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Irwin Oppenheim 《Journal of statistical physics》2006,122(2):371-372
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High‐resolution high‐performance liquid chromatography with electrospray ionization mass spectrometry and tandem mass spectrometry characterization of a new isoform of human salivary acidic proline‐rich proteins named Roma‐Boston Ser22(Phos) → Phe variant 下载免费PDF全文
Na Tian Tiziana Cabras Irene Messana Eva J. Helmerhorst Frank G. Oppenheim Massimo Castagnola 《Journal of separation science》2014,37(14):1896-1902
During a survey of human saliva by a top‐down reversed‐phase high‐performance liquid chromatography with electrospray ionization mass spectrometry approach, two proteins eluting at 27.4 and 28.4 min, with average masses of 15 494 ± 1 and 11 142 ± 1 Da, were detected in a subject from Boston. The Δmass value (4352 Da) of the two proteins was similar to the difference in mass values between intact (150 amino acids, [a.a.]) and truncated acidic proline‐rich proteins (aPRPs; 106 a.a.) suggesting an a.a. substitution in the first 106 residues resulting in a strong reduction in polarity, since under the same experimental conditions aPRPs eluted at ~22.5 min (intact) and 23.5 min (truncated forms). Manual inspection of the high‐resolution high‐performance liquid chromatography with electrospray ionization tandem mass spectra of the truncated isoform showed the replacement of the phosphorylated Ser‐22 in PRP‐3 with a Phe residue. Inspection of the tandem mass spectra of the intact isoform confirmed the substitution, which is allowed by the code transition TCT→TTT and is in agreement with the dramatic increase in elution time. The isoform was also detected in two other subjects, one from Boston (unrelated to the previous) and one from Rome. For this reason we propose to name this variant PRP‐1 (PRP‐3) RB (Roma‐Boston) Ser22(phos)→Phe. 相似文献
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Horodecki M Horodecki K Horodecki P Horodecki R Oppenheim J Sen De A Sen U 《Physical review letters》2003,90(10):100402
A new paradigm for distributed quantum systems where information is a valuable resource is developed. After finding a unique measure for information, we construct a scheme for its manipulation in analogy with entanglement theory. In this scheme, instead of maximally entangled states, two parties distill local states. We show that, surprisingly, the main tools of entanglement theory are general enough to work in this opposite scheme. Up to plausible assumptions, we show that the amount of information that must be lost during the protocol of concentration of local information can be expressed as the relative entropy distance from some special set of states. 相似文献
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We study the influence of boundaries on the equal-time thermal correlations in a three-dimensional fluid maintained under a constant temperature gradient. Within the confines of the model for an idealized fluid bounded by two infinite, parallel walls, we show that it is crucial to retain the unbounded spatial components in the problem so that the solutions approach meaningful results as we move the walls infinitely far apart. In addition, we consider a composite system by including the dynamics of the walls, and we investigate the conditions for the relevant physical parameters under which the details of wall dynamics may be neglected by employing the simple boundary condition T=0. 相似文献