New terahertz dispersive device for single-shot spectral measurements of terahertz pulse

A new terahertz dispersive device designed for single-shot spectral measurements of broadband terahertz pulses is proposed. With two-dimensional quasi-randomly distributed element design, the device exhibits approximately the dispersive property of single-order diffraction in far field. Its far-field diffraction pattern is experimentally verified employing a continuous terahertz source centered at 2.52 THz and a pyroelectric focal-plane-array camera, which is in good agreement with the numerical result. The device provides a new approach for direct single-shot spectral measurements of broadband terahertz waves.     

离线测量钍快中子裂变反应率方法

钍快中子裂变反应率是钍铀燃料循环中的重要数据.为了测量基于聚变-裂变混合能源堆包层概念设计的钍样品在宏观中子学装置中的钍快中子裂变数据,发展了钍快中子裂变率的离线活化γ测量方法.通过测量232Th裂变碎片85mKr的β衰变产物85Rb发射的151.16 keV特征γ射线,并结合钍裂变产额数据,获得了钍样品装置中232Th裂变反应率的分布.详细介绍了此方法的原理和影响因素,并利用14 MeV的D-T中子源在贫铀球壳中开展了校验实验,实验不确定度为5.3%—5.5%.采用MCNP5程序和ENDF/B-VI及ENDF/B-VII数据库模拟计算的结果与实验结果在实验不确定度内基本符合,这证明该方法能够有效地模拟装置中232Th裂变反应率.     

以光子计数技术为基础的极低照度测量

微照度计的测量灵敏度通常限于1×10~(-6)lx水平,这在许多场合都不能满足要求。但只要确定了光通量与光子速率之间的内在联系,利用光子计数器和微照度计的结合,就可以把微照度的测量灵敏度提高到1×10~(-10)lx水平。文中导出了光通量与光子速率的理论计算公式;介绍了极低照度测量实验系统;并根据光子计数器的时间分辨率和光子的泊松分布以及暗记数水平,分别分析了微照度测量的上、下限范围。     

黑腔靶中超热电子特性研究

近几年来,在“神光”装置上进行了1.053μm激光与平面靶及一系列柱形黑腔靶相互作用实验。用一台多道滤波—荧光X光能谱仪(FFS)测得各种靶发射的超热X射线谱,由谱推导超热电子温度T_h和超热电子总能量E_h当照射靶单束激光能量E_(tar)为400～670J、脉宽τ=650～1150ps时,发现黑腔内明显存在两群服从Maxwell分布高能电子(T_h=35～45keV;T_(hh)=150～350kev),而且E_(he)占E_(tar)的份额为10％～12％。实验还表明:腔内的E_(he)与非线性过程特征量(SRS)有较好的线性关系,因此推断出腔内超热电子产生的主要机制是受激Raman散射。在相同照射条件下,黑腔靶产生的超热电子比平面靶严重。     

Design of Enhanced Catalysts by Coupling of Noble Metals (Au,Ag) with Semiconductor SnO2 for Catalytic Reduction of 4‐Nitrophenol

The reduction of 4‐nitrophenol (Nip) into 4‐aminophenol (Amp) by NaBH₄, which is catalyzed by both binary and ternary yolk–shell noble‐metal/SnO₂ heterostructures, is reported. The binary heterostructures contain individual Au or Ag nanoparticles (NPs) and the ternary heterostructures contain both Au and Ag NPs. The Au@SnO₂ yolk–shell NPs are synthesized via a silica seeds‐mediated hydrothermal method. Subsequently, the Au@SnO₂@Ag and Au@SnO₂@Au yolk–shell–shell (YSS) NPs are synthesized, whereby SnO₂ is located between the Au and Ag NPs. The morphology, composition, and optical properties of the as‐prepared samples are analyzed. For the binary heterostructures, the rate of the reduction reaction increases with decreasing particle size. The catalytic results demonstrate the synergistic effect of Au and Ag in the ternary metal–semiconductor heterostructures, which is beneficial to the catalytic reduction of Nip into Amp. Both the binary and ternary heterostructures exhibit significantly better catalytic performances than the corresponding bare Au and Ag NPs. It is envisaged that the current synthesized strategy will promote further interest in the field of bimetal NP‐based catalysis.     

含有AlGaAs插入层的InAs/GaAs三色量子点红外探测器

本文报道了采用分子束外延技术制备的三色InAs/GaAs量子点红外探测器. 器件采用nin型结构, 吸收区结构是在InGaAs量子阱中生长含有AlGaAs插入层的InAs量子点, 器件在77 K下的红外光电流谱有三个峰值: 6.3, 10.2和11 μm. 文中分析了它们的跃迁机制, 并且分别进行了指认. 因为有源区采用了不对称结构, 所以器件在外加偏压正负方向不同时, 光电流谱峰值的强度存在一些差异. 不论在正偏压或者负偏压下, 当偏压达到较高值, 再进一步增大偏压时, 都出现了对应于连续态的跃迁峰强度明显下降的现象, 这是由量子点基态与阱外连续态的波函数交叠随着偏压进一步增大而迅速减小导致的.     

Application of the first collision source method to CSNS target station shielding calculation

Ray effects are an inherent problem of the discrete ordinates method. RAY3 D, a functional module of ARES, which is a discrete ordinates code system, employs a semi-analytic first collision source method to mitigate ray effects. This method decomposes the flux into uncollided and collided components, and then calculates them with an analytical method and discrete ordinates method respectively. In this article, RAY3 D is validated by the Kobayashi benchmarks and applied to the neutron beamline shielding problem of China Spallation Neutron Source(CSNS)target station. The numerical results of the Kobayashi benchmarks indicate that the solutions of DONTRAN3 D with RAY3 D agree well with the Monte Carlo solutions. The dose rate at the end of the neutron beamline is less than10.83 μSv/h in the CSNS target station neutron beamline shutter model. RAY3 D can effectively mitigate the ray effects and obtain relatively reasonable results.     

闪光X射线高速摄影荧光转换屏的设计和性质研究

本文描述了用于中间弹道高速摄影荧光转换屏的设计特点、性能测试和实验结果。文中讨论了Gd2O2S:Tb和(Zn,Cd)S对X射线的吸收系数、发光效率以及荧光光谱与变象管S-20阴极光谱灵敏度曲线相匹配的相关曲线;测试了转换屏的相对发光强度、分辨率及其余辉。实验证明本屏发光亮度比钨酸钙屏高60倍左右,屏分辩率达51p/mm,余辉时间为8μs,多幅摄影结果证明第一幅的图象对第二幅照片无“拖尾”现象,本屏已达到了中间弹道高速摄影转换屏的实用水平。