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IntroductionTetrathiometallateanions [MS4 ]2 - (M =Mo ,W )andtheirclusterswithvarioustransitionmetalsarewell knownfortheirrichcoordinationchemistry ,1 7andtheirrelationtoindustrialcatalysisprocess ,8biologicalsystems ,9andNLOmaterials .10 12 However,thechemistryoftheorganometallictrisulfidecomplexes [PPh4 ][(η5 C5Me5) MS3](M =Mo ,13W14 )andtheirrelatedmixed metalclus tershavebeenlessinvestigated .15,16 Inordertoextendourknowledgeaboutthechemistryof [PPh4 ][(η5 C5Me5) MS3]andconti… 相似文献
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A femtosecond laser pulse can be tailored to control the two-photon transitions using the ultra-fast pulse-shaping technique. This paper theoretically and experimentally demonstrates that two-photon transitions in molecular system with broad absorption line can be effectively controlled by square phase-modulation in frequency domain, and the influence of all parameters characterizing the square phase-modulation on two-photon transitions is systemically investigated and discussed. The obtained results have potential application in nonlinear spectroscopy and molecular physics. 相似文献
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Population trapping via quantum interference in a multi-level system driven by a coherent field is investigated. The influences of the alignment of the transition dipole moments and the energy-level separation of the upper levels are taken into account. Detailed trapping population profiles under the different conditions are given. The research result is helpful for simplifying the theoretical model and selection rational energy level system. 相似文献
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SPECIAL LINE-SHAPES OF TWO-PHOTON TRANSITIONS IN A Y-TYPE FOUR-LEVEL SYSTEM BASED ON QUANTUM INTERFERENCE 下载免费PDF全文
The experimentally observed special line-shape induced by the interaction between two counter-propagating equal-frequency fields and an Y-type four-level system with two mixed upper levels has been analyzed theoretically. Serious line-shape variations of the two-photon transitions due to the quantum interference are discussed and predicted. 相似文献