Stable generation of high-order harmonics of femtosecond laser radiation from laser produced plasma plumes at 1 kHz pulse repetition rate

We present a method for the creation of stable weakly ionized plasmas from laser ablation of solid targets using a 1 kHz pulse repetition rate laser, which can be used for stable high-order harmonic generation from plasma plumes. The plasma plumes were generated from cylindrical rotating targets. Without target rotation the intensity of harmonics in the 40-80 nm range drops by more than one order of magnitude during less than 10(3) shots, while, with rotation of the target at typically 30 revolutions per minute, stable emission of high-order harmonics from aluminum plasma plumes with variation of less than 10% was maintained for >10(6) laser shots.     

Comparing contact and dipolar interactions in a Bose-Einstein condensate

We have measured the relative strength epsilon dd of the magnetic dipole-dipole interaction compared with the contact interaction in a dipolar chromium Bose-Einstein condensate. We analyze the asymptotic velocities of expansion of the condensate with different orientations of the atomic magnetic moments. By comparing the experimental results with numerical solutions of the hydrodynamic equations for dipolar condensates, we obtain epsilon dd = 0.159+/-0.034. We use this result to determine the s-wave scattering length a = (5.08+/-1.06 x 10(-9)) m = (96+/-20) a0 of 52Cr. This is fully consistent with our previous measurements on the basis of Feshbach resonances and therefore confirms the validity of the theoretical approach used to describe the dipolar Bose-Einstein condensate.     

General entanglement scaling laws from time evolution

We establish a general scaling law for the entanglement of a large class of ground states and dynamically evolving states of quantum spin chains: we show that the geometric entropy of a distinguished block saturates, and hence follows an entanglement-boundary law. These results apply to any ground state of a gapped model resulting from dynamics generated by a local Hamiltonian, as well as, dually, to states that are generated via a sudden quench of an interaction as recently studied in the case of dynamics of quantum phase transitions. We achieve these results by exploiting ideas from quantum information theory and tools provided by Lieb-Robinson bounds. We also show that there exist noncritical fermionic systems and equivalent spin chains with rapidly decaying interactions violating this entanglement-boundary law. Implications for the classical simulatability are outlined.     

Statistical mechanics of combinatorial auctions

Combinatorial auctions are formulated as frustrated lattice gases on sparse random graphs, allowing the determination of the optimal revenue by methods of statistical physics. Transitions between computationally easy and hard regimes are found and interpreted in terms of the geometric structure of the space of solutions. We introduce an iterative algorithm to solve intermediate and large instances, and discuss competing states of optimal revenue and maximal number of satisfied bidders. The algorithm can be generalized to the hard phase and to more sophisticated auction protocols.     

Nonlinear refractive indices of nonlinear liquids: wavelength dependence and influence of retarded response

We use liquid-filled capillary fibers with different core diameters to precisely characterize the nonlinear refractive index of the highly nonlinear liquids carbon disulfide, nitrobenzene, and toluene. We present measurements with two different femtosecond pump sources at wavelengths of 1032 and 1560 nm. The large nonlinearity of the liquids results from the retarded nonlinear optical response of the liquid molecules which includes a strong non-instantaneous contribution due to molecular reorientation. The nonlinear refractive index of the liquids is determined by fitting numerical simulations based on solving the generalized nonlinear Schrödinger equation including retarded response to the measured broadened output spectra. Our work is important for the novel field of near- and mid-IR supercontinuum generation in liquid-core optical fibers.     

Gold nanoparticle growth on self-assembled monolayers of ferrocenyl-substituted terpyridine on graphite

In this contribution we demonstrate that densely packed gold nanoparticles can be grown by Volmer–Weber mode on ferrocenyl functionalized terpyridine (FcTerp) on graphite. FcTerp forms highly ordered and dense self-assembled monolayers (SAMs) on graphite which significantly reduces the diffusion length of gold atoms and increases the sticking coefficient compared to bare graphite. Both effects lead to an increased nucleation and thus, to the growth of densely packed gold nanoparticles with diameters in the nanometer range. The optical properties of the nanoparticles as well as their morphology and the structure of the SAMs were characterized by optical extinction spectroscopy and scanning tunneling microscopy.     

Integrated waveguide sensor utilizing organic photodiodes

We present a novel optical sensor platform, combining monolithically integrated ring‐like sensor waveguides together with ring‐shaped thin‐film organic photodiodes (OPDs) on one substrate. The OPDs serve as integrated light detectors, simplifying the detection system by minimizing the number of required optical components. The waveguide structures, including a means of coupling light in and out of the waveguides, serve as sensing elements. The functionality of the concept is demonstrated by an integrated carbon dioxide sensor, utilizing absorbance as sensing principle. The integrated optical sensor platform is suitable for the parallel detection of multiple parameters in a single sensor chip using sensor arrays. (© 2011 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

Spallation neutron production and the current intra-nuclear cascade and transport codes

A recent renascent interest in energetic proton-induced production of neutrons originates largely from the inception of projects for target stations of intense spallation neutron sources, like the planned European Spallation Source (ESS), accelerator-driven nuclear reactors, nuclear waste transmutation, and also from the application for radioactive beams. In the framework of such a neutron production, of major importance is the search for ways for the most efficient conversion of the primary beam energy into neutron production. Although the issue has been quite successfully addressed experimentally by varying the incident proton energy for various target materials and by covering a huge collection of different target geometries --providing an exhaustive matrix of benchmark data-- the ultimate challenge is to increase the predictive power of transport codes currently on the market. To scrutinize these codes, calculations of reaction cross-sections, hadronic interaction lengths, average neutron multiplicities, neutron multiplicity and energy distributions, and the development of hadronic showers are confronted with recent experimental data of the NESSI collaboration. Program packages like HERMES, LCS or MCNPX master the prevision of reaction cross-sections, hadronic interaction lengths, averaged neutron multiplicities and neutron multiplicity distributions in thick and thin targets for a wide spectrum of incident proton energies, geometrical shapes and materials of the target generally within less than 10% deviation, while production cross-section measurements for light charged particles on thin targets point out that appreciable distinctions exist within these models. Received: 22 May 2001 / Accepted: 3 September 2001     

Fiber‐based light sources for biomedical applications of coherent anti‐Stokes Raman scattering microscopy

During the past decade coherent anti‐Stokes Raman scattering (CARS) microscopy has evolved to one of the most powerful imaging techniques in the biomedical sciences, enabling the label‐free visualization of the chemical composition of tissue in vivo in real time. While the acquisition of high‐contrast images of single cells up to large tissue sections enables a wide range of medical applications from routine diagnostics to surgical guidance, to date CARS imaging is employed in fundamental research only, essentially because the synchronized multiple wavelength pulsed laser sources required for CARS microscopy are large, expensive and require regular maintenance. Laser sources based on optical fibers can overcome these limitations combining highest efficiency and peak powers with an excellent spatial beam profile and thermal stability. In this review we summarize the different fiber‐based approaches for laser sources dedicated to coherent Raman imaging, in particular active fiber technology and passive fiber‐based frequency conversion processes, i.e. supercontinuum generation, soliton self‐frequency shift and four‐wave mixing. We re‐evaluate the ideal laser parameters for CARS imaging and discuss the suitability of different laser concepts for turn‐key operation required for routine application in clinics.

     

Electron diffraction self-imaging of molecular fragmentation in two-step double ionization of water

We doubly ionize H(2)O by single photon absorption at 43 eV leading to H(+) + OH(+). A direct double ionization and a sequential process in which single ionization is followed by rapid dissociation into a proton and an autoionizing OH(*) are identified. The angular distribution of this delayed autoionization electron shows a preferred emission in the direction of the emitted proton. From this diffraction feature we obtain internuclear distances of 700 to 1100 a.u. at which the autoionization of the OH(*) occurs. The experimental findings are in line with calculations of the excited potential energy surfaces and their lifetimes.