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排序方式: 共有148条查询结果,搜索用时 15 毫秒
101.
102.
Grajcar M Izmalkov A van der Ploeg SH Linzen S Plecenik T Wagner T Hübner U Il'ichev E Meyer HG Smirnov AY Love PJ Maassen van den Brink A Amin MH Uchaikin S Zagoskin AM 《Physical review letters》2006,96(4):047006
We present the first experimental results on a device with more than two superconducting qubits. The circuit consists of four three-junction flux qubits, with simultaneous ferro- and antiferromagnetic coupling implemented using shared Josephson junctions. Its response, which is dominated by the ground state, is characterized using low-frequency impedance measurement with a superconducting tank circuit coupled to the qubits. The results are found to be in excellent agreement with the quantum-mechanical predictions. 相似文献
103.
Boyen HG Ethirajan A Kästle G Weigl F Ziemann P Schmid G Garnier MG Büttner M Oelhafen P 《Physical review letters》2005,94(1):016804
Gold nanoclusters of a size approaching the molecular limit (<3 nm) were prepared on Si substrates in order to study alloy formation on the nanometer scale. For this purpose, indium atoms are deposited on top of the gold particles at room temperature and the formation of AuIn(2) is studied by x-ray photoelectron spectroscopy in situ. It is observed that the alloy formation takes place independent of whether the particles electronically are in an insulating molecular or in a metallic state. Most important, however, closed packed full-shell clusters containing 55 Au atoms are found to exhibit an outstanding stability against alloying despite a large negative heat of formation of the bulk Au-In system. Thus, Au(55) clusters may play a significant role in the design of nanoscaled devices where chemical inertness is of crucial importance. 相似文献
104.
105.
We report on the first experimental observation of a concentric-ring pattern in a short planar dielectric barrier gas-discharge system and study its spatiotemporal behavior. While increasing the gas pressure the destabilization of the rings into a filamentary structure is observed. The charge carriers deposited on the dielectric electrodes determine the spatiotemporal behavior of the pattern. 相似文献
106.
Pranzas PK Knöchel A Kneifel K Kamusewitz H Weigel T Gehrke R Funari SS Willumeit R 《Analytical and bioanalytical chemistry》2003,376(5):602-607
Polymeric membranes are used in industrial and analytical separation techniques. In this study small-angle X-ray scattering (SAXS) with synchrotron radiation has been applied for in-situ characterisation during formation of polymeric membranes. The spinning of a polyetherimide (PEI) hollow fibre membrane was chosen for investigation of dynamic aggregation processes during membrane formation, because it allows the measurement of the dynamic equilibrium at different distances from the spinning nozzle. With this system it is possible to resolve structural changes in the nm-size range which occur during membrane formation on the time-scale of milliseconds. Integral structural parameters, like radius of gyration and pair-distance distribution, were determined. Depending on the chosen spinning parameters, e.g. the flow ratio between polymer solution and coagulant water, significant changes in the scattering curves have been observed. The data are correlated with the distance from the spinning nozzle in order to get information about the kinetics of membrane formation which has fundamental influence on structure and properties of the membrane. 相似文献
107.
Hermsdorf N Stamm M Förster S Cunis S Funari SS Gehrke R Müller-Buschbaum P 《Langmuir : the ACS journal of surfaces and colloids》2005,21(25):11987-11993
Self-supported particle-track-etched polycarbonate membranes with nearly perfect cylindrical pores are used for the preparation of similarly perfect cylindrical polypyrrole nanowires and nanotubes. A complete investigation of the structural properties that result at different stages of the preparation route of polypyrrole nanowires and nanotubes is based on a combination of real and reciprocal space techniques. Nanoporous membranes with nominal pore size ranging from 5 to 150 nm and pore density up to 10(9) pores/cm(2) made from 21-microm-thick polycarbonate films are used. Polypyrrole nanotubes or nanowires are synthesized inside the pores. A real-space picture of the nanomaterial results from scanning force microscopy (SFM) on ultrathin sections made in two directions to obtain structures in the sample surface as well as perpendicular to the surface. From a model-based fit to the small-angle and ultra-small-angle X-ray scattering (SAXS/USAXS) data, the geometric pore structure is obtained and compared to values determined with scanning electron microscopy (SEM). Nanopores, nanowires, and nanotubes are described by uniform solid cylinders or hollow tubes, which are oriented highly parallel to each other and exhibit a small size distribution. Below a critical pore diameter, solid nanowires are produced whereas above this limit hollow nanotubes result. 相似文献
108.
C W Gehrke T P Waalkes E Borek W F Swartz T F Cole K C Kuo M Abeloff D S Ettinger N Rosenshein R C Young 《Journal of chromatography. A》1979,162(4):507-528
A precise and accurate gas-liquid chromatographic (GLC) method has been developed for the quantitative analysis of the neutral sugars L-fucose (6-deoxygalactose), mannose, galactose, and glucose in ethanol precipitates of human serum proteins. The chromatographic conditions and sample preparation resulted in short analysis time (20 min per run) and made routine analyses practicable (twelve samples per day). The alditol acetate derivatization yielded single derivatives for each sugar. Complete separation was achieved on a 2.0 m X 2 mm I.D. column with 2.0% Silar-7CP on Chromosorb W AW 80--100 mesh. The results of hydrolysis showed that the release of fucose and galactose preceded the release of mannose. Hydrolysis with AG 50 W-X8 (H+) ion-exchange resin in 0.5 N HCl at 100 degrees for 7 h optimized glycosidic bond cleavage with only minimal destruction of fucose, mannose and galactose. A combination of strong cation- and anion-exchange resin columns was used to remove chromatographic background of peptides, amino acids, amino sugars, and inorganic ions. An average R.S.D. of less than 4% with recovery of greater than 86% for the three sugars was achieved. The homogeneity of the chromatographic peaks for the neutral sugars of normal human serum glycoproteins was confirmed by GLC--mass spectrometry. Significantly elevated ratios of fucose, galactose, and mannose to serum protein were observed for patients with small cell lung and ovarian carcinomas. 相似文献
109.
R. G. Helmer R. J. Gehrke J. R. Davidson J. W. Mandler 《Journal of Radioanalytical and Nuclear Chemistry》2000,243(1):109-117
The original Gamma-ray Spectrum Catalogue, Ge(Li) and Si(Li) Spectrometry published in 1974 by R. L. Heath has been recreated and enhanced as an electronic file and is available on CD-ROM or over the Internet. This electronic version includes 1998 -ray data from the Evaluated Nuclear Structure Data File database as downloaded in 1998 as well as decay scheme drawings. Future developments of similar catalogues will include -ray spectra from radioactive decay with newer detectors and spectra from neutron interactions with elemental samples and separated isotopes. The electronic form of these catalogues will allow the creation of tutorials on -ray spectrometry and on the data included. 相似文献
110.