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101.
(--)-Muricatacin, a potent cytotoxic (4R,5R)-5-hydroxyheptadecan-4-olide, has been synthesized through alpha-C--H hydroxyalkylation and alpha'-C--H oxidation of tetrahydrofuran. This study presents a novel method for C--H bond functionalization as a means for preparing gamma-(hydroxyalkyl)-gamma-butyrolactones. 相似文献
102.
Murakami T Nishikiori T Nohira T Ito Y 《Journal of the American Chemical Society》2003,125(2):334-335
Ammonia was successfully synthesized by using a new electrochemical reaction with high current efficiency at atmospheric pressure and at lower temperatures than the Haber-Bosch process. In this method, nitride ion (N3-), which is produced by the reduction from nitrogen gas at the cathode, is anodically oxidized and reacts with hydrogen to produce ammonia at the anode. 相似文献
103.
M. Nurhuda A. Suda M. Kaku K. Midorikawa 《Applied physics. B, Lasers and optics》2007,89(2-3):209-215
We present a study on the optimization of multi-mJ spectral broadening in neon-filled hollow fibers using pressure gradients.
It is found that the intensity of the laser pulse at the entrance of the hollow fiber should be below or at the level where
multi-photon ionization (MPI) starts to occur. If the intensity is higher than the threshold value for MPI, ionization can
significantly reduce the throughput efficiency. The extension of the scheme to a terawatt power level is also addressed.
PACS 42.65.Re; 42.65.Jx; 42.65.k 相似文献
104.
H. Mardanpour H. R. Amir-Ahmadi A. Deltuva K. Itoh N. Kalantar-Nayestanaki T. Kawabata H. Kuboki Y. Maeda J. G. Messchendorp S. Sakaguchi H. Sakai N. Sakamoto Y. Sasamoto M. Sasano K. Sekiguchi K. Suda Y. Takahashi T. Uesaka H. Witała K. Yako 《The European Physical Journal A - Hadrons and Nuclei》2007,31(3):383-391
High-precision vector and tensor analyzing powers of elastic deuteron-proton ( d + p) scattering have been measured at intermediate energies to investigate effects of three-nucleon forces. Angular distributions
in the range of 70°-120° in the center-of mass frame for incident-deuteron energies E
d
lab = 130 and 180 MeV were obtained using the RIKEN facility. The beam polarization was unambiguously determined by measuring
the ^12C (d, α)^10B(2+) reaction at 0°. Results of the measurements are compared with state-of-the-art three-nucleon calculations. The present modeling of nucleon-nucleon
forces and its extension to the three-nucleon system is not sufficient to describe the high-precision data consistently and
requires, therefore, further investigation. 相似文献
105.
Zhi-Peng Li Toshiyuki Mori Jin Zou John Drennan 《Journal of solid state chemistry》2011,184(9):2458-2461
Analytical transmission electron microscopy, in particular with the combination of energy dispersive X-ray spectroscopy (EDX) and electron energy-loss spectroscopy (EELS), has been performed to investigate the microstructure and microchemistry of the interfacial region between the cathode (La0.6Sr0.4Co0.8Fe0.2O3, LSCF) and the electrolyte (Gd-doped ceria, GDC). Two types of diffusions, mutual diffusion between cathode and electrolyte as well as the diffusion along grain boundaries, have been clarified. These diffusions suggest that the chemical stability of LSCF and GDC are not as good as previously reported. The results are more noteworthy if we take into consideration the fact that such interdiffusions occur even during the sintering process of cell preparation. 相似文献
106.
107.
A fundamental research is carried out into convergence and stability properties of IMEX (implicit–explicit) Runge–Kutta schemes applied to reaction–diffusion equations. It is shown that a fully discrete scheme converges if it satisfies certain conditions using a technique of the B-convergence analysis, developed by Burrage, Hundsdorfer and Verwer in 1986. Stability of the schemes is also examined on the basis of a scalar test equation, proposed by Frank, Hundsdorfer and Verwer in 1997. 相似文献
108.
Toshiyuki Sugawa 《Transactions of the American Mathematical Society》2001,353(9):3603-3615
In this note, we show, in a quantitative fashion, that the limit set of a non-elementary Kleinian group is uniformly perfect if the quotient orbifold is of Lehner type, i.e., if the space of integrable holomorphic quadratic differentials on it is continuously contained in the space of (hyperbolically) bounded ones. This result covers the known case when the group is analytically finite. As applications, we present estimates of the Hausdorff dimension of the limit set and the translation lengths in the region of discontinuity for such a Kleinian group. Several examples will also be given.
109.