Interferometric determination of the s and d-wave scattering amplitudes in 87Rb

We demonstrate an interference method to determine the low-energy elastic scattering amplitudes of a quantum gas. We linearly accelerate two ultracold atomic clouds up to energies of 1.2 mK and observe the collision halo by direct imaging in free space. From the interference between s- and d- partial waves in the differential scattering pattern we extract the corresponding phase shifts. The method does not require knowledge of the atomic density. This allows us to infer accurate values for the s- and d-wave scattering amplitudes from the zero-energy limit up to the first Ramsauer minimum using only the van der Waals C6 coefficient as theoretical input. For the 87Rb triplet potential, the method reproduces the scattering length with an accuracy of 6%.     

Collective modes and the periodicity of quantum Hall stripes

We investigate the quantum Hall stripe phase at filling factor 9/2 at the microscopic level by probing the dispersion of its collective modes with the help of surface acoustic waves with wavelengths down to 60 nm. The dispersion is strongly anisotropic. It is highly dispersive and exhibits a roton minimum for wave vectors aligned along the easy transport direction. In the perpendicular direction, however, the dispersion is featureless, although not flat as predicted by theory. Oscillatory behavior in the absorption intensity of the collective mode with a wave vector perpendicular to the stripes is attributed to a commensurability effect. It allows us to extract the periodicity of the quantum Hall stripes.     

Self-organized growth of quantum dot-tunnel barrier systems

Surface selective epitaxial growth on patterned substrates is used to fabricate quantum dot-tunnel barrier systems, which can be used as single-electron transistor devices. In the centre of a pre-patterned constriction a self-assembled GaAs quantum dot embedded in barrier material is formed during the molecular beam epitaxial growth of an Al_0.33Ga_0.67As/GaAs heterostructure. The quantum dot is connected via self-aligned tunnelling barriers to source and drain electrodes. In-plane-gate electrodes are also realized within the epitaxial growth process. The paper describes the fabrication process of the device and the characterization of the direct grown quantum dot-tunnel barrier system using scanning-electron microscopy, atomic-force microscopy and transport spectroscopy.     

Single‐Crystal‐to‐Single‐Crystal Transition in an Enantiopure [7]Helquat Salt: The First Observation of a Reversible Phase Transition in a Helicene‐Like Compound

Here it is reported that crystals of an enantiopure [7]helquat salt undergo reversible thermal solid–solid phase transition at 404 K. Differential scanning calorimetry (DSC), capillary electrophoresis (CE), and X‐ray diffraction analysis were used to unravel the mechanistic details of this process. The single‐crystal‐to‐single‐crystal course enabled direct monitoring of the structural changes by in situ variable‐temperature X‐ray diffraction, thus providing the first direct evidence of a solid phase transition in a helicene‐like compound.     

Versatile phase transfer of gold nanoparticles from aqueous media to different organic media

A novel, simple, and very efficient method to prepare hydrophobically modified gold particles is presented. Gold nanoparticles of different sizes and polydispersities were prepared. The diameter of the gold particles ranges from 5 to 37 nm. All systems were prepared in aqueous solution stabilized by citrate and afterwards transferred into an organic phase by using amphiphilic alkylamine ligands with different alkyl chain lengths. The chain length was varied between 8 and 18 alkyl groups. Depending on the particle size and the alkylamine, different transfer efficiencies were obtained. In some cases, the phase transfer has a yield of about 100%. After drying, the particles can be redispersed in different organic solvents. Characterization of the particles before and after transfer was performed by using UV/Vis spectroscopy, transmission electron microscopy (TEM), and small-angle X-ray scattering (SAXS) techniques. The effect of organic solvents with various refractive indices on the plasmon band position was investigated.     

Effect of ionic strength and type of ions on the structure of water swollen polyelectrolyte multilayers

This study addresses the effect of ionic strength and type of ions on the structure and water content of polyelectrolyte multilayers. Polyelectrolyte multilayers of poly(sodium-4-styrene sulfonate) (PSS) and poly(diallyl dimethyl ammonium chloride) (PDADMAC) prepared at different NaF, NaCl and NaBr concentrations have been investigated by neutron reflectometry against vacuum, H(2)O and D(2)O. Both thickness and water content of the multilayers increase with increasing ionic strength and increasing ion size. Two types of water were identified, "void water" which fills the voids of the multilayers and does not contribute to swelling but to a change in scattering length density and "swelling water" which directly contributes to swelling of the multilayers. The amount of void water decreases with increasing salt concentration and anion radius while the amount of swelling water increases with salt concentration and anion radius. This is interpreted as a denser structure in the dry state and larger ability to swell in water (sponge) for multilayers prepared from high ionic strengths and/or salt solution of large anions. No exchange of hydration water or replacement of H by D was detected even after eight hours incubation time in water of opposing isotopic composition.     

Kinetics of indirect electron-hole recombination in a wide single quantum well in a strong electric field

The kinetics of the indirect recombination of electrons and holes in wide single quantum wells in a strong electric field has been analyzed. It has been shown that the recombination time increases exponentially up to 20 μs due to the spatial separation of oppositely charged particles. The results of a theoretical model predicting the behavior of the recombination time as a function of the applied field are in good agreement with experimental data.     

Spatial correlations of recombination radiation intensities of two-dimensional electrons under the conditions of the quantum Hall effect

Correlations have been studied between the recombination radiation intensities of a two-dimensional electron gas measured at different points of the sample with giant luminescence fluctuations in the quantum Hall effect regime. It has been found that the correlation of the radiation intensities measured under these conditions at different points of the sample separated by a distance of 1–3 mm is close to unity and disappeared in a threshold way with increasing temperature. It is shown that macroscopic spatial correlations also disappear if the electron system is artificially divided into two subsystems not connected with each other.