排序方式: 共有78条查询结果,搜索用时 46 毫秒
71.
Mari Granström Jari Kavakka Alistair King Johanna Majoinen Valtteri Mäkelä Juho Helaja Sami Hietala Tommi Virtanen Sirkka-Liisa Maunu Dimitris S. Argyropoulos Ilkka Kilpeläinen 《Cellulose (London, England)》2008,15(3):481-488
Tosylation and acylation of cellulose were performed under mild reaction conditions using imidazolium based ionic liquids
(ILs) as solvents. The non-degradative nature, lower viscosity, as well as higher solubility of cellulose in [amim]Cl encouraged
us to carry out the reactions in this media. The reactions described here were optimised for this particular solvent in order
to obtain different cellulose derivatives with high yields, homogeneity and degree of substitution (DS). Two reagents employed
for the in situ activation of carboxylic acids were N,N′-carbonyldiimidazole (CDI) and 1-ethyl-3-(3′-dimethylaminopropyl)carbodiimide hydrochloride (EDCI). Final products were characterised
by solution and solid-state NMR techniques.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
72.
Athar SB Patel R Yelton J Rubin P Eisenstein BI Karliner I Mehrabyan S Lowrey N Selen M White EJ Wiss J Mitchell RE Shepherd MR Besson D Pedlar TK Cronin-Hennessy D Gao KY Hietala J Kubota Y Klein T Lang BW Poling R Scott AW Zweber P Dobbs S Metreveli Z Seth KK Tomaradze A Libby J Powell A Wilkinson G Ecklund KM Love W Savinov V Lopez A Mendez H Ramirez J Ge JY Miller DH Shipsey IP Xin B Adams GS Anderson M Cummings JP Danko I Hu D Moziak B Napolitano J He Q Insler J Muramatsu H Park CS 《Physical review letters》2008,100(18):181802
Using e+e--->Ds*-Ds+ data collected near the peak Ds production energy, Ecm=4170 MeV, with the CLEO-c detector, we present the first observation of the decay Ds+-->pn. We measure a branching fraction B(Ds+-->pn)=(1.30+/-0.36(-0.16)+0.12)x10(-3). This is the first observation of a charmed meson decaying into a baryon-antibaryon final state. 相似文献
73.
Alexander JP Berkelman K Cassel DG Duboscq JE Ehrlich R Fields L Gibbons L Gray R Gray SW Hartill DL Heltsley BK Hertz D Jones CD Kandaswamy J Kreinick DL Kuznetsov VE Mahlke-Krüger H Mohapatra D Onyisi PU Patterson JR Peterson D Riley D Ryd A Sadoff AJ Shi X Stroiney S Sun WM Wilksen T Athar SB Patel R Yelton J Rubin P Eisenstein BI Karliner I Mehrabyan S Lowrey N Selen M White EJ Wiss J Mitchell RE Shepherd MR Besson D Pedlar TK Cronin-Hennessy D Gao KY Hietala J Kubota Y Klein T Lang BW 《Physical review letters》2008,100(16):161804
The branching fractions of D(s)(+/-) meson decays serve to normalize many measurements of processes involving charm quarks. Using 298 pb(-1) of e(+)e(-) collisions recorded at a center of mass energy of 4.17 GeV, we determine absolute branching fractions for eight D(s)(+/-) decays with a double tag technique. In particular we determine the branching fraction B(D(s)(+)-->K(-)K(+}pi(+))=(5.50+/-0.23+/-0.16)%, where the uncertainties are statistical and systematic, respectively. We also provide partial branching fractions for kinematic subsets of the K(-)K(+)pi(+) decay mode. 相似文献
74.
Cronin-Hennessy D Gao KY Gong DT Hietala J Kubota Y Klein T Lang BW Poling R Scott AW Smith A Zweber P Dobbs S Metreveli Z Seth KK Tomaradze A Ernst J Severini H Dytman SA Love W Savinov V Aquines O Li Z Lopez A Mehrabyan S Mendez H Ramirez J Huang GS Miller DH Pavlunin V Sanghi B Shipsey IP Xin B Adams GS Anderson M Cummings JP Danko I Napolitano J He Q Insler J Muramatsu H Park CS Thorndike EH Yang F Coan TE Gao YS Liu F Artuso M Blusk S Butt J Li J Menaa N Mountain R Nisar S 《Physical review letters》2008,100(25):251802
By using 1.8x10{6} DDpairs, we have measured B(D{0}-->pi{-}e{+}nu{e})=0.299(11)(9)%, B(D{+}-->pi{0}e{+}nu{e})=0.373(22)(13)%, B(D{0}-->K{-}e{+}nu{e})=3.56(3)(9)%, and B(D{+}-->K{0}e{+}nu{e})=8.53(13)(23)% and have studied the q;{2} dependence of the form factors. By combining our results with recent lattice calculations, we obtain |V{cd}|=0.217(9)(4)(23) and |V{cs}|=1.015(10)(11)(106). 相似文献
75.
Bisfunctionalized Janus molecules 总被引:1,自引:0,他引:1
[reaction: see text] Bisfunctionalized dendritic multiester molecules were synthesized by combined protection-deprotection and divergent-convergent-divergent sequences in high yields leading to dendritic molecules that combine two functionally different surfaces, polar aliphatic arborol and nonpolar gallate ether moieties, resulting in a two-faced Janus molecule. 相似文献
76.
It is shown that the traveling salesman problem, where cities are bit strings with Hamming distances, is NP-complete. 相似文献
77.
Jarmo Hietarinta Da-jun Zhang 《Journal of Difference Equations and Applications》2013,19(8):1292-1316
Hirota's bilinear method (‘direct method’) has been very effective for constructing soliton solutions to many integrable equations. The construction of one-soliton solution (1SS) and two-soliton solution (2SS) is possible even for non-integrable bilinear equations, but the existence of a generic three-soliton solution (3SS) imposes severe constraints and is in fact equivalent to integrability. This property has been used before in searching for integrable partial differential equations, and in this paper we apply it to two-dimensional (2D) partial difference equations defined on a 3 × 3 stencil. We also discuss how the obtained equations are related to projections and limits of the 3D master equations of Hirota and Miwa, and find that sometimes a singular limit is needed. 相似文献
78.
Tailoring steps in aromatic polyketide antibiotic biosynthesis are an important source of structural diversity and, consequently, an intriguing focal point for enzymological studies. PgaE and PgaM from Streptomyces sp. PGA64 are representatives of flavoenzymes catalyzing early post-PKS reactions in angucycline biosynthesis. This in vitro study illustrates that the chemoenzymatic conversion of UWM6 into the metabolite, gaudimycin C, requires multiple closely coupled reactions to prevent intermediate degradation. The NMR structure of gaudimycin C confirms that the reaction cascade involves C12- and C12b-hydroxylation, C2,3-dehydration, and stereospecific ketoreduction at C6. Enzymatic 18O incorporation studies verify that the oxygens at C12 and C12b derive from O2 and H2O, respectively. The results indicate that PgaM deviates mechanistically from flavoprotein monooxygenases, and suggest an alternative catalytic mechanism involving a quinone methide intermediate. 相似文献