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81.
采用密度泛函理论的COSMO模型模拟了在DMF溶剂中三种不同体积的钯配体Pd(PR3)n (n=1,2) (PR3=PH3, PMe3, PtBu3)与溴苯氧化加成的反应过程. 对比双配体Pd(PR3)2的裂解能以及双配体钯Pd(PR3)2和单配体钯Pd(PR3)氧化加成过程的能垒;结果表明,小体积的配体PH3和PMe3是以双配位的形式参加氧化加成过程的,而较大体积的配体PtBu3是以单配位钯的形式参加氧化加成过程的. 相似文献
82.
Jin-Long Chen Yuo-Hsien Shiau Hung-Wen Chiu Niels Wessel Jürgen Kurths Woei-Chyn Chu 《Physica A》2010,389(9):1861-1868
Despite many previous studies on the association between hyperthyroidism and the hyperadrenergic state, controversies still exist. Detrended fluctuation analysis (DFA) is a well recognized method in the nonlinear analysis of heart rate variability (HRV), and it has physiological significance related to the autonomic nervous system. In particular, an increased short-term scaling exponent α1 calculated from DFA is associated with both increased sympathetic activity and decreased vagal activity. No study has investigated the DFA of HRV in hyperthyroidism. This study was designed to assess the sympathovagal balance in hyperthyroidism. We performed the DFA along with the linear analysis of HRV in 36 hyperthyroid Graves’ disease patients (32 females and 4 males; age 30 ± 1 years, means ± SE) and 36 normal controls matched by sex, age and body mass index. Compared with the normal controls, the hyperthyroid patients revealed a significant increase (P<0.001) in α1 (hyperthyroid 1.28±0.04 versus control 0.91±0.02), long-term scaling exponent , overall scaling exponent , low frequency power in normalized units (LF%) and the ratio of low frequency power to high frequency power (LF/HF); and a significant decrease (P<0.001) in the standard deviation of the R-R intervals (SDNN) and high frequency power (HF). In conclusion, hyperthyroidism is characterized by concurrent sympathetic activation and vagal withdrawal. This sympathovagal imbalance state in hyperthyroidism helps to explain the higher prevalence of atrial fibrillation and exercise intolerance among hyperthyroid patients. 相似文献
83.
The analytical expression for the propagation of a flattened laser beam array in a turbulent atmosphere is derived based on extended Huygens–Fresnel principle. The influence of beam order and turbulent atmosphere on beam quality is studied. It is revealed that the beam quality of a coherently combined laser beam array with higher order is better than its lower order counterpart when propagating in free-space, weak and medium turbulence (i.e. Cn2<10?13 m?2/3). The beam quality of higher order beam arrays degrades faster as the intensity of turbulence gets stronger. In the case of propagating in strong turbulence, the beam order has no influence on coherently combined beam quality. 相似文献
84.
Comparison between relay propagation and direct propagation of Gaussian-Schell-model beam in turbulent atmosphere along a slant path 下载免费PDF全文
The relay propagation of Gaussian-Schell-model in turbulent atmosphere along a slant path is studied in this paper. Based on the extended Huygens-Fresnel principle and a quadratic approximation, an analytical formula of average intensity for Gaussian-Schell-model beams in turbulent atmosphere along a slant path is derived, and some special cases are discussed. From the study and the comparison with the direct propagation, we can see that the relay propagation has an advantage over the direct propagation. When the altitude of the target is low, the peak intensity of relay propagation is much larger than that of direct propagation. However, because of the limitation of the relay system aperture for relay propagation and the variation of coherence length for direct propagation, the difference in peak intensity between the two propagations decreases with the increase of the target altitude. 相似文献
85.
Propagation of phase-locked partially coherent flattened beam array in turbulent atmosphere 总被引:2,自引:0,他引:2
Analytical formulae for phase-locked partially coherent flattened beam array propagating in a turbulent atmosphere are derived based on the extended Huygens–Fresnel principle. Beam propagation factor (BPF) is introduced to evaluate the beam quality at the receiving plane. The influence of beam order, transverse coherence width length and the intensity of turbulence is discussed in detail. 相似文献
86.
采用结构Glass/DBR/ITO/NPB/NPB:Alq/Alq/Al制作了有机微腔电致发光器件。将空穴传输材料与发光材料以一定比例混合作为发光层,为了便于对比,在不改变有机层的膜厚的情况下同时制作了传统的异质结微腔器件,发现两种器件的发光光谱有很大不同,器件的复合效率与传统的异质结器件相比也得到了很大提高,这是因为将两种有机材料混合能消除界面势垒,提高器件的复合效率,从而提高了器件的发光性能,实现了微腔双模发射,且两个模式的半峰全宽分别为8nm和12nm。通过进一步优化器件结构可以实现微腔白光发射。 相似文献
87.
Renhe Chu Jichang Yan Suoyuan Lian Yuehong Wang Fucheng Yan Dawei Chen 《Solid State Communications》2004,130(12):789-792
The interesting shape (shuttle-like, sphere with needles, uniform particles) rutile titania were prepared by the hydrolysis of TiCl4 in high acidic aqueous solution in the absence or presence of PEG-1000. PEG-1000 acted as dispersant, which could control the shape and size of the precipitate of titania. As a result, shuttle-like nanocrystalline appeared and the aggregation was improved with the increase of the amount of acid and the decrease of the concentration of TiCl4 in the absence of PEG-1000. Uniform nanoparticles were obtained in the presence of PEG-1000 and the diameter of the particles decreased with increasing the amount of PEG-1000. This process simplification will lower production cost and make continuous process possible. The products were analyzed using X-ray diffractometer, transmission electron microscopy. 相似文献
88.
89.
Tang D.L. Sun A.P. Qiu X.M. Chu P.K. 《IEEE transactions on plasma science. IEEE Nuclear and Plasma Sciences Society》2003,31(3):405-410
The absorption, reflection, and transmission of electromagnetic waves by a nonuniform plasma slab immersed in an ambient uniform magnetic field of various strengths are studied in this paper. The effects of the plasma parameters and magnetic field strength on the absorbed, reflected, and transmitted power are discussed. The magnetized nonuniform plasma slab is modeled by a series of magnetized uniform plasma subslabs. The calculation results show that the effects of the magnetic field strength and density gradient on the absorbed power, as well as the frequency band of resonant absorption, are significant. A complete analysis utilizing the scattering matrix method is also used to compare the above calculation results which neglect multiple reflections between subslab interfaces. Broadband absorption of electromagnetic waves can be achieved by changing the magnetic field strength and plasma density. More than 90% of the electromagnetic wave power can be absorbed in a magnetized nonuniform plasma slab with width of 12 cm and the absorption bandwidth can range from 1 to 20 GHz with different plasma parameters and external magnetic field strengths. 相似文献
90.
Sang Soo Lee Hyun Woo Cho Sang Kyu Lim Ki Ho Han Jin Soo Han Moo Jung Chu Je Soo Ko Kyeong-Mo Yoon Yong-Gi Lee 《光学学报》2003,23(Z1)
Transmission of 40Gbit/s NRZ signal was successfully demonstrated over 219km of installed SMF in KT's Daejeon area network. After transmission, the measured power penalty was 0.5dB for all the tributary channels. 相似文献