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S. Anders M.G. Blamire F.-Im. Buchholz D.-G. Crété R. Cristiano P. Febvre L. Fritzsch A. Herr E. Il’ichev J. Kohlmann J. Kunert H.-G. Meyer J. Niemeyer T. Ortlepp H. Rogalla T. Schurig M. Siegel R. Stolz E. Tarte H.J.M. ter Brake A.B. Zorin 《Physica C: Superconductivity and its Applications》2010,470(23-24):2079-2126
94.
Brugnera L Frank F Hoffmann DJ Torres R Siegel T Underwood JG Springate E Froud C Turcu EI Tisch JW Marangos JP 《Optics letters》2010,35(23):3994-3996
We demonstrate enhancement by 1 order of magnitude of the high-order harmonics generated in argon by combining a fundamental field at 1300 nm (10(14) W cm(-2)) and its orthogonally polarized second harmonic at 650 nm (2 × 10(13) W cm(-2)) and by controlling the relative phase between them. This extends earlier work by ensuring that the main effect is the combined field steering the electron trajectory with negligible contribution from multiphoton effects compared to the previous schemes with 800/400 nm fields. We access a broad energy range of harmonics (from 20 eV to 80 eV) at a low laser intensity (far below the ionization saturation limit) and observe deep modulation of the harmonic yield with a period of π in the relative phase. Strong field theoretical analysis reveals that this is principally due to the steering of the recolliding electron wave packet by the two-color field. Our modeling also shows that the atto chirp can be controlled, leading to production of shorter pulses. 相似文献
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Dell'Acqua-Bellavitis LM Siegel RW 《Langmuir : the ACS journal of surfaces and colloids》2008,24(3):957-964
The field of research focused on the synthesis of micro- and nanoparticles has not yet conclusively addressed the challenges presented by the hierarchical control of surface topography. An established approach to hierarchical multicomposite nanostructured particles is based on template-directed synthesis, while spectacular advances have been reached in nanoparticle fabrication based on a variety of physicochemical processes. These results exemplify an additive route to hierarchical control, where multiple layers are stacked onto each other or where discretely identifiable particles are assembled into a larger spherical conglomerate. We present here a new strategy for the synthesis of micro- and nanoparticles, which we refer to as "textured isomorphic synthesis", that uses only the toolbox of inorganic chemistry coupled to the physics of cavitation, viscous fingering, and bubble nucleation. The results illustrate a topological route to hierarchical control of particle topography where dimples or holes are deterministically introduced on a planar substrate later transformed into isomorphic hollow spherical micro- and nanostructures. 相似文献
97.
Xiao W Passerone D Ruffieux P Aït-Mansour K Gröning O Tosatti E Siegel JS Fasel R 《Journal of the American Chemical Society》2008,130(14):4767-4771
Corannulene (COR) buckybowls were proposed as near ideal hosts for fullerene C60, but direct complexation of C60 and COR has remained a challenge in supramolecular chemistry. We report the formation of surface-supported COR-C60 host-guest complexes by deposition of C60 onto a COR lattice on Cu(110). Variable-temperature scanning tunneling microscopy studies reveal two distinctly different states of C60 on the COR host lattice, with different binding energies and bowl-ball separations. The transition from a weakly bound precursor state to a strongly bound host-guest complex is found to be thermally activated. Simple model calculations show that this bistability originates from a subtle interplay between homo- and heteromolecular interactions. 相似文献
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