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11.
Chen DT Weeks ER Crocker JC Islam MF Verma R Gruber J Levine AJ Lubensky TC Yodh AG 《Physical review letters》2003,90(10):108301
We demonstrate how tracer microrheology methods can be extended to study submicron scale variations in the viscoelastic response of soft materials; in particular, a semidilute solution of lambda-DNA. The polymer concentration is depleted near the surfaces of the tracer particles, within a distance comparable to the polymer correlation length. The rheology of this microscopic layer alters the tracers' motion and can be precisely quantified using one- and two-point microrheology. Interestingly, we found this mechanically distinct layer to be twice as thick as the layer of depleted concentration, likely due to solvent drainage through the locally perturbed polymer structure. 相似文献
12.
John D. Weeks 《Journal of statistical physics》2003,110(3-6):1209-1218
By combining the upper and lower bounds to the free energy as given by the Gibbs inequality for two systems with the same intermolecular interactions but with external fields differing from each other only in a finite region of space , we show that the corresponding equilibrium densities must also differ from each other somewhere in . We note that the basic equations of density functional theory arise naturally from a simple rearrangement and reinterpretation of the terms in the upper bound Gibbs inequality for such systems and briefly discuss some of the complications that occur when the intermolecular interactions of the two systems also differ. 相似文献
13.
We derive an exact equation for density changes induced by a general external field that corrects the hydrostatic approximation where the local value of the field is adsorbed into a modified chemical potential. Using linear response theory to relate density changes self-consistently in different regions of space, we arrive at an integral equation for a hard sphere fluid that is exact in the limit of a slowly varying field or at low density and reduces to the accurate Percus-Yevick equation for a hard core field. This and related equations give accurate results for a wide variety of fields. 相似文献
14.
In important early work, Stell showed that one can determine the pair correlation function h(r) of the hard-sphere fluid for all distances r by specifying only the tail of the direct correlation function c(r) at separations greater than the hard-core diameter. We extend this idea in a very natural way to potentials with a soft repulsive core of finite extent and a weaker and longer ranged tail. We introduce a new continuous function T(r) which reduces exactly to the tail of c(r) outside the (soft) core region and show that both h(r) and c(r) depend only on the out projection of T(r): i.e., the product of the Boltzmann factor of the repulsive core potential times T(r). Standard integral equation closures can thus be reinterpreted and assessed in terms of their predictions for the tail of c(r) and simple approximations for its form suggest new closures. A new and very efficient variational method is proposed for solving the Ornstein–Zernike equation given an approximation for the tail of c. Initial applications of these ideas to the Lennard-Jones and the hard-core Yukawa fluid are discussed. 相似文献
15.
Weeks D.A. Weldon W.F. Zowarka R.C. 《IEEE transactions on plasma science. IEEE Nuclear and Plasma Sciences Society》1989,17(3):403-408
The authors review three popular loss models currently used at CEM-UT (Center for Electromechanics at the University of Texas at Austin) in modeling EM (electromagnetic) launchers: friction, ablation, and armature drag. In experiments at currents below 500 kA using existing railgun design, the friction model alone was acceptable in predicting performance. In an experiment incorporating a railgun structure modified for higher stiffness and a measured peak railgun current of 700 kA, the effects of each of the loss models were compared to the measured results, and the greatest success at predicting the final projectile velocity and exit time occurred using the velocity-dependent friction model. It is believed that reducing frictional losses and plasma leakage will be instrumental in achieving velocities greater than 6 km/s 相似文献
16.
17.
H. W. Gonell A. Blackie N. E. Edlefsen E. Kahane S. W. Parr P. F. Thompson C. W. Correns J. R. Bailey R. E. Remington J. F. Mc Clendon H. von Kolnitz R. G. Turner Minna Z. Weeks G. P. Baxter E. R. Bishop C. B. Dollins H. Starke K. Højendahl R. Jacquemain E. A. Werner E. André A. Oká H. T. S. Britton und B. M. Wilson 《Fresenius' Journal of Analytical Chemistry》1934,98(7-8):259-266
Ohne Zusammenfassung 相似文献
18.
Metal/superconductor/semiconductor (Ag/Hg-1212/CdSe) hetero-nanostructures have been fabricated using pulse-electrodeposition
technique and are characterized by X-ray diffraction (XRD), full-width at half-maximum (FWHM) and scanning electron microscopy
(SEM) studies. The junction capacitance of Ag/Hg-1212, Hg-1212/CdSe and Ag/Hg-1212/CdSe heterojunctions is measured in dark
and under laser irradiation at room temperature. The nature of the junction formed and built-in-junction potentials were determined.
The increase in carrier concentration across the junction due to photo-irradiation has been observed. 相似文献
19.
One of the innovative technological directions for the high-temperature superconductors has been persued by fabricating the
heteroepitaxial multilayer structures such as superconductor-semiconductor heterostructures. In the present investigation,
metal/superconductor/semiconductor (Ag/Tl-2223/CdSe) hetero-nanostructures have successfully been fabricated using dc electrodeposition
technique and were characterized by X-ray diffraction (XRD), full-width at half-maximum (FWHM) and scanning electron microscopy
(SEM) studies. The measurement of junction capacitance as a function of biasing voltage was used for the estimation of junction
built-in-potential (V
D) and to study the charge distribution in a heterojunction. The Mott-Schottky plots were measured for each junction in dark
and under the photo-irradiation. The effect of laser irradiation on C-V characteristics of hetero-nanostructure has been studied. 相似文献
20.
Semicrystalline polymers generally exhibit moduli well below their theoretical limit due to chain folding and to lack of crystal alignment. Modulus increases attainable through standard drawing procedures are limited by sample fracture before large draw ratios are reached. Using an Instron capillary rheometer which allowed a draw ratio of > 300, transparent polyethylene strands of unusually high c-axis orientation have been produced by a combination of pressure and shear. The virtually perfect crystalline orientation and evidence for extended chains confirm that a significant improvement in modulus can be realized by this technique. The dynamic tensile storage modulus was measured by Vibron over the temperature range ?160°C to +120°C. Room-temperature moduli were 7 × 1011 dyne/cm2, higher than any reported values for drawn polyethylene. Values also remained above 1011 dyne/cm2 even at 120°C. The moduli and morphological data have been related by a model consisting of an extended-chain component in paralled with a conventional drawn morphology. Experimental and calculated moduli are compared and related to available theory. 相似文献