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21.
Lars Dhne Erwin Biller Helmut Baumgrtel 《Angewandte Chemie (International ed. in English)》1998,37(5):646-649
A surprisingly broad variation of absorption wavelengths within almost the whole visible region was obtained in highly oriented, thin dye layers by variation of the molecule inclination relative to the layer plane (see sketch on the right). For the first time this phenomenon caused by polaritons was demonstrated for layers of a simple streptopolymethine dye. 相似文献
22.
The temperature dependence of the FMR and EPR linewidth of bulk nickel single crystals was measured from 260 to 410°C at 9.85 GHz. A linewidth falling off rapidly with increasing temperature was found in a region above Tc: 365<T<385°C. An interpretation by the critical behaviour of the spin system is discussed. 相似文献
23.
Ahmad QR Allen RC Andersen TC Anglin JD Barton JC Beier EW Bercovitch M Bigu J Biller SD Black RA Blevis I Boardman RJ Boger J Bonvin E Boulay MG Bowler MG Bowles TJ Brice SJ Browne MC Bullard TV Bühler G Cameron J Chan YD Chen HH Chen M Chen X Cleveland BT Clifford ET Cowan JH Cowen DF Cox GA Dai X Dalnoki-Veress F Davidson WF Doe PJ Doucas G Dragowsky MR Duba CA Duncan FA Dunford M Dunmore JA Earle ED Elliott SR Evans HC Ewan GT Farine J Fergani H Ferraris AP Ford RJ Formaggio JA Fowler MM 《Physical review letters》2002,89(1):011302
The Sudbury Neutrino Observatory (SNO) has measured day and night solar neutrino energy spectra and rates. For charged current events, assuming an undistorted 8B spectrum, the night minus day rate is 14.0%+/-6.3%(+1.5%)(-1.4%) of the average rate. If the total flux of active neutrinos is additionally constrained to have no asymmetry, the nu(e) asymmetry is found to be 7.0%+/-4.9%(+1.3%)(-1.2%). A global solar neutrino analysis in terms of matter-enhanced oscillations of two active flavors strongly favors the large mixing angle solution. 相似文献
24.
Ahmad QR Allen RC Andersen TC D Anglin J Barton JC Beier EW Bercovitch M Bigu J Biller SD Black RA Blevis I Boardman RJ Boger J Bonvin E Boulay MG Bowler MG Bowles TJ Brice SJ Browne MC Bullard TV Bühler G Cameron J Chan YD Chen HH Chen M Chen X Cleveland BT Clifford ET Cowan JH Cowen DF Cox GA Dai X Dalnoki-Veress F Davidson WF Doe PJ Doucas G Dragowsky MR Duba CA Duncan FA Dunford M Dunmore JA Earle ED Elliott SR Evans HC Ewan GT Farine J Fergani H Ferraris AP Ford RJ Formaggio JA Fowler MM 《Physical review letters》2002,89(1):011301
Observations of neutral-current nu interactions on deuterium in the Sudbury Neutrino Observatory are reported. Using the neutral current (NC), elastic scattering, and charged current reactions and assuming the standard 8B shape, the nu(e) component of the 8B solar flux is phis(e) = 1.76(+0.05)(-0.05)(stat)(+0.09)(-0.09)(syst) x 10(6) cm(-2) s(-1) for a kinetic energy threshold of 5 MeV. The non-nu(e) component is phi(mu)(tau) = 3.41(+0.45)(-0.45)(stat)(+0.48)(-0.45)(syst) x 10(6) cm(-2) s(-1), 5.3sigma greater than zero, providing strong evidence for solar nu(e) flavor transformation. The total flux measured with the NC reaction is phi(NC) = 5.09(+0.44)(-0.43)(stat)(+0.46)(-0.43)(syst) x 10(6) cm(-2) s(-1), consistent with solar models. 相似文献
25.
Biller JR Meyer V Elajaili H Rosen GM Kao JP Eaton SS Eaton GR 《Journal of magnetic resonance (San Diego, Calif. : 1997)》2011,212(2):370-377
Optimization of nitroxides as probes for EPR imaging requires detailed understanding of spectral properties. Spin lattice relaxation times, spin packet line widths, nuclear hyperfine splitting, and overall lineshapes were characterized for six low molecular weight nitroxides in dilute deoxygenated aqueous solution at X-band. The nitroxides included 6-member, unsaturated 5-member, or saturated 5-member rings, most of which were isotopically labeled. The spectra are near the fast tumbling limit with T1∼T2 in the range of 0.50–1.1 μs at ambient temperature. Both spin–lattice relaxation T1 and spin–spin relaxation T2 are longer for 15N- than for 14N-nitroxides. The dominant contributions to T1 are modulation of nitrogen hyperfine anisotropy and spin rotation. Dependence of T1 on nitrogen nuclear spin state mI was observed for both 14N and 15N. Unresolved hydrogen/deuterium hyperfine couplings dominate overall line widths. Lineshapes were simulated by including all nuclear hyperfine couplings and spin packet line widths that agreed with values obtained by electron spin echo. Line widths and relaxation times are predicted to be about the same at 250 MHz as at X-band. 相似文献
26.
We report herein the synthesis of cytotoxic cyanobactin, Wewakazole B through an efficient solution-phase approach. The key steps of the synthesis are the macrocyclic lactamization of linear dodecapeptide and construction of two hexapeptides with three different substituted oxazole rings. 相似文献
27.
With the increased number of fiber-optic couplers in use in network applications, it is imperative that device reliability be ensured. Corning has developed flexible and accurate multichannel test systems for monitoring performance during environmental testing. One such single-mode system using 90 channels has been demonstrated with a one sigma stability of <0.004dB over 136 hours of testing. 相似文献
28.
Ahmad QR Allen RC Andersen TC Anglin JD Bühler G Barton JC Beier EW Bercovitch M Bigu J Biller S Black RA Blevis I Boardman RJ Boger J Bonvin E Boulay MG Bowler MG Bowles TJ Brice SJ Browne MC Bullard TV Burritt TH Cameron K Cameron J Chan YD Chen M Chen HH Chen X Chon MC Cleveland BT Clifford ET Cowan JH Cowen DF Cox GA Dai Y Dai X Dalnoki-Veress F Davidson WF Doe PJ Doucas G Dragowsky MR Duba CA Duncan FA Dunmore J Earle ED Elliott SR Evans HC Ewan GT Farine J Fergani H Ferraris AP Ford RJ 《Physical review letters》2001,87(7):071301
Solar neutrinos from (8)B decay have been detected at the Sudbury Neutrino Observatory via the charged current (CC) reaction on deuterium and the elastic scattering (ES) of electrons. The flux of nu(e)'s is measured by the CC reaction rate to be straight phi(CC)(nu(e)) = 1.75 +/- 0.07(stat)(+0.12)(-0.11)(syst) +/- 0.05(theor) x 10(6) cm(-2) s(-1). Comparison of straight phi(CC)(nu(e)) to the Super-Kamiokande Collaboration's precision value of the flux inferred from the ES reaction yields a 3.3 sigma difference, assuming the systematic uncertainties are normally distributed, providing evidence of an active non- nu(e) component in the solar flux. The total flux of active 8B neutrinos is determined to be 5.44+/-0.99 x 10(6) cm(-2) s(-1). 相似文献
29.
30.
Ahmed SN Anthony AE Beier EW Bellerive A Biller SD Boger J Boulay MG Bowler MG Bowles TJ Brice SJ Bullard TV Chan YD Chen M Chen X Cleveland BT Cox GA Dai X Dalnoki-Veress F Doe PJ Dosanjh RS Doucas G Dragowsky MR Duba CA Duncan FA Dunford M Dunmore JA Earle ED Elliott SR Evans HC Ewan GT Farine J Fergani H Fleurot F Formaggio JA Fowler MM Frame K Frati W Fulsom BG Gagnon N Graham K Grant DR Hahn RL Hall JC Hallin AL Hallman ED Hamer AS Handler WB Hargrove CK Harvey PJ Hazama R Heeger KM 《Physical review letters》2004,92(10):102004
Data from the Sudbury Neutrino Observatory have been used to constrain the lifetime for nucleon decay to "invisible" modes, such as n-->3nu. The analysis was based on a search for gamma rays from the deexcitation of the residual nucleus that would result from the disappearance of either a proton or neutron from 16O. A limit of tau(inv)>2 x 10(29) yr is obtained at 90% confidence for either neutron- or proton-decay modes. This is about an order of magnitude more stringent than previous constraints on invisible proton-decay modes and 400 times more stringent than similar neutron modes. 相似文献