Identification of a new isotope,168Dy

A previously unreported nuclide,¹⁶⁸Dy, has been identified and found to have a half-life of 8.5+-0.5 min. The activity was produced in the spontaneous fission of²⁵²Cf and transported via a He jet system to a rapid radiochemical separative facility where the Dy fraction was removed from the mixed fission products. The assignment of this activity to¹⁶⁸Dy decay was based on the presence of five γ rays in the chemically separated Dy fraction which were associated with the decay of an 8.5-min activity and on the observation of the grow-in and subsequent decay of the daughter, 2.98-min¹⁶⁸Ho, with approximately an 8-min half-life. The γ-ray emission probabilities have been determined.     

Sparse Partially Linear Additive Models

The generalized partially linear additive model (GPLAM) is a flexible and interpretable approach to building predictive models. It combines features in an additive manner, allowing each to have either a linear or nonlinear effect on the response. However, the choice of which features to treat as linear or nonlinear is typically assumed known. Thus, to make a GPLAM a viable approach in situations in which little is known a priori about the features, one must overcome two primary model selection challenges: deciding which features to include in the model and determining which of these features to treat nonlinearly. We introduce the sparse partially linear additive model (SPLAM), which combines model fitting and both of these model selection challenges into a single convex optimization problem. SPLAM provides a bridge between the lasso and sparse additive models. Through a statistical oracle inequality and thorough simulation, we demonstrate that SPLAM can outperform other methods across a broad spectrum of statistical regimes, including the high-dimensional (p ? N) setting. We develop efficient algorithms that are applied to real datasets with half a million samples and over 45,000 features with excellent predictive performance. Supplementary materials for this article are available online.     

Controllable coupling of superconducting flux qubits

We have realized controllable coupling between two three-junction flux qubits by inserting an additional coupler loop between them, containing three Josephson junctions. Two of these are shared with the qubit loops, providing strong qubit-coupler interaction. The third junction gives the coupler a nontrivial current-flux relation; its derivative (i.e., the susceptibility) determines the coupling strength J, which thus is tunable in situ via the coupler's flux bias. In the qubit regime, J was varied from approximately 45 (antiferromagnetic) to approximately -55 mK (ferromagnetic); in particular, J vanishes for an intermediate coupler bias. Measurements on a second sample illuminate the relation between two-qubit tunable coupling and three-qubit behavior.     

Spatially resolved surface-charge measurement in a planar dielectric-barrier discharge system

We investigate a laterally extended dielectric helium discharge system with plane electrodes. The system is operated in the glow mode and is known to exhibit a rich variety of self-organized lateral patterns in the current distribution, most of them being filamentary. It is known from theory that surface charges on the dielectrics play a major role for the emerging patterns. In this work we present a method to measure the spatial charge distribution on the dielectrics via the Pockels effect of a bismuth-silicon-oxide crystal. The experimental results of the surface-charge distribution measurements are in good agreement with previous numerical solutions of the corresponding transport equations.     

Morphological Changes of Linear,Branched Polyethylenes and their Blends during Crystallization and Subsequent Melting by Synchrotron SAXS and DSC

Summary: The crystalline structure and phase morphology of linear, branched polyethylenes and their blends during crystallization and subsequent melting were investigated, using a combination of differential scanning calorimetry (DSC), and synchrotron small angle X-ray scattering (SAXS). A linear polyethylene (PE1) with weight-average molecular weight (M_w) of 114 000 g/mol, and two branched polyethylene copolymers, containing 4.8 mol% (PE4) and 15.3 mol% (PE10) hexane, with molecular weights of 93 000 g/mol and 46 000 g/mol were used as pure samples. Two blends, PE1-4 and PE1-10, each with a weight ratio of 50/50, were prepared by solution blending. Our results indicate that in PE4 a phase separation within the branched component itself occurred, forming a broad distribution of lamellar thicknesses during the crystallization process. PE10 on the other hand did hardly crystallize because of the high degree of branching. Co-crystallization of both components took place in blend PE1-4 and liquid-liquid phase separation occurred in the melt of PE1-10. Morphological parameters were determined by using Bragg's law and the correlation function, respectively. The detected semicrystalline morphology can be well described by the lamellar insertion mode where thin lamellae develop between thicker primary lamellae. During subsequent heating, lamellae melted in the reversed sequence of their formation. The evolution of the structural parameters as a function of temperature revealed that surface melting began at first, and then the complete melting of stacks occurred until the final melting temperature was reached.     

Colloidal Flower‐Shaped Iron Oxide Nanoparticles: Synthesis Strategies and Coatings

The assembly of magnetic cores into regular structures may notably influence the properties displayed by a magnetic colloid. Here, key synthesis parameters driving the self‐assembly process capable of organizing colloidal magnetic cores into highly regular and reproducible multi‐core nanoparticles are determined. In addition, a self‐consistent picture that explains the collective magnetic properties exhibited by these complex assemblies is achieved through structural, colloidal, and magnetic means. For this purpose, different strategies to obtain flower‐shaped iron oxide assemblies in the size range 25–100 nm are examined. The routes are based on the partial oxidation of Fe(OH)₂, polyol‐mediated synthesis or the reduction of iron acetylacetonate. The nanoparticles are functionalized either with dextran, citric acid, or alternatively embedded in polystyrene and their long‐term stability is assessed. The core size is measured, calculated, and modeled using both structural and magnetic means, while the Debye model and multi‐core extended model are used to study interparticle interactions. This is the first step toward standardized protocols of synthesis and characterization of flower‐shaped nanoparticles.     

The High Data Rate Processing and Analysis Initiative of the Helmholtz Association in Germany

The Helmholtz Association is the largest scientific organization in Germany. It operates all major German research infrastructures involved in research with photons, neutrons, and ions. These are DESY in Hamburg; the Karlsruhe Institute of Technology (KIT); the Research Centre Jülich (FZJ); the Helmholtz Centres in Geesthacht (HZG), Berlin (HZB), and Dresden-Rossendorf (HZDR); and the GSI Centre for research with heavy ions in Darmstadt. In common, all these centers are facing similar challenges related to dramatically increasing data rates and volumes generated with more and more powerful radiation sources together with larger and faster detectors. On the other hand, each center has its own specific portfolio of long-lasting technical expertise in areas like data analysis, information technology, or hardware development. Therefore, it was obvious to address the challenges by acting in concert. This was the main motivation in 2010 for the launch of a joint project among the partners called the “High Data Rate Processing and Analysis Initiative (HDRI).” The initiative is organized into three basic work packages: “Data Management,” “Real-time Data Processing,” and “Data Analysis, Modelling, and Simulation.” The aim is to carry out the development of methods, hardware components, and software for data acquisition, real-time and offline analysis, documentation and archiving, and for remote access to data. The solutions are finally meant to be integrated at the various experimental stations and thus have to be versatile and flexible to cope with the heterogeneous requirements of the different experiments. The claim to create standard solutions makes it mandatory to closely collaborate with large international activities in the field of data handling, like the European PaNdata project (see article in this issue), but also with vendors of detectors, data evaluation software, etc., as well as with corresponding standardization bodies.     

Artifact (α, x) Reaction Gamma-Ray Peaks Reported as 241Am Decay Gamma-Rays; Comments to the Paper by Abdulrahman Abdul-Hadi, J. Radioanal. Nucl. Chem., 231 (1998) 147

Review of a recent paper reporting the -ray energies and intensities associated with the decay of ²⁴¹Am has resulted in the conclusion that some of the rays were misidentified. The misidentified -rays are not associated with the decay of ²⁴¹Am, but rather are prompt -rays from alpha-induced reactions.