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211.
The electron localization function (ELF) has been proven so far a valuable tool to determine the location of electron pairs. Because of that, the ELF has been widely used to understand the nature of the chemical bonding and to discuss the mechanism of chemical reactions. Up to now, most applications of the ELF have been performed with monodeterminantal methods and only few attempts to calculate this function for correlated wave functions have been carried out. Here, a formulation of ELF valid for mono- and multiconfigurational wave functions is given and compared with previous recently reported approaches. The method described does not require the use of the homogeneous electron gas to define the ELF, at variance with the ELF definition given by Becke. The effect of the electron correlation in the ELF, introduced by means of configuration interaction with singles and doubles calculations, is discussed in the light of the results derived from a set of atomic and molecular systems. 相似文献
212.
Güell M Matito E Luis JM Poater J Solà M 《The journal of physical chemistry. A》2006,110(40):11569-11574
Our research group has recently defined two new aromaticity indexes based on the analysis of electron delocalization in aromatic species using the quantum theory of atoms-in-molecules. One of these indexes is the para-delocalization index (PDI) that measures the electronic delocalization between para-related carbon atoms in six-membered rings. In this paper, we show that this index can be partitioned into individual molecular orbital contributions. We have applied this PDI decomposition to several polycyclic aromatic hydrocarbons showing that this partitioning provides new insight into the origin of aromaticity. 相似文献
213.
The aim of our work is to develop optimal dielectric composite structures with specific qualities. The task is to design interfaces of given material components such that the originated structure attains certain optical properties. Propagation of the electromagnetic waves in the composite is described by the Helmholtz equation. Success of the structure is enumerated by the objective function which is to be minimized. Interfaces of the given materials are parametrized by the cubic B–spline curves. The design variables are afterwards the positions of B–spline control points. For objective function evaluation one forward computation of the Helmholtz equation is needed. To get the sensitivity of the objective function we solve the backward (adjoint) equation. (© 2008 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim) 相似文献
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Daniel Fernández Jordi Madrenas Eduard Alarcón 《Analog Integrated Circuits and Signal Processing》2013,74(1):227-238
In this paper we present an asynchronous finite-state machine digital controller co-integrated with an on-chip non-inverting buck-boost power converter with dynamic signal-tracking capabilities. The mostly-digital controller functionally implements a non-PWM zone-wise control law through asynchronous circuitry, thus exhibiting self-timed minimum latency and ultra low power operation due to gate switching activity. Experimental results on a 0.35 μm CMOS technology demonstrate an efficiency up to 80 % with a switching frequency of 2.86 MHz. 相似文献
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Ignacio Llatser Christian Kremers Albert Cabellos-Aparicio Josep Miquel Jornet Eduard Alarcón Dmitry N. Chigrin 《Photonics and Nanostructures》2012,10(4):353-358
The scattering of terahertz radiation on a graphene-based nano-patch antenna is numerically analyzed. The extinction cross section of the nano-antenna supported by silicon and silicon dioxide substrates of different thickness are calculated. Scattering resonances in the terahertz band are identified as Fabry–Perot resonances of surface plasmon polaritons supported by the graphene film. A strong tunability of the antenna resonances via electrostatic bias is numerically demonstrated, opening perspectives to design tunable graphene-based nano-antennas. These antennas are envisaged to enable wireless communications at the nanoscale. 相似文献
219.
Eduard N. Tsoy Sadulla Sh. Tadjimuratov Fatkhulla Kh. Abdullaev 《Optics Communications》2012,285(16):3441-3444
Linear and nonlinear localized modes of a slab waveguide with distributed gain and loss are studied. The structure is an optical analog of parity-time symmetric potentials in quantum mechanics. Such waveguide structures support stable localized modes. The explicit equation for the propagation constant of linear modes is obtained. The existence of stable nonlinear modes in such waveguides is demonstrated. Bend losses in such structures are analyzed. 相似文献
220.
MB Serrano-Santos E Llobet VC Ozalp T Schäfer 《Chemical communications (Cambridge, England)》2012,48(81):10087-10089
The dimension of the conformational changes of DNA-aptamers which can be used as stimulus-responsive gate-keepers in controlled delivery nanodevices has been determined by acoustic wave-based sensors upon molecular recognition of a small-sized target, adenosine-5'-monophosphate (AMP). 相似文献