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991.
Transforming Computed Energy Landscapes into Experimental Realities: The Role of Structural Rugosity
Dr. Riccardo Montis Prof. Roger J. Davey Sarah E. Wright Dr. Grahame R. Woollam Dr. Aurora J. Cruz-Cabeza 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(46):20537-20540
We exploit the possible link between structural surface roughness and difficulty of crystallisation. Polymorphs with smooth surfaces may nucleate and crystallise more readily than polymorphs with rough surfaces. The concept is applied to crystal structure prediction landscapes and reveals a promising complementary way of ranking putative crystal structures. 相似文献
992.
Roger C Walker II Hossein Hamedi William Hunter Woodward Michael Lanagan 《Journal of polymer science. Part A, Polymer chemistry》2020,58(22):3142-3152
Cross-linked polyethylene (XLPE) is notable for its use as power cable insulation. Its longevity is limited by space charge buildup linked to impurities such as the byproducts left behind by the cross-linking agent dicumyl peroxide (DCP). The goal of this work is to determine the impacts of these byproducts on charge trapping and detrapping in XLPE using the thermally stimulated depolarization current technique. XLPE with byproducts has one source of trapped charge, which originates from the byproducts. XLPE that was thermally treated via degassing exhibits two other sources of trapped charge, which are charge injection and dipolar relaxations. Oxidation from degassing was shown to control the trapping from these sources, which is useful knowledge for processing this material prior to its use. Reintroducing acetophenone, one of the major byproducts of DCP, suppresses those two peaks once more, showing that it controls the overall space charge buildup characteristics in XLPE. 相似文献
993.
Structural Chemistry - A cluster of 10 vanadium (5+) atoms bridged by 22 oxygen atoms and having six of the vanadiums around the periphery each bound to a single bidentate acetylacetone is... 相似文献
994.
995.
A supply chain design problem based on a two-echelon single-product system is addressed. The product is distributed from plants to distribution centers and then to customers. There are several transportation channels available for each pair of facilities between echelons. These transportation channels introduce a cost?Ctime tradeoff in the problem that allows us to formulate it as a bi-objective mixed-integer program. The decisions to be taken are the location of the distribution centers, the selection of the transportation channels, and the flow between facilities. Three variations of the classic ??-constraint method for generating optimal Pareto fronts are studied in this paper. The procedures are tested over six different classes of instance sets. The three sets of smallest size were solved completely obtaining their efficient solution set. It was observed that one of the three proposed algorithms consistently outperformed the other two in terms of their execution time. Additionally, four schemes for obtaining lower bound sets are studied. These schemes are based on linear programming relaxations of the model. The contribution of this work is the introduction of a new bi-objective optimization problem, and a computational study of the ??-constraint methods for obtaining optimal efficient fronts and the lower bounding schemes. 相似文献
996.
This paper proves Hua's Theorem and, from this, the Fundamental Theorem of Projective Geometry for the projective line over a commutative ring with “many units”. 相似文献
997.
998.
Roger Waldeck 《Computational & Mathematical Organization Theory》2016,22(2):135-160
Criminal behavior has been explained in the literature by rational or normative arguments. We propose a game theory framework of criminal behavior integrating both concepts. Specifically the modeling includes three factors, namely the gain from criminality, the adherence to a legal norm and social pressure from criminal peers. We show that criminality cannot be lower with increasing gain from criminality, lower adherence to the legal norm or higher social pressure from criminal peers. Finally, we observe by agent-based simulations that small local interaction structures lead to spatial segregation in criminality in the case where a polymorphic equilibrium is expected. 相似文献
999.
Despite its huge potential in risk analysis, the Dempster–Shafer Theory of Evidence (DST) has not received enough attention in construction management. This paper presents a DST-based approach for structuring personal experience and professional judgment when assessing construction project risk. DST was innovatively used to tackle the problem of lacking sufficient information through enabling analysts to provide incomplete assessments. Risk cost is used as a common scale for measuring risk impact on the various project objectives, and the Evidential Reasoning algorithm is suggested as a novel alternative for aggregating individual assessments. A spreadsheet-based decision support system (DSS) was devised to facilitate the proposed approach. Four case studies were conducted to examine the approach's viability. Senior managers in four British construction companies tried the DSS and gave very promising feedback. The paper concludes that the proposed methodology may contribute to bridging the gap between theory and practice of construction risk assessment. 相似文献
1000.