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201.
Aubert B Barate R Bona M Boutigny D Couderc F Karyotakis Y Lees JP Poireau V Tisserand V Zghiche A Grauges E Palano A Chen JC Qi ND Rong G Wang P Zhu YS Eigen G Ofte I Stugu B Abrams GS Battaglia M Brown DN Button-Shafer J Cahn RN Charles E Gill MS Groysman Y Jacobsen RG Kadyk JA Kerth LT Kolomensky YG Kukartsev G Lynch G Mir LM Oddone PJ Orimoto TJ Pripstein M Roe NA Ronan MT Suzuki A Troost D Wenzel WA Barrett M Ford KE Harrison TJ Hart AJ Hawkes CM Morgan SE Watson AT Goetzen K Held T Koch H 《Physical review letters》2007,98(8):081801
We report the observation of decays B{0}-->D{s}{(*)+}pi- and B{0}-->D{s}{(*)-}K+ in a sample of 230 x 10(6) Upsilon(4S)-->BB[over] events recorded with the BABAR detector at the SLAC PEP-II asymmetric-energy e+ e- storage ring. We measure the branching fractions B(B{0}-->D{s}{+}pi-)=(1.3+/-0.3(stat)+/-0.2(syst))x10(-5), B(B{0}-->D{s}{-} K+)=(2.5+/-0.4(stat)+/-0.4(syst))x10(-5), B(B{0}-->D{s}{*+}pi-)=(2.8+/-0.6(stat)+/-0.5(syst))x10(-5), and B(B{0}-->D{s}{*-}K+)=(2.0+/-0.5(stat)+/-0.4(syst))x10(-5). The significances of the measurements to differ from zero are 5, 9, 6, and 5 standard deviations, respectively. This is the first observation of B{0}-->D{s}{+}pi-, B{0}-->D{s}{*+}pi-, and B{0}-->D{s}{*-}K+ decays. 相似文献
202.
Curutchet C Scholes GD Mennucci B Cammi R 《The journal of physical chemistry. B》2007,111(46):13253-13265
This paper presents a quantum-mechanical study of electronic energy transfer (EET) coupling on over 100 pairs of chromophores taken from photosynthetic light-harvesting antenna proteins. Solvation effects due to the protein, intrinsic waters, and surrounding medium are analyzed in terms of screening and reaction field contributions using a model developed recently that combines a linear response approach with the polarizable continuum model (PCM). We find that the screening of EET interactions is quite insensitive to the quantum-mechanical treatment adopted. In contrast, it is greatly dependent on the geometrical details (distance, shape, and orientation) of the chromophore pair considered. We demonstrate that implicit (reaction field) as well as screening effects are dictated mainly by the optical dielectric properties of the host medium, while the effect of the static properties is substantially less important. The empirical distance-dependent screening function we proposed in a recent letter (Scholes, G. D.; Curutchet, C.; Mennucci, B.; Cammi, R.; Tomasi, J. J. Phys. Chem. B 2007, 111, 6978-6982) is analyzed and compared to other commonly used screening factors. In addition, we show that implicit medium effects on the coupling, resulting from changes in the transition densities upon solvation, are strongly dependent on the particular system considered, thus preventing the possibility of defining a general empirical expression for such an effect. 相似文献
203.
204.
Aubert B Bona M Boutigny D Karyotakis Y Lees JP Poireau V Prudent X Tisserand V Zghiche A Garra Tico J Grauges E Lopez L Palano A Eigen G Ofte I Stugu B Sun L Abrams GS Battaglia M Brown DN Button-Shafer J Cahn RN Groysman Y Jacobsen RG Kadyk JA Kerth LT Kolomensky YG Kukartsev G Lopes Pegna D Lynch G Mir LM Orimoto TJ Pripstein M Roe NA Ronan MT Tackmann K Wenzel WA Del Amo Sanchez P Hawkes CM Watson AT Held T Koch H Lewandowski B Pelizaeus M Schroeder T Steinke M Boyd JT Burke JP 《Physical review letters》2007,99(8):081801
We report a measurement of the time-dependent CP-asymmetry parameters S and C in color-suppressed B{0}-->D{(*)0}h{0} decays, where h{0} is a pi{0}, eta, or omega meson, and the decays to one of the CP eigenstates K+K-, K{S}{0}pi{0}, or K{S}{0}omega. The data sample consists of 383 x 10{6} Upsilon(4S)-->BB decays collected with the BABAR detector at the PEP-II asymmetric-energy B factory at SLAC. The results are S=-0.56+/-0.23+/-0.05 and C=-0.23+/-0.16+/-0.04, where the first error is statistical and the second is systematic. 相似文献
205.
Aubert B Bona M Boutigny D Karyotakis Y Lees JP Poireau V Prudent X Tisserand V Zghiche A Garra Tico J Grauges E Lopez L Palano A Eigen G Stugu B Sun L Abrams GS Battaglia M Brown DN Button-Shafer J Cahn RN Groysman Y Jacobsen RG Kadyk JA Kerth LT Kolomensky YG Kukartsev G Lopes Pegna D Lynch G Mir LM Orimoto TJ Ronan MT Tackmann K Wenzel WA del Amo Sanchez P Hawkes CM Watson AT Held T Koch H Lewandowski B Pelizaeus M Schroeder T Steinke M Walker D Asgeirsson DJ Cuhadar-Donszelmann T Fulsom BG 《Physical review letters》2007,99(7):071801
We present updated measurements of CP-violating asymmetries in the decays B0-->D*(+/-)D(-/+) and B0-->D+D- using (383+/-4) x 10(6)B(B) pairs collected by the BABAR detector at the SLAC PEP-II B factory. We determine the time-integrated CP asymmetry A(D*(+/-)D(-/+))=0.12+/-0.06+/-0.02, and the time-dependent asymmetry parameters to be C(D*+D-)=0.18+/-0.15+/-0.04, S(D*+D-)=-0.79+/-0.21+/-0.06, C(D*-D+)=0.23+/-0.15+/-0.04, S(D*-D+)=-0.44+/-0.22+/-0.06, C(D+D-)=0.11+/-0.22+/-0.07, and S(D+D-)=-0.54+/-0.34+/-0.06, where the first uncertainty is statistical and the second is systematic. 相似文献
206.
The purpose of this paper is to generalize the theory of “equal share analysis”, developed by Selten in 1972, to the one in which every player has a positive weight. We show that for any positive vector of weights, α∈R ++ N , it is always possible to find a coalition structure and a payoff vector forming a proportional regular configuration. 相似文献
207.
Željana Bonačić Lošić 《Central European Journal of Physics》2013,11(1):111-118
In this paper we study the excitation spectrum of the organic conductor tetrathiafulvalene-tetracyanoquinodimethane (TTF-TCNQ) using finite temperature calculations. The effect of electronelectron interaction is considered within the random phase approximation (RPA). Our results show the temperature dependent plasmon and dipolar mode corresponding qualitatively to the modes obtained previously using zero temperature formalism assigned to the observed excitations at 10 meV and 0.75 eV. These modes have an essential influence on the energy-loss function. The obtained results are in good qualitative agreement with the optical and EELS data of TTF-TCNQ. 相似文献
208.
Treatment of alk-2-ynyl derivatives of enantiopure phenylglycidol with NaN(3) triggers a cascade reaction consisting of stereospecific and regioselective epoxide ring opening followed by intramolecular azide-alkyne cycloaddition under strictly metal-free conditions. This simple one-pot procedure allows a fast buildup of molecular complexity, generating a wide array of triazolooxazepinols, triazolodiazepinols, and triazolothiazepinols. 相似文献
209.
Aparicio-Anglès X Clotet A Bo C Poblet JM 《Physical chemistry chemical physics : PCCP》2011,13(33):15143-15147
The adsorption of a polyoxometalate (POM) on a metal surface has been studied by means of a periodic plane wave DFT based method for the first time. In particular, we have analysed the most favourable adsorption sites of anion [SiW(12)O(40)](4-) on the Ag(111) surface and computed the infrared spectrum. Despite the intrinsic complexity of the system we have been able to fairly reproduce the observed IR spectrum and unambiguously discern the signal corresponding to W-O-Ag symmetric stretching, which appears at around 800 cm(-1). 相似文献
210.
Tyo EC Nossler M Mitrić R Bonačić-Koutecký V Castleman AW 《Physical chemistry chemical physics : PCCP》2011,13(10):4243-4249
We present the results of a reactivity study of titanium cationic clusters towards CO, C(2)H(2), C(2)H(4) and C(3)H(6) based on guided-ion-beam mass spectrometry and DFT calculations. We identified Ti(2)O(4)(+) and to a lesser extent TiO(2)(+) species which preferentially undergo oxidation reactions. An oxygen centered radical of Ti(2)O(4)(+) is responsible for selective oxidation. Energy profiles and MD simulations reveal the mechanisms of the reactions. Regeneration of the oxygen centered radical was achieved experimentally and theoretically through the reaction of N(2)O with Ti(2)O(3)(+). 相似文献