光脉冲在半导体中非线性传输特性的时域和频域分析

本文从理论上研究了半导体非共振透明区光脉冲非线性传输的时域和频域行为,并对应用自由载流子非线性折射效应来构造非线性方向耦合器的可能性进行了分析。     

Li+和稀土离子共掺ZrO2上转换发光特性

采用溶胶-凝胶(Sol-gel)法制备了Li+/Er3+/Yb3+三掺ZrO2纳米晶粉末.对纳米晶粉末样品进行了XRD检测,表明Li+掺入并没有改变晶体结构.在室温下用980 nm激光研究了烧结温度为800℃样品的上转换发光特性,掺入Li+后纳米晶粉末样品红绿光波段的荧光强度都有很好的增强.通过对激发功率与荧光强度的关...     

啁啾脉冲频域干涉仪相位重建方法的理论研究

理论研究了啁啾脉冲频域干涉仪的时域相移重建技术,对于接近实际的频谱干涉条纹,分别采用傅里叶变换和小波变换的方法完成了时域相位扰动信号的重建。傅里叶变换方法产生的重建误差受到滤波参数的影响,相对而言,小波变换方式解谱过程中,不需要进行特意的滤波操作,从而避免了重建结果存在误差不确定性的问题。     

The theory and experiment of solute migration caused by excited state absorptions

Nonsymmetrical transition from reverse-saturable absorption (RSA) to saturable absorption (SA) caused by excited state absorption induced mass transport of the CuPcTs dissolved in dimethyl sulfoxide is observed in an open aperture Z-scan experiment with a 21-ps laser pulse. The nonsymmetrical transition from RSA to SA is ascribed neither to saturation of excited state absorption nor to thermal induced mass transport, the so-called Soret effect. In our consideration, strong nonlinear absorption causes the rapid accumulation of the non-uniform kinetic energy of the solute molecules. The non-uniform kinetic field in turn causes the migration of the solute molecules. Additionally, an energy-gradient-induced mass transport theory is presented to interpret the experimental results, and the theoretical calculations are also taken to fit our experimental results.     

飞秒光纤激光自相关谱畸变产生机理的研究

用自相关法测量超短脉冲的实验中,随着输入脉冲的能量、脉冲形状、分束比以及延迟时间的改变,在一定的条件下可得到产生畸变的自相关谱.畸变的自相关谱会使准确估算脉冲宽度产生偏差.文中从理论和实验两方面,着重研究了自相关信号产生畸变的物理机制,用数值计算的方法分析了参考信号和延迟信号的分束比、线性啁啾、脉冲形状对相关谱产生畸变的影响.理论分析结果和实验测量结果相吻合,验证了理论的正确性.     

NONLINEAR REFRACTION IN MULTILEVEL MOLECULAR SYSTEMS

The intensity-dependent nonlinear refraction phenomena in a non-resonant multilevel molecular system is studied using rate equations in steady state, including saturable refraction, reverse saturable refraction, and the turnover between these two effects. The relationship between the refraction saturation and the optical Kerr effect is also discussed.     

含光学非线性介质薄膜对表面等离子波的影响

表面等离子体是在金属和电介质交界面上所形成的电荷层,在电磁波的激励下表面等离子体会发生共振现象,影响电磁波的传播。为了拓宽表面等离子体共振技术的应用,研究了多层纳米膜结构中的表面等离子体共振,并且根据Fresnel公式和Walpita描述的矩阵方法,计算了光在含有非线性介质的多层纳米膜中传播时的反射率R,其中非线性介质具有光克尔效应和双光子吸收。应用Matlab软件,画出了反射系数R和入射角θ之间的关系曲线。进一步讨论了光学非线性对表面等离子体共振角谱的影响,其中光强在0.5×1012W/m2到1.5×1012W/m2的范围内,Rmin随着入射光强的增加而变大,而θp随入射光强的增加而呈递减的趋势。     

有机分子系统中反饱和吸收向饱和吸收转化的条件

由多能级稳态速率方程导出反饱和喟收向饱少吸收转化的能级参数条件和阈值光强，并与动态理论导出的结果作了比较，讨论了阈值光强在光限幅材料设计中的应用。     

Measurement of Ultrashort Laser Pulse Width in a Wide Spectrum Range Using Dimethyl Sulfoxide by Optical Kerr Effect Technique

We illustrate that applying the optical Kerr effect technique to dimethyl sulfoxide （DMSO） can determine the width of laser pulses in a wide spectrum range that is transparent. Different from many other simple molecular liquids, such CS2, and toluene, DMSO responds to both 130 fs 800 nm laser pulses and 248 fs 400 nm laser pulses with electronic motions only. Therefore, the observed signal as a function of time reflects the temporal distribution of the intensity. We verify our illustration by both the autocorrelation technique and spectra analysis.     

有机分子系统非线性折射的类型

从分子系统的微观机制出发,采用单重态四能级模型讨论非线性折射随光强的变化情况,分析了非线性折射的各种形式产生的条件,定义了非线性折射的饱和现象、反饱和现象相互转化的阈值光强.发现了非线性折射率随光强发生正负变化的现象.