pairing in opposition to correlations along each chain. We show that a disordered base paired double chain presents truly or, at least, effectively delocalized states. This effect is irrespective to the sequencing along each chain. 相似文献