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D. Rychel R. Gyufko B. van Krüchten M. Lahanas P. Singh C. A. Wiedner 《Zeitschrift für Physik A Hadrons and Nuclei》1987,326(4):455-461
Coulomb-nuclear interference in inelastic scattering of 35.4 MeVα-particles from the stable even Zr isotopes was studied. In the framework of a collective DWBA analysis isoscalar and electromagnetic transition rates for low lying 2+ and 3? states were derived. The experimentalB (E2) values are in good agreement with results obtained by purely electromagnetic methods. The deducedM n /M p ratios of the 2 1 + levels exhibit a surprisingly large increase with increasing neutron number. 相似文献
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Alber T Bächler J Bartke J Bialkowska H Bloomer MA Bock R Braithwaite WJ Brinkmann D Brockmann R Buncic P Chan P Cramer PB Cramer JG Derado I Eckardt V Eschke J Favuzzi C Ferenc D Fleischmann B Foka P Freund P Fuchs M Gazdzicki M Gladysz E Harris JW Hoffman M Jacobs P Kabana S Kadija K Kosiec J Kowalski M Kühmichel A Lahanas M Lee JY Ljubicic A Margetis S Mitchell JT Morse RJ Nappi E Odyniec G Paic G Panagiotou AD Petridis A Piper A Posa F Poskanzer AM Pühlhofer F Rauch W Renfordt R Retyk W 《Physical review letters》1995,74(8):1303-1306
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Nicole Lahanas Pavel Kucheryavy Roger A. Lalancette Jenny V. Lockard 《Acta Crystallographica. Section C, Structural Chemistry》2019,75(3):304-312
Studying the axial ligation behavior of metalloporphyrins with nitrogenous bases helps to better understand not only the biological function of heme‐based protein systems, but also the catalytic properties of porphyrin‐based reaction sites in other biomimetic synthetic support environments. Unlike iron porphyrin complexes, little is known about the axial ligation behavior of Mn porphyrins, particularly in the solid state with Mn in the +3 oxidation state. Here, we present the syntheses and crystal and molecular structures of three new high‐spin manganese(III) porphyrin complexes with the different amine‐based axial ligands imidazole (im), piperidine (pip), and 1,4‐diazabicyclo[2.2.2]octane (DABCO), namely bis(imidazole)(5,10,15,20‐tetraphenylporphyrinato)manganese(III) chloride chloroform disolvate, [Mn(C44H28N4)(C3H4N2)2]Cl·2CHCl3 or [Mn(TPP)(im)2]Cl·2CHCl3 (TPP = 5,10,15,20‐tetraphenylporphyrin), (I), bis(piperidine)(5,10,15,20‐tetraphenylporphyrinato)manganese(III) chloride, [Mn(C44H28N4)(C5H11N)2]Cl or [Mn(TPP)(pip)2]Cl, (II), and chlorido(1,4‐diazabicyclo[2.2.2]octane)(5,10,15,20‐tetraphenylporphyrin)manganese(III)–1,4‐diazabicyclo[2.2.2]octane–toluene–water (4/4/4/1), [Mn(C44H28N4)Cl(C6H12N2)]·C6H12N2·C7H8·0.25H2O or [Mn(TPP)Cl(DABCO)]·(DABCO)·(toluene)·0.25H2O, (IV). A fourth complex, chlorido(pyridine)(5,10,15,20‐tetraphenylporphryinato)manganese(III) pyridine disolvate, [Mn(C44H28N4)Cl(C5H5N)]·2C5H5N or [Mn(TPP)Cl(py)]·2(py), (III), acquired using different crystallization methods from published data, is also reported and compared to the previous structures. 相似文献
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