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41.
The low-frequency Raman scattering spectra of the DKDP ferroelectric crystal are studied in the temperature range 30–393 K. At temperatures above 150 K, the Raman spectra exhibit a central peak which reflects the lattice relaxation susceptibility. The width and integrated intensity of the central peak are derived from the experimental spectra. The critical slowing down of the relaxation response predicted by the Ginzburg-Landau-Devonshire theory is observed throughout the temperature range in which the central peak persists. Its integrated intensity does not, however, follow the predictions of the theory and reveals a strong temperature dependence in the ferroelectric phase and a weaker dependence in the paraphase. It is shown that the thermal activation law describes well the temperature dependence of the intensity of the central peak. An interpretation is proposed according to which the intensity of order parameter fluctuations is related to the activation barrier whose height is proportional to the deviation from the phase transition temperature.  相似文献   
42.
The temperature dependence of the viscosity of water in the range of 240–340 K has been studied by the molecular dynamics method. The analysis of the data has revealed an anomaly in the behavior of the viscosity of water near 0°C. The appearance of this anomaly has been attributed to the formation of cluster structures at a decrease in the temperature.  相似文献   
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We demonstrate the strong dependence of the entanglement dynamics of two distinguishable qubits in a trap on the relative phase of the pulses used for excitation. We show that the population and entanglement exhibits collapses and full revivals when the initial distribution of phonons is a coherent state.  相似文献   
44.
The generation of the second optical harmonic in a series of SBN-x crystals (x = 0.75, 0.61, 0.50, 0.33) is studied in the 200–900 K temperature range. It is shown that the spectral width of nonlinear response in all samples is less than 1 cm?1 and does not depend on the temperature. Its integral intensity follows the Arrhenius law. The parameters of this Arrhenius presentation are determined and compared with the corresponding parameters for a number of ferroelectrics and relaxors.  相似文献   
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48.
By dynamic Stark shift using strong nonresonant pulses, we show that it is in principle possible to prepare arbitrary superposition states of mixed multiplicity. By a proper choice of parameters, the transfer of population is shown to follow the Rabi formula, where the initial and target states are now vibrational states of two light-induced molecular potentials of different multiplicity. Starting from nonstationary wave packets, the spin transfer can proceed via parallel transfer using a single pulse or by sequential transfer using a pulse sequence. A simple model is proposed to analyze the properties of both schemes and the feasibility of their experimental implementation for spin-orbit transitions in Rb2.  相似文献   
49.
This article overviews recent developments in the use of multicollector inductively coupled plasma mass spectrometry (MC-ICPMS) in studies of mass-independent isotope chemistry of heavy elements. Origins of mass-independent isotope effects and their relevance to isotope ratio measurements by MC-ICPMS are briefly described. The extent to which these effects can affect instrumental mass bias in MC-ICPMS is critically discussed on the basis of the experimental observations. Furthermore, key findings reported in studies of mass-independent isotope fractionation (MIF) of mercury in the field of environmental sciences are reviewed. MIF of heavy elements is not only of interest from a fundamental point of view, but also provides scientists with a new and effective means of studying the biogeochemistry of these elements.  相似文献   
50.
We have studied the dynamics of intramolecular vibrational redistribution (IVR) from the initially excited mode v1 ≈ 3330 cm−1 (acetylene-type H-C bond) in H-C≡C-CF3 molecules in the gaseous phase by means of anti-Stokes spontaneous Raman scattering. The time constant of this process is estimated as 2.3 ns—this is the slowest IVR time reported so far for the room-temperature gases. It is suggested that so long IVR time with respect to the other propyne derivatives can be explained by a larger defect, in this case, of the Fermi resonance of v1 with v2 + 2v7—the most probable doorway state leading to IVR from v1 to the bath of all vibrational-rotational states with the close energies. In addition, it is shown that the observed dynamics is in agreement with a theoretical model assuming strong vibrational-rotational mixing.  相似文献   
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