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Chukwuemeka Okolie Yasmeen F. Belhseine Yimeng Lyu Dr. Matthew M. Yung Dr. Mark H. Engelhard Dr. Libor Kovarik Dr. Eli Stavitski Dr. Carsten Sievers 《Angewandte Chemie (International ed. in English)》2017,56(44):13876-13881
The conversion of methane into alcohols under moderate reaction conditions is a promising technology for converting stranded methane reserves into liquids that can be transported in pipelines and upgraded to value‐added chemicals. We demonstrate that a catalyst consisting of small nickel oxide clusters supported on ceria–zirconia (NiO/CZ) can convert methane to methanol and ethanol in a single, steady‐state process at 723 K using O2 as an abundantly available oxidant. The presence of steam is required to obtain alcohols rather than CO2 as the product of catalytic combustion. The unusual activity of this catalyst is attributed to the synergy between the small Lewis acidic NiO clusters and the redox‐active CZ support, which also stabilizes the small NiO clusters. 相似文献
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Elucidation and identification of amino acid containing membrane lipids using liquid chromatography/high‐resolution mass spectrometry
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136.
Omar R. Musaev Eli A. Sutter Jerzy M. Wrobel Michael B. Kruger 《Journal of nanoparticle research》2012,14(2):654-6
A eutectic AuGe target immersed in distilled water was ablated by pulsed ultraviolet laser light. The structure of the ablated
material was investigated by high-resolution transmission electron microscopy (HRTEM). The images show formation of nanowire
structures of AuGe up to 100 nm in length, with widths of 5–10 nm. These nanostructures have Ge content significantly lower
than the target material. Electron diffraction demonstrates that they crystallize in the α-AuGe structure. For comparison,
laser ablation of pure Au and pure Ge targets was also performed under the same conditions. HRTEM shows that Ge forms spherical
nanoparticles with a characteristic size of ~30 nm. Au forms spherical nanoparticles with diameters of ~10 nm. Similar to
AuGe, it also forms chainlike structures with substantially lower aspect ratio. 相似文献
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Ruckenstein E 《Journal of colloid and interface science》2002,246(2):393-400
The problem of coating a plate or a fiber through their withdrawal from a large reservoir was treated in the literature in various limiting cases. In the present paper, interpolation expressions are derived by scaling for Newtonian, Bingham, and viscoelastic fluids. The scaling analysis was also employed to explain the sharp increase in film thickness produced by inertia and the occurrence of a maximum thickness for an optimum velocity. It is also shown that, for a viscoelastic fluid, the film thickness tends to a finite value at very large withdrawal rates. An explanation is also provided for the existence of a maximum film thickness for an optimum surfactant concentration. 相似文献
140.
Clemens Berger 《Advances in Mathematics》2002,169(1):118-175