The influence of exciton motion on spin-resonance absorption

We use a stochastic model for the exciton motion which comprises both the coherent and the incoherent motion. The incoherent part is taken care of by a stochastic process which allows the local excitation energy and the transition matrix element to fluctuate by means of a Markovian process. The interaction between the spins and their surroundings is described by the usual spin-Hamiltonian which is, however, simplified to a spin 1/2 particle (instead of the triplet state). In the present paper we solve exactly the two limiting cases of completely coherent and incoherent motion (for two molecules). In the incoherent case the influence of the exchange interaction integral is taken into account by perturbation theory. We find expressions which are immediately comparable with ESR-experimental data. This comparison and additional information derived from optical absorption measurements allow us to determine all free parameters of our model uniquely. In particular, the fluctuations of the exchange interaction integral (with strength γ₁) play an important role. From these parameters we may furthermore calculate the correlation time of the proton spin resonance in agreement with experimental data. The results show clearly that at room temperature in anthracene crystals the exciton undergoes a hopping process.     

Quantummechanical solutions of the laser masterequation. II

A Fokker-Planck equation for a distribution function over the macroscopic observables of the laser essentially equivalent to that recently obtained byRisken,Schmid andWeidlich is derived from the fundamental quantummechanical laser masterequation. The general method used is the expansion of the statistical operator in a complete set of projection operators of the atoms and the lightfield. The assumptions leading from the microscopic equation of motion to the macroscopic semiclassical Fokker-Planck equation are explicitly introduced and discussed.     

Nonlinear interaction of laser modes

The interaction of N atoms each with 3 levels at random lattice sites with a set of cavity modes is considered. The optical transition between the lowest two atomic levels is taken into account explicitely assuming a Lorentzian line shape, whereas the third level just serves for the pumping process. If homogeneous inversion of the atoms is assumed, only one coherent mode oscillates in the steady state. It is the one being closest to the atomic resonance and having highestQ. If, however, in the next approximation a mode-dependent depletion of the excited atomic states is taken into account, with increasing pumping rate several modes may oscillate simultaneously. The behaviour of two such modes is treated in detail and it is shown, that one obtains a stable configuration. Using a higher approximation the nonlinear interaction between these two modes brought about by the amplifying material is studied in detail. As a special result one obtains a repulsion of the frequencies of the modes as a function of pumping power in accordance with gaslaser experiments. Quantum noise effects are neglected throughout the present paper.     

A theoretical derivation of cellular structures of flames

Using an equation for the formation of flame fronts derived by Sivashinsky and augmented by an additional term describing buoyancy effects we present an analytical treatment of the formation of cellular structures of flames formed by plane burners. In particular we find rectangular and square patterns. We first study the stability of the plane flame front by linear stability analysis and then transform the basic equation into a set of equations for the amplitudes of the stable and unstable modes. The amplitudes of the stable modes can be eliminated by the slaving principle so that generalized Ginzburg-Landau equations result which in a general frame were previously derived by one of us (H.H.). These equations are then solved explicitly and the stability of the resulting pattern is proven.     

Effect of delay on phase locking in a pulse coupled neural network

Using a slightly simplified version of the integrate and fire model of a neural network with delay, I study the stability of the phase-locked state dependent on the coupling between the neurons and especially on a delay time. The coupling between neurons may be arbitrary. It is shown that the phase-locked state becomes less stable with increasing delay and that relaxation oscillations occur. Received 28 December 1999 and Received in final form 13 June 2000     

Self-pulsing instabilities in the generation of higher harmonics

We consider nonlinear optical processes in a cavity. The processes are driven by an external coherent pump. We predict self-pulsing instabilities in the generation of higher harmonics. We also derive formulas for the threshold pump strength and critical selfpulsing frequency.     

Numerical calculation of current density distributions in high temperature superconducting tapes with finite thickness in self field and external field

The current density distribution of high temperature superconducting (HTS) tapes is modeled for the combined case of an alternating self and applied magnetic field. This numerical analysis is based on the two-dimensional Poisson equation for the vector potential. A one-dimensional current (z-direction) and a one-dimensional applied field (y-direction) are assumed. The vector potential is rewritten into an equation of motion for the current density J(x,y,t). The model covers the finite thickness of the conductor and an n-power E–J relation. The magnetic field dependence of J_c is also included in this E–J relation. A time-dependent two-dimensional current distribution that is influenced by the aspect ratio of the conductor and the material properties in E=f(J,B) is calculated numerically. The numerical results are compared with the experimental results for the AC loss of a tape driven by a transport current. Finally, a total AC loss factor is given for two cases in magnetic field direction, perpendicular and parallel to the conductor broad side.     

Theory of two-photon lasers III

We treat the semiclassical equations and the Fokker-Planck equation of a two-photon laser with one or two injected signals and treat both the degenerate and nondegenerate case. The resulting behaviour in the two-photon laser is discussed by means of potential functions which allows one to determine the stable, unstable, and metastable states.     

Learning in synergetic systems for pattern recognition and associative action

Synergetic systems are in particular physical systems which can produce spatial or temporal patterns by means of the interaction of their individual parts. We show how such a system can be devised or even learn by itself to reproduce given patterns described by their probability distribution function. If an initial state close to one of the learned patterns is presented to such a system, it will pull the initial state into an attractor belonging to the learned state (pattern recognition via associative memory). Furthermore we show how such a system can be devised or can learn to perform any prescribed stationary continous Markov process. If a set of incomplete or partly incorrect initial data is offered to such a system, it may correct it and perform associative action.     

Elimination of variables in simple laser equations

The usual way of obtaining rate equations (RE) and a single equation for the field amplitude (EFA) from the semiclassical laser equations (Lorenz-Haken model) is reexamined by undertaking a systematic elimination procedure developed in synergetics. The RE and EFA are justified in the case 1 (, ) and case 2 (, ), respectively. We show that, because the eliminated variable happens to contain a considerable contribution from an unstable mode, the usual elimination technique in the case 3 (, ) leads to an inconsistency. As important by-products we obtain the RE and EFA for arbitrary cavity relaxation constant (). Some remarks are given on the direct elimination technique in the non-diagonal representation in the study of instabilities.