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351.
Timothy I. Mattox James P. Larentzos Stan G. Moore Christopher P. Stone Daniel A. Ibanez Aidan P. Thompson 《Molecular physics》2018,116(15-16):2061-2069
ABSTRACTSimulating energetic materials with complex microstructure is a grand challenge, where until recently, an inherent gap in computational capabilities had existed in modelling grain-scale effects at the microscale. We have enabled a critical capability in modelling the multiscale nature of the energy release and propagation mechanisms in advanced energetic materials by implementing, in the widely used LAMMPS molecular dynamics (MD) package, several novel coarse-graining techniques that also treat chemical reactivity. Our innovative algorithmic developments rooted within the dissipative particle dynamics framework, along with performance optimisations and application of acceleration technologies, have enabled extensions in both the length and time scales far beyond those ever realised by atomistic reactive MD simulations. In this paper, we demonstrate these advances by modelling a shockwave propagating through a microstructured material and comparing performance with the state-of-the-art in atomistic reactive MD techniques. As a result of this work, unparalleled explorations in energetic materials research are now possible. 相似文献
352.
Stan Chiriţă Alexandre Danescu 《International Journal of Solids and Structures》2008,45(17):4850-4859
The present paper studies the strong ellipticity for all crystal classes of tetragonal system in a linearly elastic material. Explicit conditions characterizing the strong ellipticity of the elasticity tensor are established for the tetragonal system with six elasticities (that is tetragonal–scalenohedral, ditetragonal–pyramidal, tetragonal–trapezohedral, ditetragonal–dipyramidal crystal classes) as well as for the tetragonal system with seven elasticities (tetragonal–disphenoidal, tetragonal–pyramidal and tetragonal–dipyramidal crystal classes). 相似文献
353.
The combination of on-line methylation using trimethylsulfonium hydroxide with large volume injection of 100 μL was evaluated for the analysis of organic acids and phenols in water. Solvent split injection was applied with complete evaporation of the solvent before analytes were transferred onto the GC column. Despite complete solvent removal, losses were very low compared to conventional splitless injection even for volatile acidic compounds such as propionic acid and phenol. This is explained by intermediate formation of low volatility trimethylsulfonium salts of the analytes which were held in the injector for long evaporation times of up to 10 min, if the evaporation temperature was as low as 10°C. Using a simple liquid/liquid extraction procedure, volatile fatty acids, dicarboxylic acids, benzoic acids and phenols could be detected in 5 mL of water at concentrations of 0.04–0.1 μmol/L with GC/MS in full scan mode. Lactic, pyruvic, and also malonic acids could only be detected at higher levels because of their limited extractability from water as well as their poorer methylation yields. The method provides an easy way to sensitively detect acidic compounds of medium to high volatility in water. It was applied for screening of organic acids and phenols in batch cultures of anaerobic bacteria of which one example is shown. 相似文献
354.
In this paper a mono–objective optimum design procedure for a six–degree of freedom parallel micro robot is outlined by using optimality criterion of workspace and numerical aspects. A mono–objective optimization problem is formulated by referring to a basic performance of parallel robots. Additional objective functions can be used to extend the proposed design procedure to more general but specific design problems. A kinematic optimization was performed to maximize the workspace of the mini parallel robot. Optimization was performed using Genetic Algorithms. (© 2008 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim) 相似文献
355.
356.
This paper applies a general Bayesian inference approach, based on Bayesian evidence computation, to geoacoustic inversion of interface-wave dispersion data. Quantitative model selection is carried out by computing the evidence (normalizing constants) for several model parameterizations using annealed importance sampling. The resulting posterior probability density estimate is compared to estimates obtained from Metropolis-Hastings sampling to ensure consistent results. The approach is applied to invert interface-wave dispersion data collected on the Scotian Shelf, off the east coast of Canada for the sediment shear-wave velocity profile. Results are consistent with previous work on these data but extend the analysis to a rigorous approach including model selection and uncertainty analysis. The results are also consistent with core samples and seismic reflection measurements carried out in the area. 相似文献
357.
Stan?AlamaEmail authorView authors OrcID profile Lia?Bronsard Xavier?Lamy 《Journal of Nonlinear Science》2018,28(4):1443-1465
We consider a nematic liquid crystal occupying the exterior region in \({\mathbb {R}}^3\) outside of a spherical particle, with radial strong anchoring. Within the context of the Landau-de Gennes theory, we study minimizers subject to an external field, modeled by an additional term which favors nematic alignment parallel to the field. When the external field is high enough, we obtain a scaling law for the energy. The energy scale corresponds to minimizers concentrating their energy in a boundary layer around the particle, with quadrupolar symmetry. This suggests the presence of a Saturn ring defect around the particle, rather than a dipolar director field typical of a point defect. 相似文献
358.
359.
In this paper we consider the state of plane strain in an elastic material with voids occupying a curvilinear strip as an arch‐like region described by R: a<r<b, 0<θ<ω, where r and θ are polar coordinates and a, b, and ω (<2π) are prescribed positive constants. Such a curvilinear strip is maintained in equilibrium under self‐equilibrated traction and equilibrated force applied on one of the edges, whereas the other three edges are traction free and subjected to zero volumetric fraction or zero equilibrated force. In fact, we study the case when one right or curved edge is loaded. Our aim is to derive some explicit spatial estimates describing how some appropriate measures of a specific Airy stress function and volume fraction evolve with respect to the distance to the loaded edge. The results of the present paper prove how the spatial decay rate varies with the constitutive profile. For the problem corresponding to a loaded right edge, we are able to establish an exponential decay estimate with respect to the angle θ. Whereas for the problem corresponding to a loaded curved edge, we establish an algebraical spatial decay with respect to the polar distance r, provided the angle ω is lower than the critical value $\pi\sqrt{2}$. The intended applications of these results concern various branches of medicine as for example the bone implants. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
360.
Stan Bondzyski 《Fresenius' Journal of Analytical Chemistry》1893,32(1):296-302
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