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排序方式: 共有71条查询结果,搜索用时 20 毫秒
61.
62.
An analysis of the effect that chemical and hydrostatic pressures have on the thermodynamic properties of perovskite-like
fluorine-oxygen compounds A
2
A′MeO
x
F6 − x
has revealed that materials under-going order-disorder transitions and having significant external-pressure compliance have
the highest caloric efficiency. Some of the fluorides and oxyfluorides under study can be considered promising solid coolants. 相似文献
63.
V. S. Bondarev E. A. Mikhaleva I. N. Flerov M. V. Gorev 《Physics of the Solid State》2017,59(6):1118-1126
The direct and indirect measurements of intensive electrocaloric effect in a triglycine sulfate ferroelectric crystal are performed under equilibrium and nonequilibrium thermodynamic conditions implemented in the adiabatic calorimeter. The effect of the electric field parameters (frequency, profile, and strength) on the value of the effect and degree of its reversibility are studied. The difference between the temperature variation values in a switched-on and switched-off dc field under quasi-isothermal conditions is established. The low-frequency periodic electric field induces the temperature gradient along the electrocaloric element and heat flux from its free end to the thermostated base. A significant excess of the field switching-off rate over the switching-on rate leads to a noticeable intensification of the cooling effect. 相似文献
64.
E. A. Mikhaleva I. N. Flerov A. V. Kartashev M. V. Gorev M. S. Molokeev L. N. Korotkov E. Rysiakiewicz-Pasek 《Physics of the Solid State》2018,60(7):1338-1343
The effect of restricted geometry on specific heat capacity and thermal expansion of the triglycine sulfate (TGS)–borosilicate glass composites have been studied first. A decrease in the entropy and temperature of the P21 ? P21/m phase transition in the TGS component with decreasing the glass matrix pore diameter at the invariable specific heat and thermal expansion coefficient has been observed. The estimates are indicative of the minor effect of internal pressure on the TGS pressure coefficient dTC/dp in the composites. 相似文献
65.
V. D. Fokina I. N. Flerov M. S. Molokeev E. I. Pogorel’tsev E. V. Bogdanov A. S. Krylov A. F. Bovina V. N. Voronov N. M. Laptash 《Physics of the Solid State》2008,50(11):2175-2183
Elpasolite Rb2KTiOF5 (space group, Fm $ \bar 3 Elpasolite Rb2KTiOF5 (space group, Fm
m, Z = 4) was synthesized using a solid-phase reaction method. The temperature dependences of the heat capacity, the unit cell
parameters, the structure, the permittivity, the response to an external pressure, and the Raman spectra were studied. A nonferroelectric
phase transition was revealed at T
0 = 215 K; the transition is accompanied by a tetragonal distortion of the unit cell (space group I4/m, Z = 10) and a change in the entropy (ΔS
0 = Rln8), which is anomalously large for perovskite-like oxyfluorides with atomic cations. The specific features of the mechanism
of structure distortion are discussed in combination with the previous experimental data obtained for cryolite (NH4)3TiOF5 and elpasolite Rb2KGaF6.
Original Russian Text ? V.D. Fokina, I.N. Flerov, M.S. Molokeev, E.I. Pogorel’tsev, E.V. Bogdanov, A.S. Krylov, A.F. Bovina,
V.N. Voronov, N.M. Laptash, 2008, published in Fizika Tverdogo Tela, 2008, Vol. 50, No. 11, pp. 2084–2092. 相似文献
66.
A. V. Kartashev I. N. Flerov N. V. Volkov K. A. Sablina 《Physics of the Solid State》2008,50(11):2115-2120
The temperature dependences of the intense magnetocaloric effect ΔT AD(T, H) and the heat capacity C p (T) of the (La0.4Eu0.6)0.7Pb0.3MnO3 manganite are directly measured using adiabatic calorimetry. The experimental dependences ΔT AD(T) are in satisfactory agreement with those calculated from the data on the behavior of the magnetization. The factors responsible for the absence of an anomaly in the experimental temperature dependence of the heat capacity C p (T) in the range of the magnetic phase transition are discussed. 相似文献
67.
I. N. Flerov M. V. Gorev V. D. Fokina M. S. Molokeev A. D. Vasil’ev A. F. Bovina N. M. Laptash 《Physics of the Solid State》2006,48(8):1559-1567
The heat capacity, T-p phase diagrams, and unit cell parameters of cryolite (NH4)3Ti(O2)F5 were studied over a wide temperature range. A phase transition was found near 226 K, and its thermodynamic characteristics and their dependence on the crystallization conditions were determined. The coordinates and thermal parameters of atoms in the Fm3m phase were refined. An analysis of the electron density distribution and the transition entropy showed that the mechanism of the structural transition involves, above all, rotation of the Ti(O2)F5 octahedra. Possible models of disordering of tetrahedral ammonium groups are considered. 相似文献
68.
I. N. Flerov M. V. Gorev M. L. Afanas’ev T. V. Ushakova 《Physics of the Solid State》2001,43(12):2301-2306
The heat capacity of (NH4)2KGaF6 elpasolite is measured in the temperature range from 80 to 350 K. A sequence of three phase transitions at T 1=288.5 K, T 2=250 K, and T 3=244.5 K is revealed, and the thermodynamic characteristics of these transitions are determined. The influence of hydrostatic pressure on the phase transition temperature is investigated. The results obtained are discussed within the model of orientational ordering of NH 4 + and GaF 6 3? ionic groups. 相似文献
69.
V. D. Fokina A. F. Bovina E. V. Bogdanov E. I. Pogoreltsev N. M. Laptash M. V. Gorev I. N. Flerov 《Physics of the Solid State》2011,53(10):2147-2153
The temperature dependences of the specific heat, unit cell parameters, susceptibility to hydrostatic pressure, and permittivity
of cryolite (NH4)3Nb(O2)2F4 have been studied. Phase transitions of nonferroelectric nature have been detected. Entropy parameters point to the relation
of structure distortions to ordering processes. 相似文献
70.
Yu. V. Gerasimova A. S. Oreshonkov A. A. Ivanenko M. S. Molokeev L. I. Isaenko I. N. Flerov E. V. Bogdanov M. V. Gorev A. V. Kartashev A. S. Krylov 《Physics of the Solid State》2014,56(3):599-605
The structure, infrared and Raman spectra, heat capacity, and thermal expansion have been investigated. It has been shown that, down to liquid-helium temperatures, the cubic pyrochlore structure of the CsMnMoO3F3 and CsZnMoO3F3 oxyfluorides remains stable. The influence of cation substitution on individual features of the properties of the oxyfluorides has been analyzed. 相似文献