Nucleon transfer reactions to rotational states induced by206, 208Pb projectiles

In a systematic study of nucleon transfer reactions accompanied by Coulomb excitation we have bombarded¹⁵²Sm,¹⁶⁰Gd and²³²Th with^{206, 208}pb beams at incident energies close to the Coulomb barrier. Particle-gamma coincidence techniques were used to identify excited states of reaction products populated through inelastic scattering and in nucleon transfer reactions. One-neutron stripping and pick-up reactions on¹⁵²Sm were observed leading to known states of the rotation alignedi _13/2-bands in¹⁵³Sm and¹⁵¹Sm. In the¹⁶⁰Gd+^{206, 208}Pb systems no significant population of low lying states of product nuclei was found in the nucleon-transfer channels. Large cross sections were observed for one- and two-neutron pick-up from²³²Th at an incident energy of 6.4 MeV/u. Around the grazing angle they are of the same order of magnitude as the cross section measured for inelastic scattering. The results are analyzed in the framework of semiclassical models.     

Combinatorial Chemistry for Ligand Development in Catalysis: Synthesis and Catalysis Screening of Peptidosulfonamide Tweezers on the Solid Phase

On the basis of a pyrrolidine tweezer 1, a library of peptidosulfonamide tweezers (15a-e, 16a-e) was synthesized on the solid phase. This library was screened in a simultaneous substrate screening procedure for the ability to enantioselectively catalyze the Ti(O-i-Pr)(4)-mediated addition of diethylzinc to aldehydes. One of the best solid-phase tweezer catalyst (i.e., 16d, giving an ee of 32% in solid-phase catalysis) was resynthesized in solution (compounds 20 and 21). The now homogeneous solution-phase catalysis showed even better enantioselectivity (i.e., up to 66%).     

Selection of cold transfer and enhanced neutron-pair transfer in the 206 Pb + 118 Sn reaction

The neutron transfer in a very heavy asymmetric nuclear system, in ²⁰⁶Pb + ¹¹⁸Sn has been measured using particle- coincidence techniques with position-sensitive detectors, 5 EUROBALL-Cluster detectors (EB) and the Heidelberg-Darmstadt NaI-CRYSTAL BALL (CB). The fragments are identified via the known -decays of the lowest excited states using the high resolution of EB. Using the unique feature of the set-up with the CB, transfer to well-defined final channels with known quantum numbers is selected using the high-efficiency multiplicity filter of the CB with no second -ray, i.e. without feeding. The enhancement in the two-neutron transfer is deduced, for population of the low-lying super-fluid 2 ⁺ states in ¹²⁰Sn and ¹¹⁶Sn, while the 2n-transition remains in the ground state for the recoiling ^20XPb-nuclei. Large enhancements up to EF are observed. This is the first observation of neutron pair-transfer enhancement for a heavy nuclear binary system with superfluid properties with experimentally separated levels.Received: 6 November 2002, Revised: 25 March 2003, Published online: 23 March 2004PACS: 24.10.Eq Coupled-channel and distorted-wave models - 25.70.Hi Transfer reactions     

Experimental details of the Stopped Beam RISING campaign

The RISING (Rare ISotope INvestigations at GSI) project constitutes a major pan-european initiative to study nuclear structure in exotic nuclei. A brief outline of the technical details specific to studies of isomeric decays following relativistic projectile fragmentation reactions is presented.     

Measurement ofg-factors in160Yb by aγ-γ coincidence technique

Aγ-γ coincidence technique has been developed forg-factor measurements of short-lived nuclear states. The method involvesγ-detection in 4π geometry as well as transient magnetic fields and the recoil-distance technique. A first experiment was performed for the isotope¹⁶⁰Yb produced in the reaction⁶⁴Ni(¹⁰⁰Mo, 4n) at 430 MeV beam energy. The valueg=? 0.23(31) of the 14⁺ yrast state, which is compatible with zero, establishes thevi _13/2 quasiparticle structure to be responsible for the first backbend. A meang-factor for low spin states around the 4⁺ state,g=+0.48(26) was also derived as well as lifetimes for yrast states up toI ^π=8⁺.     

Gamma-ray spectroscopy with relativistic exotic heavy-ions

Feasibility of gamma-ray spectroscopy at relativistic energies with exotic heavy-ions and new generation of germanium detectors (segmented Clover) is discussed. An experiment with such detector array and radioactive is discussed.     

Triaxiality andγ-softness in196Pt

The nuclear level structure and electromagnetic properties of¹⁹⁶Pt were investigated withγ-spectroscopic techniques using multiple Coulomb excitation by²⁰⁸Pb projectiles. Particle-γ, and particle-γ-γ coincidences were measured over a wide range of scattering angles.E2-transition moments and static quadrupole moments have been determined by a comparison of experimental scattering-angle dependentγ yields with calculated yields in a largely model-independent procedure. The results are compared with different theoretical models: the Asymmetric-Rotor Model, the Generalized Collective Model, and the Interacting Boson Model. The best agreement is obtained with the Generalized Collective Model representing a triaxial nucleus which is soft in theγ degree of freedom.     

In-beam spectroscopy of 253, 254No

In-beam conversion electron spectroscopy experiments have been performed on the transfermium nuclei ^{253, 254}No using the conversion electron spectrometer SACRED in nearly collinear geometry in conjunction with the gas-filled separator RITU at the University of Jyv?skyl?. The experimental setup is discussed and the spectra are compared to Monte Carlo simulations. The implications for the ground-state configuration of ²⁵³No are discussed. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: rdh@ns.ph.liv.ac.uk RID="b" ID="b"Present address: GANIL, F-14021 Caen, France. RID="c" ID="c"Permanent address: IReS Strasbourg, IN2P3-CNRS, F-67037-Strasbourg, France. RID="d" ID="d"Present address: CEA/DIF DCRE/SDE/LDN F-91680 Bruyeres-le-Chatel. RID="e" ID="e"Present address: Daresbury Laboratory, Daresbury WA4 4AD, UK. RID="f" ID="f"Permanent address: IPN Lyon, IN2P3-CNRS, F-69037 Lyon, France.