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Karl Strambach C. G. Bartolone 《Abhandlungen aus dem Mathematischen Seminar der Universit?t Hamburg》1989,59(1):93-99
This research was supported by M.P.I. (R.S. 40%). 相似文献
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Marko D. Mihovilovic Bernhard Müller Markus Spina Arjumand I. Durrani Peter Stanetty Georg Dazinger Karl Kirchner 《Monatshefte für Chemie / Chemical Monthly》2006,137(6):785-794
Summary. Recombinant Escherichia coli overexpressing Pseudomonas sp. NCIMB 9872 cyclopentanone monooxygenase (CPMO, EC 1.14.13.16) and Acinetobacter sp. NCIMB 9871 cyclohexanone monooxygenase (CHMO, EC 1.14.13.22) have been utilized in whole-cell Baeyer-Villiger biotransformations of prochiral bicycloketones. A significant difference in substrate acceptance and stereoselectivity was
observed for bicyclo[3.3.0] and bicyclo[4.3.0] substrates. A plausible mechanism of these transformations was established
by means of high level DFT/B3LYP calculations suggesting an essential difference in electronic requirements for a successful
enzymatic conversion, which was similarly encountered in recombinant whole-cell mediated biooxidations. Some of the lactones
produced in the biocatalytic Baeyer-Villiger oxidation represent key intermediates for the synthesis of indole alkaloids. 相似文献
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Karl F. Canter 《Hyperfine Interactions》1992,73(1-2):159-171
The present status of low energy positron diffraction (LEPD) and positron reemission microscopy (PRM) is reviewed in the context
of unanswered questions regarding the elastic scattering of positrons in the 1–300 eV energy range from atoms in solids and
at solid surfaces. Recent LEPD studies yield an agreement between theoretical and experimental diffraction intensities for
semiconductors that has never been equalled in electron diffraction studies. This situation is discussed in terms of the repulsive
interaction between the positron and the embedded atomic potential and the lack of exchange with the nonspherically distributed
valence electrons. The scattering of re-emitted positrons in PRM from atoms chemisorbed or physisorbed on the re-emitting
surface has not yet received the same theoretical attention as scattering from embedded atoms in LEPD. Possible ways in which
positron scattering from overlying atomic structures manifests itself in PRM as well as positron re-emission holography are
discussed, both from the practical viewpoint of observing these structures and in the context of fundamental questions regarding
the positron re-emission process itself. 相似文献
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Multistage stochastic programs with continuous underlying distributions involve the obstacle of high-dimensional integrals where the integrands' values again are given by solutions of stochastic programs. A common solution technique consists of discretizing the support of the original distributions leading to scenario trees and corresponding LPs which are – up to a certain size – easy to solve. In order to improve the accuracy of approximation, successive refinements of the support result in rapidly expanding scenario trees and associated LPs. Hence, the solvability of the multistage stochastic program is limited by the numerical solvability of sequences of such expanding LPs. This work describes an algorithmic technique for solving the large-scale LP of refinement ν based on the solutions at the previous ν?1 refinements. Numerical results are presented for practical problem statements within financial applications demonstrating significant speedup (depending on the size of the LP instances). 相似文献
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