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We report the results of 7Li nuclear magnetic resonance (NMR) studies of LiVGe2O6, a quasi-one-dimensional spin S = 1 model system, at low temperatures. Our data, including NMR spectra and the temperature dependence of the spin-lattice relaxation rate T-11, indicate that a first-order phase transition occurs at T(c) approximately 23 K. The NMR response of LiVGe2O6 below T(c) suggests that the ordered phase is antiferromagnetic and has unusual features. Possible reasons for this unexpected behavior are discussed. 相似文献
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B. Pedrini S. Wessel J. L. Gavilano H. R. Ott S. M. Kazakov J. Karpinski 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,55(3):219-228
We report results of susceptibility χ and 7Li NMR measurements on LiVSi2O6. The temperature dependence of the magnetic susceptibility χ(T) exhibits a broad maximum, typical for low-dimensional magnetic
systems. Quantitatively it is in agreement with the expectation for an S=1 spin chain, represented by the structural arrangement
of V ions.
The NMR results indicate antiferromagnetic ordering below TN=24 K. The intra- and interchain coupling J and Jp for LiVSi2O6, and also for its sister compounds LiVGe2O6, NaVSi2O6 and NaVGe2O6, are obtained via a modified random phase approximation which takes into account results of quantum Monte Carlo calculations.
While Jp is almost constant across the series, J varies by a factor of 5, decreasing with increasing lattice constant along the chain
direction. The comparison between experimental and theoretical susceptibility data suggests the presence of an easy-axis magnetic
anisotropy, which explains the formation of an energy gap in the magnetic excitation spectrum below TN, indicated by the variation of the NMR spin-lattice relaxation rate at T≪TN. 相似文献
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P. Vonlanthen J.L. Gavilano B. Ambrosini H.R. Ott Y. Aoki H. Sugawara H. Sato 《The European Physical Journal B - Condensed Matter and Complex Systems》1999,9(1):15-20
We report the results of 69Ga- and 71Ga-NMR measurements on NdGa2 at temperatures between 0.1 and and in applied magnetic fields between zero and 74 kOe. NdGa2 orders antiferromagnetically below and undergoes several metamagnetic transitions in external magnetic fields. In zero applied magnetic field and below the temperature dependence of the spin-lattice relaxation rate T1
-1
(
T
) shows a large linear-in-T term, about two orders of magnitude higher than for the reference compound LaGa2. This strong enhancement confirms the presence of low-energy excitations in the antiferromagnetic phase of NdGa2 as was previously indicated by specific heat data. Above , T1
-1
(
T
) is dominated by an exponential term, which we associate with excitations between the lowest energy levels of the f-electron system. The separation of these energy levels is determined by exchange, crystal-field and Zeeman interactions.
Received 3 September 1998 and Received in final form 3 November 1998 相似文献
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B. Ambrosini J.L. Gavilano P. Vonlanthen H.R. Ott 《Zeitschrift für Physik B Condensed Matter》1997,104(3):523-528
We report results of 89Y-NMR measurements on U0.2Y0.8Pd3 as well as YPd3, performed at frequencies between 9 and 16MHz and at temperatures between 0.25 and 2 K. In this temperature range the average Knight shift is +0.5%, temperature-independent and the same for both materials. Also the NMR linewidth for both compounds was found to be temperature and field independent but one order of magnitude larger for U0.2Y0.8Pd3 than for YPd3. For U0.2Y0.8Pd3 our results indicate a distribution of internal static fields at the Y sites and a small temperature-dependent enhancement of the spin-lattice relaxation rate T 1 ?1 with respect to YPd3. The NMR spectra are consistent with the presence of very small frozen U moments, but the temperature dependence of the spin-lattice relaxation rate indicates a more complicated situation. In particular (T1T)?1 shows an anomalous temperature dependence. 相似文献
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Thermodynamic calculations, developed here, show that a considerable fraction of the observed low-temperature nuclear spin-lattice relaxation rate and specific heat of CeAl2-both varying linearly with temperature-may be due to the existence of new low-frequency features in the spin-excitation spectrum of incommensurate magnetic structures. 相似文献
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We report the results of measurements of the dc susceptibility and the 23Na-NMR response of Na2V3O7, a recently synthesized, nonmetallic low dimensional spin system. Our results indicate that, upon reducing the temperature to below 100 K, the V4+ moments are gradually quenched, leaving only one moment out of nine active. The NMR data reveal a phase transition at very low temperatures. With decreasing applied field H, the critical temperature shifts towards T=0 K, suggesting that Na2V3O7 may be regarded as an insulator reaching a quantum critical point at H=0. 相似文献
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Egetenmeyer N Gavilano JL Maisuradze A Gerber S MacLaughlin DE Seyfarth G Andreica D Desilets-Benoit A Bianchi AD Baines Ch Khasanov R Fisk Z Kenzelmann M 《Physical review letters》2012,108(17):177204
We report on muon spin rotation studies of the noncentrosymmetric heavy fermion antiferromagnet CeRhSi3. A drastic and monotonic suppression of the internal fields, at the lowest measured temperature, was observed upon an increase of external pressure. Our data suggest that the ordered moments are gradually quenched with increasing pressure, in a manner different from the pressure dependence of the Néel temperature. At 23.6 kbar, the ordered magnetic moments are fully suppressed via a second-order phase transition, and T(N) is zero. Thus, we directly observed the quantum critical point at 23.6 kbar hidden inside the superconducting phase of CeRhSi3. 相似文献