新型纳米合成物的光限幅特性研究

报道了基于富勒烯 C6 0 结构体系的零价金纳米粒子合成物的光限幅特性。使用 Z- scan技术对实验结果进行了分析。结果表明 ,材料的限幅机理主要起源于非线性吸收和吸收所致的非线性散射     

基于富勒烯纳米结构材料光限幅特性研究

应用倍频Nd:YAG脉冲激光,在波长为532nm,脉宽8ns,重复频率10Hz的条件下,研究了新型基于富勒烯纳米结构材料(C₆₀-bpy-Au)的光限幅特性.实验结果表明,其限幅特性较C₆₀有所提高,初步分析了光限幅和溶剂效应.     

飞秒激光改性6H-碳化硅晶体表面光电导增益现象研究

半绝缘6H型碳化硅(6H-SiC)具有高电阻率性质,在可见光照射下进行光电导测量时,通常光生电流很小;然而经过飞秒激光辐照改性之后,发现在可见光波段的光电导有明显的增益.本文利用紫外-可见-近红外吸收谱、X射线光电子能谱和发光光谱测量分析了激光改性之后碳化硅样品的光谱吸收、发射和晶体元素比例变化情况.分析认为碳化硅光电导增益的原因是飞秒激光辐照过程改变了碳化硅表面的硅碳元素的原子浓度比,形成新的物质结构形式,从而导致了表面光电导性能的提高.     

Measurements of femtosecond temporal speckle field of a random medium

The femtosecond temporal speckle field of a random medium is studied theoretically and experimentally. Femtosecond temporal speckle arises from the interference of multiple randomly scattered electric fields. The femtosecond temporal speckle field is measured with a cross-correlation frequency-resolved optical gating method. The spatial average of the speckle field yields a smooth transmitted profile. The speckle field is a circular complex Gaussian variable because the scattered light beams from different trajectories have no correlation with each other. The field and the intensity profiles of individual speckle spots fluctuate randomly in time. The ensemble average of the temporal intensity profiles converges, thereby yielding the photon travel time probability distribution function.     

Surface mico-structures on amorphous alloys induced by vortex femtosecond laser pulses

This paper investigates the generation of self-organized surface structures on amorphous alloys by vortex femtosecond laser pulses. The scanning electron microscope characterizations show that the as-formed structures are periodic ripples, aperiodic ripples, and `coral-like' structures. Optimal conditions for forming these surface structures are determined in terms of pulses number at a given pulse energy. The applicable mechanism is suggested to interpret the formation and evolution of the `coral-like' structures.     

用反射式达曼光栅产生飞秒激光双脉冲

采用反射式达曼光栅建立了一种产生飞秒激光双脉冲的新装置.由于采用反射式结构，避免了材料色散和吸收导致的脉冲畸变，并构建了一台二次谐波-频率分辨光学开关装置对产生的双脉冲进行了测量.实验结果表明可以实现脉冲强度相等、时间宽度相同、不同间隔的双脉冲输出.产生双脉冲的装置在飞秒激光领域有着应用的价值. 关键词： 飞秒激光双脉冲 达曼光栅 二次谐波-频率分辨光学开关     

基于富勒烯C60结构体系的金纳米粒子合成物光学非线性研究

使用532nm,8ns激光脉冲研究了两种新型的基于富勒烯C₆₀结构体系的金纳米粒子合成物的光学非线性.Z-scan实验结果和理论分析的比较表明,材料的非线性吸收强烈地依赖于材料中的配合体,而非线性折射主要来自金纳米粒子的贡献.而且与熟知的C₆₀甲苯溶液光限幅特性作了比较,分析了光限幅机理. 关键词： 60结构体系')" href="#">基于富勒烯C₆₀结构体系 金纳米粒子 等离子体 光限幅     

The effects of heat treatment on microfluidic devices fabricated in silica glass by femtosecond lasers

We fabricated complex microfluidic devices in silica glass by water-assisted femtosecond laser ablation and subsequent heat treatment.The experimental results show that after heat treatment,the diameter of the microchannels is significantly reduced and the internal surface roughness is improved.The diameters of the fabricated microchannels can be modulated by changing the annealing temperature and the annealing time.During annealing,the temperature affects the diameter and shape of the protrusions in microfluidic devices very strongly,and these changes are mainly caused by uniform expansion and the action of surface tension.     

Properties and Stability of Nanosecond Optical Limiting of Gold Nanoclusters

Optical limitation(OL) performances of the gold nanoclusters protected by C60-tpy have been investigated with 8 ns pulses at 532nm.The experimental results show that the nanocomposite possesses OL effects superior to C60 in toluene.The main mechanism of OL is attributed to the nonlinear absorption and subsequently induced nonlinear scattering during excitation of the pulse.Ageing of the nanocomposite chloroform solution in air lowers the OL performances by a factor of 2.4,which can be due to the formation of aggregates of large gold particles.     

激光诱导玻璃内部金纳米颗粒的析出及光谱

使用钛宝石飞秒激光引发和热处理相结合，实现了在含有金离子的硅酸盐玻璃内部，有空间选择性地析出金纳米颗粒。对吸收光谱的研究表明，随着热处理温度的升高，吸收峰强度增大且红移；随着激光功率密度的增大，金纳米颗粒也增大。在特定的激光和热处理条件作用下，可以在玻璃内部有空间选择性的使金离子还原后聚集，形成金纳米颗粒，具有量子尺寸效应。改变激光功率和热处理温度可以控制所析出的金属纳米粒子的尺寸，从而实现多色显示，飞秒激光诱导金纳米颗粒具有稳定性，颜色具有持久性。