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141.
Summary
Bis(cyclopentadienyl)titanium(IV) diisothiocyanate [(Cp)2-Ti(NCS)2] reacts with MCl2 (M = Cu, Pd or Pt), [CuCl(PPh3)3], [RuCl2(PPh3)3] and [RuCl2(DMSO)4] (DMSO = dimethylsulphoxide) giving solid compounds of stochiometry [(Cp)2Ti(-NCS)2MCl2] (M = Cu, Pd or Pt), [(Cp)2Ti(-NCS)2CuCl(PPh3)], [(Cp)2Ti(-NCS)2-RuCl(PPh3)2]Cl and [(Cp)2Ti(-NCS)2RuCl2(DMSO)2]. These products have been characterized by physicochemical and spectroscopic methods. 相似文献
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143.
Aishani Mazumder Chung Kim Nguyen Thiha Aung Mei Xian Low Md. Ataur Rahman Salvy P. Russo Sherif Abdulkader Tawfik Shifan Wang James Bullock Vaishnavi Krishnamurthi Nitu Syed Abhishek Ranjan Ali Zavabeti Irfan H. Abidi Xiangyang Guo Yongxiang Li Taimur Ahmed Torben Daeneke Akram Al-Hourani Sivacarendran Balendhran Sumeet Walia 《Advanced functional materials》2023,33(36):2303641
Miniaturization and energy consumption by computational systems remain major challenges to address. Optoelectronics based synaptic and light sensing provide an exciting platform for neuromorphic processing and vision applications offering several advantages. It is highly desirable to achieve single-element image sensors that allow reception of information and execution of in-memory computing processes while maintaining memory for much longer durations without the need for frequent electrical or optical rehearsals. In this work, ultra-thin (<3 nm) doped indium oxide (In2O3) layers are engineered to demonstrate a monolithic two-terminal ultraviolet (UV) sensing and processing system with long optical state retention operating at 50 mV. This endows features of several conductance states within the persistent photocurrent window that are harnessed to show learning capabilities and significantly reduce the number of rehearsals. The atomically thin sheets are implemented as a focal plane array (FPA) for UV spectrum based proof-of-concept vision system capable of pattern recognition and memorization required for imaging and detection applications. This integrated light sensing and memory system is deployed to illustrate capabilities for real-time, in-sensor memorization, and recognition tasks. This study provides an important template to engineer miniaturized and low operating voltage neuromorphic platforms across the light spectrum based on application demand. 相似文献
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145.
Joshua M. Little Jiayue Sun Ali Kamali Amy Chen Asher C. Leff Yang Li Leah K. Borden Thilini U. Dissanayake Deborah Essumang Benita O. Oseleononmen Dongxia Liu Taylor J. Woehl Po-Yen Chen 《Advanced functional materials》2023,33(30):2215222
Assembling 2D-material (2DM) nanosheets into micro- and macro-architectures with augmented functionalities requires effective strategies to overcome nanosheet restacking. Conventional assembly approaches involve external binders and/or functionalization, which inevitably sacrifice 2DM's nanoscale properties. Noble metal ions (NMI) are promising ionic crosslinkers, which can simultaneously assemble 2DM nanosheets and induce synergistic properties. Herein, a collection of NMI–2DM complexes are screened and categorized into two sub-groups. Based on the zeta potentials, two assembly approaches are developed to obtain 1) NMI-crosslinked 2DM hydrogels/aerogels for heterostructured catalysts and 2) NMI–2DM inks for templated synthesis. First, tetraammineplatinum(II) nitrate (TPtN) serves as an efficient ionic crosslinker to agglomerate various 2DM dispersions. By utilizing micro-textured assembly platforms, various TPtN–2DM hydrogels are fabricated in a scalable fashion. Afterward, these hydrogels are lyophilized and thermally reduced to synthesize Pt-decorated 2DM aerogels (Pt@2DM). The Pt@2DM heterostructures demonstrate high, substrate-dependent catalytic activities and promote different reaction pathways in the hydrogenation of 3-nitrostyrene. Second, PtCl4 can be incorporated into 2DM dispersions at high NMI molarities to prepare a series of PtCl4–2DM inks with high colloidal stability. By adopting the PtCl4–graphene oxide ink, various Pt micro-structures with replicated topographies are synthesized with accurate control of grain sizes and porosities. 相似文献
146.
El-Moursy Ali A. Sibai Fadi N. Rehman Jahanzeb Gouda Omar M. Gaber Abdelrahman T. Khedr Ahmed M. 《Wireless Personal Communications》2022,124(2):1525-1555
Wireless Personal Communications - The development of Smart Home Controllers has seen rapid growth in recent years, especially for smart devices, that can utilize the Internet of Things (IoT).... 相似文献
147.
Syed Ali Fathima S. J. Lalitha T. Ahmad Faiyaz Karthick S. 《Wireless Personal Communications》2022,124(2):1815-1839
Wireless Personal Communications - Wireless Underground Networks comprise the ability to constantly monitor several physical parameters such as ground temperature, water level and soil condition,... 相似文献
148.
Wireless Personal Communications - Software-defined networking (SDN) is widely perceived to simplify network management and monitoring. The introduction of the SDN model into wireless sensor... 相似文献
149.
Obeidat Huthaifa A. Ahmad Imran Rawashdeh Mohammad R. Abdullah Ali A. Shuaieb Wafa S. Obeidat Omar A. Abdallhameed Raed A. 《Wireless Personal Communications》2022,123(4):3463-3464
Wireless Personal Communications - 相似文献
150.
准确的内部温度估计对动力电池的安全使用至关重要,为了在线获取准确的电池内部温度,本文提出一种基于温度估计模型的ESO-UKF电池内部温度估计方法。其中温度估计模型由Bernardi生热模型与热路传热模型组成,生热模型中端电压由神经网络获取,传热模型参数由递推最小二乘法辨识得到;该算法利用温度估计模型的离散状态空间描述,提出ESO-UKF进行电池内部温度的在线估计,将影响估计精度的传感器偏差视为扩展状态与原状态一起估计,实现了对不确定状态的估计;测试验证表明该算法的估计误差小于1℃,能够实现多工况下内部温度的在线估计,估计精度高、适应性强。 相似文献