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591.
A new, mild, and efficient method has been developed for the synthesis of 2-substituted benzothiazoles via the intramolecular cyclization of thioformanilides by using hypervalent iodine reagents in CH2Cl2 at ambient temperature. The reaction proceeds via a thiyl radical in high yields to give the novel compound oxybis benzothiazole and is also amenable to generating combinatorial libraries of heterocyclic compounds by solid-phase synthesis. 相似文献
592.
Neutron resonance spin-echo spectroscopy was used to monitor the temperature evolution of the linewidths of transverse acoustic phonons in lead across the superconducting transition temperature over an extended range of the Brillouin zone. For phonons with energies below the superconducting energy gap, a linewidth reduction of maximum amplitude was observed below . The electron-phonon contribution to the phonon lifetime extracted from these data is in satisfactory overall agreement with ab initio lattice-dynamical calculations, but significant deviations are found. 相似文献
593.
Abazov VM Abbott B Abolins M Acharya BS Adams M Adams T Alexeev GD Alkhazov G Alton A Alverson G Alves GA Ancu LS Aoki M Arnoud Y Arov M Askew A Asman B Atramentov O Avila C BackusMayes J Badaud F Bagby L Baldin B Bandurin DV Banerjee S Barberis E Baringer P Barreto J Bartlett JF Bassler U Beale S Bean A Begalli M Begel M Belanger-Champagne C Bellantoni L Benitez JA Beri SB Bernardi G Bernhard R Bertram I Besançon M Beuselinck R Bezzubov VA Bhat PC Bhatnagar V Blazey G Blessing S Bloom K 《Physical review letters》2010,105(19):191802
We report the results of a search for R parity violating (RPV) interactions leading to the production of supersymmetric sneutrinos decaying into eμ final states using 5.3 fb-1 of integrated luminosity collected by the D0 experiment at the Fermilab Tevatron Collider. Having observed no evidence for production of eμ resonances, we set direct bounds on the RPV couplings λ311' and λ312 as a function of sneutrino mass. 相似文献
594.
We propose a mechanism where high entanglement between very distant boundary spins is generated by suddenly connecting two long Kondo spin chains. We show that this procedure provides an efficient way to route entanglement between multiple distant sites. We observe that the key features of the entanglement dynamics of the composite spin chain are well described by a simple model of two singlets, each formed by two spins. The proposed routing mechanism is a footprint of the emergence of a Kondo cloud in a Kondo system and can be engineered and observed in varied physical settings. 相似文献
595.
Tapas KuilaSaswata Bose Ananta Kumar MishraPartha Khanra Nam Hoon KimJoong Hee Lee 《Polymer Testing》2012,31(1):31-38
Dodecyl amine-modified graphene (DA-G)/linear low density polyethylene (LLDPE) nanocomposites were prepared through solution mixing. Field emission scanning electron microscopy analysis revealed homogeneous dispersions of graphene layers in the nanocomposites. X-ray diffraction analysis showed that the average crystallite size of the nanocomposites was increased. However, the % crystallinity was found to decrease due to the formation of a random interface. Dynamic mechanical analysis showed that the storage moduli of the nanocomposites were much higher than that of neat LLDPE. The nanocomposites were also more thermally stable than neat LLDPE. Isothermal thermogravimetry showed that homogeneously distributed graphene could act as a good inhibitor during thermal degradation of the nanocomposites. Differential scanning calorimetry showed that the crystallization temperature of the nanocomposites increased with increasing DA-G content. Thermomechanical analysis showed that the dimensional stability of the nanocomposites was significantly increased by the addition of the DA-G. The coefficients of thermal expansion decreased with increasing DA-G content. The oxygen and nitrogen permeability of the nanocomposites was lower than that of neat LLDPE. 相似文献
596.
We present some solutions of late time transition to an accelerating universe showing a quintessence or a de-Sitter era of
expansion at late time using Gauss-Bonnet interaction in a Jordan Brans-Dicke theory in FLRW spacetime. The Gauss-Bonnet term
yields an effective cosmological constant characterized by a de-Sitter era of late time expansion when the Gauss-Bonnet interaction
is equivalent with an ideal fluid. The quintessence era of late time expansion have been obtained assuming the evolution of
scalar field is a single valued function. The Chameleon mechanism shows that the correction to the Newton law could be small. 相似文献
597.
A. K. Pal I. Bose 《The European Physical Journal B - Condensed Matter and Complex Systems》2012,85(1):36
The transverse Ising Model (TIM) in one dimension is the simplest model which exhibits a quantum phase transition (QPT). Quantities
related to quantum information theoretic measures like entanglement, quantum discord (QD) and fidelity are known to provide
signatures of QPTs. The issue is less well explored when the quantum system is subjected to decoherence due to its interaction,
represented by a quantum channel, with an environment. In this paper we study the dynamics of the mutual information I(ρ
AB
), the classical correlations C(ρ
AB
) and the quantum correlations Q(ρ
AB
), as measured by the QD, in a two-qubit state the density matrix of which is the reduced density matrix obtained from the
ground state of the TIM in 1d. The time evolution brought about by system-environment interactions is assumed to be Markovian
in nature and the quantum channels considered are amplitude damping, bit-flip, phase-flip and bit-phase-flip. Each quantum
channel is shown to be distinguished by a specific type of dynamics. In the case of the phase-flip channel, there is a finite
time interval in which the quantum correlations are larger in magnitude than the classical correlations. For this channel
as well as the bit-phase-flip channel, appropriate quantities associated with the dynamics of the correlations can be derived
which signal the occurrence of a QPT. 相似文献
598.
Amrita Mandal Anindita Bose Sreemanta Mitra Anindya Datta Sourish Banerjee Dipankar Chakravorty 《Journal of magnetism and magnetic materials》2012
Nanoplates of NiS with thickness 0.6 nm were grown within the crystal channels of Na-4 mica. The thickness of the nanoplates is confirmed by atomic force microscopy. The nanocomposites exhibited multiferroic (both ferromagnetic and ferroelectric) behavior at room temperature. Ferromagnetism was adduced to an increase of surface defects as a result of the two-dimensional configuration of the sample. Ferroelectric behavior was explained as arising due to a small distortion in the crystal structure of NiS grown within the Na-4 mica channels. This was substantiated by the refined values of lattice constants as determined by profile matching of X-ray data by a computer program. A magnetodielectric effect was also observed in this nanocomposite with a change of 0.77% in the dielectric constant for a magnetic field of 0.6 T. 相似文献
599.
Abazov VM Abbott B Acharya BS Adams M Adams T Alexeev GD Alkhazov G Alton A Alverson G Alves GA Aoki M Arov M Askew A Asman B Atramentov O Avila C BackusMayes J Badaud F Bagby L Baldin B Bandurin DV Banerjee S Barberis E Baringer P Barreto J Bartlett JF Bassler U Bazterra V Beale S Bean A Begalli M Begel M Belanger-Champagne C Bellantoni L Beri SB Bernardi G Bernhard R Bertram I Besançon M Beuselinck R Bezzubov VA Bhat PC Bhatnagar V Blazey G Blessing S Bloom K Boehnlein A Boline D Boos EE 《Physical review letters》2012,108(2):021801
We present a search for pair production of doubly charged Higgs bosons in the processes qqˉ→H(++)H(--) decaying through H(±±)→τ(±)τ(±),μ(±)τ(±),μ(±)μ(±). The search is performed in ppˉ collisions at a center-of-mass energy of √s = 1.96 TeV using an integrated luminosity of up to 7.0 fb(-1) collected by the D0 experiment at the Fermilab Tevatron Collider. The results are used to set 95% C.L. limits on the pair production cross section of doubly charged Higgs bosons and on their mass for different H(±±) branching fractions. Models predicting different H(±±) decays are investigated. Assuming B(H(±±)→τ(±)τ(±))=1 yields an observed (expected) lower limit on the mass of a left-handed H(L)(±±) boson of 128 (116) GeV and assuming B(H(±±)→μ(±)τ(±))=1 the corresponding limits are 144 (149) GeV. In a model with B(H(±±)→τ(±)τ(±))=B(H(±±)→μ(±)τ(±))=B(H(±±)→μ(±)μ(±))=1/3, we obtain M(H(L)(±±))>130 (138) GeV. 相似文献
600.
The measurement of absorption, luminescence, and relative intensity of cerium and manganese emission during fluorescence, on single crystals of CaF2:(Ce+Mn), have been reported in this paper. The occurence of the absorption bands have been explained in the following manner: (i) 250 mu band due to the transfer transition from F? to2D, the excited state of Ce3+, (ii) 305 mμ band due to the characteristic transition of Ce3+ and (iii) 335 mμ band due to the perturbed level of the lattice. The emission bands have been explained like this, (i) 320 and 340 mμ bands due to the transitions of2D to2F5/2,7/2 levels of Ce3+ (ii) 380 and 440 mμ bands corresponding to the perturbed levels and (iii) 520 mμ band due to transfer of energy from cerium centres to manganese centres. The results of the present investigation indicate that energy transfer in this system occures not only from cerium to manganese centres but also from cerium to cerium and cerium to perturbed levels of the lattice. It has also been observed that energy transfer process is temperature dependent in this case. An energy level scheme is proposed to explain the transfer mechanism. 相似文献