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51.
J Zhu S Kais A Aspuru-Guzik S Rodriques B Brock PJ Love 《The Journal of chemical physics》2012,137(7):074112
We investigate the evolution of entanglement in the Fenna-Matthew-Olson (FMO) complex based on simulations using the scaled hierarchical equations of motion approach. We examine the role of entanglement in the FMO complex by direct computation of the convex roof. We use monogamy to give a lower bound for entanglement and obtain an upper bound from the evaluation of the convex roof. Examination of bipartite measures for all possible bipartitions provides a complete picture of the multipartite entanglement. Our results support the hypothesis that entanglement is maximum primary along the two distinct electronic energy transfer pathways. In addition, we note that the structure of multipartite entanglement is quite simple, suggesting that there are constraints on the mixed state entanglement beyond those due to monogamy. 相似文献
52.
Ji Kaifang Chen Xuegao Aldahan Ala Yi Peng Murad Ahmed Hussein Saber Alshamsi Dalal Mohamed Mohamed M. Yu Zhongbo 《Journal of Radioanalytical and Nuclear Chemistry》2020,324(3):1469-1470
Journal of Radioanalytical and Nuclear Chemistry - In the original publication of the article, the eighth author’s name and Figure 1 were published incorrectly. 相似文献
53.
This paper presents a review on kaurane diterpenes and their glycoside derivatives, covering aspects of their occurrence, biological activities and the synthesis of these natural products and their analogues. First, it shows and classifies diterpenes, in accordance with the already established structural criteria in the literature. Then, kaurane diterpenes are presented, focusing on their chemical structures, occurrence in the plant kingdom and their main, recently described, biological activities. Moreover, the most significant works, published between 1964 and November 2006, which describe the total synthesis or structural transformations of some kaurane diterpenes, including either semisynthetic and/or microbiological methodologies, are consisely reviewed. At this point, some general considerations on glycosides are introduced, and kaurane glycosides are presented and discussed on the basis of their toxic importance and occurrence in the plant kingdom, having focused on related aspects of their biological activities and the relationships between these activities and the structural factors of their molecules. Finally, the principal methods of glycosidation by enzymatic and chemical processes are both presented, and a few papers on the synthesis of kaurane glycosides are succinctly discussed. 相似文献
54.
Traffic and communication between different parts of a complex system are fundamental elements in maintaining its overall
cooperativity. Because a complex system consists of many different parts, it matters where signals are transmitted. Thus signaling
and traffic are in principle specific, with each message going from a unique sender to a specific recipient. In the current
paper we review some measures of network topology that are related to its ability to direct specific communication. 相似文献
55.
We discuss merging-and-creation as a self-organizing process for scale-free topologies in networks. Three power-law classes characterized by the power-law exponents
, 2 and
are identified and the process is generalized to networks. In the network context the merging can be viewed as a consequence of optimization related to more efficient signaling. 相似文献
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Increasingly stringent demands on the production of biopharmaceuticals demand monitoring of process parameters that impact on their quality. We developed an automated platform for on-line, near real-time monitoring of suspension cultures by integrating microfluidic components for cell counting and filtration with a high-resolution separation technique. This enabled the correlation of the growth of a human lymphocyte cell line with changes in the essential metabolic markers, glucose, glutamine, leucine/isoleucine and lactate, determined by Sequential Injection-Capillary Electrophoresis (SI-CE). Using 8.1 mL of media (41 μL per run), the metabolic status and cell density were recorded every 30 min over 4 days. The presented platform is flexible, simple and automated and allows for fast, robust and sensitive analysis with low sample consumption and high sample throughput. It is compatible with up- and out-scaling, and as such provides a promising new solution to meet the future demands in process monitoring in the biopharmaceutical industry. 相似文献
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