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941.
942.
The atomic structure and magnetic and electric properties of the Cr0.5TiSe2-Cr0.5TiTe2 system of intercalated phases were studied in detail by gradually replacing selenium by tellurium. It was revealed that this replacement changes the crystalline structure from monoclinic in the initial compounds to hexagonal in the compounds containing various types of chalcogen atoms; this is accompanied by disordering of chromium atoms in the van der Waals gaps. The electrical resistance and magnetic characteristics vary nonmonotonically on replacement of selenium by tellurium, which is associated with a change in the degree of atomic disordering during the transition from Cr0.5TiSe2 to Cr0.5TiTe2. 相似文献
943.
D. K. Kuznetsov I. S. Baturin V. Ya. Shur N. Menou C. Muller T. Schneller A. Sternberg 《Physics of the Solid State》2006,48(6):1174-1176
The effect of irradiation with electrons and neutrons and of exposure to synchrotron radiation on cyclic switching of polarization in thin films of lead zirconate titanate Pb(Zr,Ti)O3 (PZT) was studied. It is shown that variations in the shape of switching currents are due to the generation of a spatially nonuniform bound internal field with account for an increase in the rate of bulk screening caused by irradiation. A correlation between structural variations and the evolution of the switching current measured during and after irradiation is established. 相似文献
944.
V. P. Nekhoroshev Yu. P. Turov A. V. Nekhorosheva V. D. Ogorodnikov K. N. Gaevoi 《Russian Journal of Applied Chemistry》2006,79(5):833-840
The composition and structure of low-molecular-weight products of thermal oxidative degradation of atactic polypropylene were studied. 相似文献
945.
946.
V. A. Zayats A. N. Nikolaevskii T. A. Filippenko O. P. Kniga G. A. Tikhonova 《Russian Journal of Applied Chemistry》2006,79(10):1651-1654
Specific features of the initiated oxidation of polyethylene and its low-molecular-weight analogue tridecane, associated with the occurrence of the process in the short-chain mode, were studied. 相似文献
947.
V. P. Korolev 《Russian Journal of Applied Chemistry》2006,79(11):1779-1784
An equation for the standard enthalpy of solvation of a compound in a binary solvent is derived. The enthalpies of solvation in water-methanol mixtures are estimated for 1,3-propane-and 1,6-hexanediols, 1,2,4-butane-and 1,3,5-pentanetriols, 2-methoxy-and 2-propoxyethanols, and diethylene glycol. The enthalpy of solvation of 1,2-dimethoxyethane in the water-methanol mixed solvent is determined experimentally. 相似文献
948.
The not-sufficient-enough conductance of semioxidized protonated polyaniline (PANI) is usually attributed to the presence of ordered quasi-metallic domains surrounded by a poorly conducting amorphous phase. The paper presents experimental results testifying to the existence, in semioxidized PANI, of multilevel redox heterogeneity that crucially effects the conductance magnitude in view of specific topology at which higher-oxidized (conducting) domains are surrounded by less oxidized (poorly conducting) domains and because the PANI conduction is extremely sensitive to the oxidation degree. It is shown experimentally that the interphase doping with metals and degenerate semiconductors of a semioxidized salt of PANI and poly(2-acrylamide-2-methyl-1-propanesulfonic acid) (PAMPSA) with a 1: 2 ratio between PANI and PAMPSA raises the PANI-PAMPSA conductivity by 3–8 orders of magnitude due to the formation near the interface of thin layers whose conductance depends on the work function of the material in contact with PANI-PAMPSA and in extreme cases substantially exceeds the conductance of gold and copper at room temperature. 相似文献
949.
950.
We examine the optical near-field interaction between different types of scanning tips and single oriented fluorescent molecules.
We demonstrate the influence of a tip on the excitation intensity as well as on the integrated fluorescence signal, the excited
state lifetime, and the angular emission of single molecules. By using a standard model describing the radiation of an oscillating
dipole close to a nanosphere or a flat interface, we interpret our observations and describe some central criteria for obtaining
fluorescence enhancement or quenching.
PACS 33.80.-b; 07.79.Fc; 78.90.+t 相似文献