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M.E. Mora-Ramos C.A. Duque E. Kasapoglu H. Sari I. Sökmen 《Journal of luminescence》2012,132(4):901-913
In this work we are studying the intense laser effects on the electron-related linear and nonlinear optical properties in GaAs–Ga1?xAlxAs quantum wells under applied electric and magnetic fields. The calculated quantities include linear optical absorption coefficient and relative change of the refractive index, as well as their corresponding third-order nonlinear corrections. The nonlinear optical rectification and the second and third harmonic generation coefficients are also reported. The DC applied electric field is oriented along the hererostructure growth direction whereas the magnetic field is taken in-plane. The calculations make use of the density matrix formalism to express the different orders of the dielectric susceptibility. Additionally, the model includes the effective mass and parabolic band approximations. The intense laser effects upon the system enter through the Floquet method that modifies the confinement potential associated to the heterostructure. The results correspond to several configurations of the dimensions of the quantum well, the applied electric and magnetic fields, and the incident intense laser radiation. They suggest that the nonlinear optical absorption and optical rectification are nonmonotone functions of the dimensions of the heterostructure and of the external perturbations considered in this work. 相似文献
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F. Duque A. Maanes L. M. Molina M. J. Lpez J. A. Alonso 《International journal of quantum chemistry》2002,86(2):226-238
Density functional theory is used to investigate the assembling of metallic clusters to yield stable or metastable cluster solids. Motivated by the observed high stability of the Al13H cluster, which has a substantial highest occupied and lowest unoccupied molecular orbitals (HOMO–LUMO) gap, we have modeled the assembling of those clusters. For a favorable relative orientation of each cluster with respect to all its neighbors, a cluster solid is predicted and its structure appears to be stable at least up to 150 K, which is the highest temperature in our simulations. We have also studied the chemical bonding in the stoichiometric solid alloys PbA, where A is one of the alkali elements Na, K, Rb, or Cs. Those crystals exist in an ordered phase formed by tetrahedral Pb4 clusters surrounded by the alkali atoms. The study of this family of natural cluster compounds reveals the coating role played by the cations, providing further insight into the favorable conditions required for the formation of cluster solids. © 2001 John Wiley & Sons, Inc. Int J Quantum Chem, 2001 相似文献
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The Crank–Nicolson–Galerkin finite element method for a nonlocal parabolic equation with moving boundaries
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Rui M. P. Almeida José C. M. Duque Jorge Ferreira Rui J. Robalo 《Numerical Methods for Partial Differential Equations》2015,31(5):1515-1533
The aim of this article is to establish the convergence and error bounds for the fully discrete solutions of a class of nonlinear equations of reaction–diffusion nonlocal type with moving boundaries, using a linearized Crank–Nicolson–Galerkin finite element method with polynomial approximations of any degree. A coordinate transformation which fixes the boundaries is used. Some numerical tests to compare our Matlab code with some existing moving finite element methods are investigated. © 2014 Wiley Periodicals, Inc. Numer Methods Partial Differential Eq 31: 1515–1533, 2015 相似文献
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Carmenza Duque Mónica Puyana Andrea Arias Oscar Osorno Noriyuki Hara 《Tetrahedron》2006,62(17):4205-4213
Chemical investigations of the MeOH-CH2Cl2 extract of Pseudopterogorgia elisabethae specimens collected in the islands of San Andrés and Providencia, Colombian Caribbean, yielded four new diterpenes (1, 3, 5, 7) along with seco-pseudopterosin J (8), and amphilectosins A (9) and B (10). The structures of the new compounds were established through spectral studies as an elisabethatriene analog named elisabethatrienol (1), 10-acetoxy-9-hydroxy- and 9-acetoxy-10-hydroxy-amphilecta-8,10,12,14-tetraenes (isolated as an interconverting mixture) (3), amphilecta-8(13),11,14-triene-9,10-dione (5), and a seco-pseudopterosin 7-O-α-l-fucopyranoside named seco-pseudopterosin K (7). Elisabethatrienol can be regarded as a biosynthetic intermediate leading to erogorgiaene. 相似文献