废生物质衍生碳修饰多孔石墨氮化碳异质结用于海水中氧四环素的高效光降解

以香蕉皮(BP)和尿素为原料,采用单步热处理工艺合成了一种无金属光催化剂。生物质衍生碳(BC)与多孔石墨相氮化碳(pg-C₃N₄)间的紧密界面效应显著增加了复合材料(pg-C₃N₄/BC)的比表面积,扩大了光响应范围,并提升了光诱导电子的迁移速率及光催化剂的稳定性。在可见光照射70 min后,pg-C₃N₄/BC降解人工海水中氧四环素(OTC)的反应速率常数为pg-C₃N₄的9.4倍。另外,由于光生电荷分离和转移的促进作用,pg-C₃N₄/BC在连续流反应过程中对OTC也具有更优异的光催化降解效果。此外,提出了一种潜在的光催化机制,以解释pg-C₃N₄/BC复合材料性能增强的原因。     

Ordered C*-Modules

In this first part of a study of ordered operator spaces, wedevelop the basic theory of ‘ordered C^*-bimodules’.A crucial role is played by ‘open tripotents’, aJB^*-triple variant of Akemann's notion of open projection. 2000Mathematics Subject Classification 46L08, 47L07 (primary), 46L07,47B60, 47L05 (secondary).     

Subspaces of L(H) That Are *-Invariant

A result of Choi and Effros says how *-invariant spaces of bounded operators on Hilbert space that contain the identity can be abstractly characterized in terms of their order structure. The aim here is to dispose of the identity and to prove a similar theorem for spaces of bounded operators that are merely *-invariant. Absence of a unit will also permit to deal with duals in a satisfactory way.