γ-ray spectroscopy of excited states in 61 30Zn31

The ⁶¹ ₃₀Zn₃₁ isotope has been produced at the Oak Ridge National Laboratory in the fusion-evaporation reaction ⁴⁰Ca(²⁴Mg, 2pn)⁶¹Zn at 104MeV. The experimental set-up allowed γ-rays to be detected in the CLARION Ge detector array in coincidence with the detection of recoiling nuclei in the focal plane at the end of the recoil mass spectrometer. This provides a unique identification of γ-rays belonging to ⁶¹Zn. The excited states have been explored by means of recoil- γγ coincidences, and the resulting decay scheme comprises almost 70 transitions. The data reveal numerous non-yrast states and suggest a revised spin and parity assignment for a previously observed superdeformed band. The resulting decay scheme is compared to predictions from different sets of large-scale shell model calculations.     

Critical exponents of uranium telluride

Neutron and magnetization experiments have been used to determine the critical exponents β, γ and δ of the ferromagnet UTe, T_c = 100.7(3) K, near the Curie temperature. The values are β = 0.291(4), γ = 1.326(9) and δ = 5.23(7). Comparisons are made with values from other ferromagnetic systems.     

Zur Halbwertszeit des 1,49 MeV-Niveaus im Co57

For the halflife of the 1,49 MeV state in Co⁵⁷ an upper limit of 3,0 × 10^?10 sec. has been found.     

Incomplete fusion in 12C+160Gd collisions

The mechanism of the production of fast α-particles in ¹²C induced reactions was studied over a wide range of bombarding energies (7.5–16.7 MeV/A) by measuring α-γ coincidences. Absolute cross sections for ${}^{160}\text{Gd}\text{(}{}^{12}\text{C}\text{, αx}\text{n}\text{)}{}^{\mathrm{168?x}}\text{Er and}{}^{160}\text{Gd}\text{(}{}^{12}\text{C}\text{, 2αx}\text{n}\text{)}{}^{\mathrm{164?x}}\text{Dy}$ reactions, as well as inclusive α-particle production cross sections, have been determined. Depending on the bombarding energy, a fraction of 0.2–0.4 of the singles α-particles can be explained as resulting from incomplete fusion reactions (¹²C, α) and (¹²C, 2α) which correspond to a capture of “⁸Be” and “⁴He”, respectively. The remaining fragments of the projectile have, on the average, the beam-velocity energies and their angular distributions are forward peaked. Distributions of side-feeding to the yrast bands in the target-residue nuclei indicate that low partial waves are strongly hindered in the incomplete fusion reactions. The energy dependence of the cross sections for (¹²C, α) and (¹²C, 2α) incomplete fusion as well as for (¹²C, 3α) projectile breakup is given. A generalized concept of critical angular momentum which explains a competition between complete fusion, incomplete fusion and breakup reactions is proposed.     

Neutron diffraction study of UAs in high magnetic fields

Magnetization experiments have shown that at low temperature and in an applied magnetic field of ～90 kOe antiferromagnetic (AF) uranium arsenide transforms to a new ferrimagnetic state. The high-field transition produces a state with magnetic components $\text{parallel}$ to the applied field. A small ferromagnetic component (0.4 μ_B) is seen in magnetization experiments but with neutron diffraction we have observed directly the large AF component (～ 1.8 μ_B) which has a $\text{q}$ value of 0.58 ± 0.01 $\text{c}$¹ in contrast to the zero field type IA structure with $\text{q}\text{= (0,0,0.50)}$. This transition is quite different from that occuring in the conventional spin-flop transition.     

Uranium oligomerization in chloride-based high temperature melts: in situ XAS studies

In situ EXAFS spectroscopic studies of uranium compounds in high temperature alkali chloride melts indicate the presence of oligomeric species. An investigation into UCl(3) and UCl(4) dissolved in LiCl reveals long range ordering of uranium atoms in the molten state which is not maintained on quenching. Studies of uranium dioxide dissolved in LiCl-KCl eutectic with HCl exhibit long range ordering in both molten and quenched states, and the EXAFS data can be modeled using multiple coordination shells.