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TIME DECAY BEHAVIOR OF FULLERENE-C60 STUDIED BY TIME-RESOLVED PHOTOLUMINESCENCE 总被引:1,自引:0,他引:1
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The time-resoved photoluminescence spectra of C60 have been studied from toluence solution at room temperature and from thin film at both room temperature and 77K. A photoluminescence peak at about 730nm was detected from solution at room temperature and film at 77K, in which lifetimes waz determined to be 1.1 and 0.9ns, respectively. At room temperature, the photoluminescence peak of thin film shifted to 740 nm with fast decay behavior which was fitted well to a double-exponential lifetimes with τ1 = 0.087ns, τ2= 0.68 ns. Two relaxation mechanisms are given tentatively in explaining this phenomenon. 相似文献
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Using Nd:YAG second harmonic pulse (100 ps), the optical storage proper-ties of two novel polyesters, poly [4'-bis (N, N-oxyethylene) imino-4-nitroazobenzene suc-cinyl] and poly [2'-chloro-4'-bis (N, N-oxyethylene) iminth-4-nitroazobenzene succiny] havebeen studied by multiwave mixing. The high-order diffractions of the orientation gratingsinduced by anisotropy via the reorientation of nitroazobenzene groups and optical infor-mation storage with long-term stability have been realized by multiwave mixing in theirfilms. Up to 3rd order forward diffraction was detected in two wave mixing, while up to 4thorder backward diffraction was observed in degenerated four wave mixing. The recordingmechanism was explained by the trans-cis-trans isomerization cycles of azobenzene groups.The isomerization of these azobenzene groups probably undergoes with inversion mecha-nism under the experimental conditions. The information recorded in these films has beenkept for more than 6 months. 相似文献
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STUDIES ON THE DYNAMICS OF OPTICAL BISTABILITY SWITCHING IN THE INTERNAL FABRY-PEROT CAVITY WITH A CdSxSe1-x-DOPED GLASS CHANNEL WAVEGUIDE
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We report the optical bistability in CdSxSe1-x-doped glass channel waveguide with rise and fall times of about 24 and 30ps, respectively, in bistable switching by means of fiber coupling input with a power of about 3mW. The third-order nonlinear susceptibility (x(3)) of CdSxSe1-x-doped glass is estimated experimentally to be 1.8×10-9 esu. The high speed switching and the value of x(1) show that the optical bistability is caused by an optical nonlinearity which can be attributed to the band-filling effect. 相似文献