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121.
Theoretical studies on structure and performance of [1,2,5]‐oxadiazolo‐[3,4‐d]‐pyridazine‐based derivatives 下载免费PDF全文
Ke Wang Yuanjie Shu Ning Liu Weipeng Lai Tao Yu Xiaoyong Ding Zongkai Wu 《Journal of Physical Organic Chemistry》2017,30(1)
Based on energetic compound [1,2,5]‐oxadiazolo‐[3,4‐d]‐pyridazine, a series of functionalized derivatives were designed and first reported. Afterwards, the relationship between their structure and performance was systematically explored by density functional theory at B3LYP/6‐311 g (d, p) level. Results show that the bond dissociation energies of the weakest bond (N–O bond) vary from 157.530 to 189.411 kJ · mol?1. The bond dissociation energies of these compounds are superior to that of HMX (N–NO2, 154.905 kJ · mol?1). In addition, H1, H2, H4, I2, I3, C1, C2, and D1 possess high density (1.818–1.997 g · cm?3) and good detonation performance (detonation velocities, 8.29–9.46 km · s?1; detonation pressures, 30.87–42.12 GPa), which may be potential explosives compared with RDX (8.81 km · s?1, 34.47 GPa ) and HMX (9.19 km · s?1, 38.45 GPa). Finally, allowing for the explosive performance and molecular stability, three compounds may be suggested as good potential candidates for high‐energy density materials. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
122.
一种基于结构性改变的光子晶体光纤光栅理论研究 总被引:2,自引:0,他引:2
对一种新型基于结构性改变的光子晶体光纤光栅原理进行了研究.采用多极法分析了结构性改变对折射率的影响,得到有效折射率与包层气孔塌缩之间的关系,建立了结构性改变光子晶体光纤光栅模型.利用耦合模理论对所成光栅性能进行了分析,重点研究了包层空气孔层数、空气孔占空比、气孔塌缩程度对光栅谐振波长、带宽的影响.研究结果表明,光子晶体... 相似文献
123.
���� 《Frontiers of Physics》2011,6(1):109-123
Amorphous systems undergo the jamming transition when the density increases, temperature drops, or external shear stress decreases, as described by the jamming phase diagram which was proposed to unify different processes such as the glass transition, random close packing, and yielding under shear stress. At zero temperature and shear stress, the jamming transition occurs at a critical density at Point J. In this paper, we review recent studies of the material properties of marginally jammed solids and the glassy dynamics in the vicinity of Point J. As the only singular point in the jamming phase diagram, Point J exhibits special criticality in both mechanical and vibrational quantities. Dynamics approaching the glass transition in the vicinity of Point J show critical scalings, suggesting that the molecular glass transition and the colloidal glass transition are equivalent in the hard sphere limit. All these studies shed light on the long-standing puzzles of the glass transition and unusual properties of amorphous solids. 相似文献
124.
西藏羊八井位于东经90.53°, 北纬30.11°, 海拔4310m, 垂直地磁截止刚度14.1GV. 2005年1月20日羊八井太阳中子望远镜和中子监测器探测到与X7.1/2b太阳耀斑相关的GLE事件, 其中太阳中子望远镜能量>40MeV的能道在5min(07:00—07:05UT)和20min(07:00—07:20UT)的时间间隔内计数率增长的统计显著性分别是3.7σ和6.0σ, 同时羊八井中子监测器也探测到计数率的增长,初始时间为06:51—06:52UT. 观测表明在这次GLE事件中太阳质子可被加速到能量大于10GeV. 相似文献
125.
126.
A modified Woods-Saxon (MWS) potential is proposed for describing nucleus-nucleus interaction based on the Skyrme energy-density functional approach. Fusion barriers for a large number of fusion reactions from light to heavy systems can be described well with this potential. The suitable incident energies for fusion reactions leading to superheavy nuclei are also explored. It seems to us that the MWS potential is useful for selecting the suitable incident energies for fusion reactions for producing super-heavy nuclei. 相似文献
127.
Dependences of spin polarization on the control parameters in the spin-polarized injection through the magnetic p-n junction 下载免费PDF全文
Effective spin-polarized injection from magnetic semiconductor (MS)
to nonmagnetic semiconductor (NMS) has been highlighted in recent
years. In this paper we study theoretically the dependence of
nonequilibrium spin polarization (NESP) in NMS during spin-polarized
injection through the magnetic p-n junction. Based on the theory in
semiconductor physics, a model is established and the boundary
conditions are determined in the case of no external spin-polarized
injection and low bias. The control parameters that may influence the
NESP in NMS are indicated by calculating the distribution of spin
polarization. They are the doping concentrations, the equilibrium
spin polarization in MS and the bias. The effective spin-polarized
injection can be realized more easily by optimizing the above
parameters. 相似文献
128.
张文 李宁蒋玲 缪巍林镇辉 姚骑均史生才陈健 吴培亨S.I.Svechnikov Yu. B. Vachtomin S. V. Antipov B. M. voronov G. N. Gol'tsman 《中国物理快报》2007,24(6):1778-1781
A quasi-optical superconducting NbN hot-electron bolometer (HEB) mixer is measured in the frequency range of 0.5-2.5 THz for understanding of the frequency dependence of noise temperature of THz coherent detectors. It has been found that noise temperature increasing with frequency is mainly due to the coupling loss between the quasioptical planar antenna and the superconducting HEB bridge when taking account of non-uniform distribution of high-frequency current. With the coupling loss corrected, the superconducting HEB mixer demonstrates a noise temperature nearly independent of frequency. 相似文献
129.
Coronary magnetic resonance angiography (MRA) acquired using steady-state free precession (SSFP) sequences tends to suffer from image artifacts caused by local magnetic field inhomogeneities. Flow- and gradient-switching-induced eddy currents are important sources of such phase errors, especially under off-resonant conditions. In this study, we propose to reduce these image artifacts by using a linear centric-encoding (LCE) scheme in the phase-encoding (PE) direction. Abrupt change in gradients, including magnitude and polarity between consecutive radiofrequency cycles, is minimized using the LCE scheme. Results from numeric simulations and phantom studies demonstrated that signal oscillation can be markedly reduced using LCE as compared to conventional alternating centric-encoding (ACE) scheme. The image quality of coronary arteries was improved at both 1.5 and 3.0 T using LCE compared to those acquired using ACE PE scheme (1.5 T: ACE/LCE=2.2+/-0.8/3.0+/-0.6, P=.02; 3.0 T: ACE/LCE=2.1+/-1.1/3.0+/-0.8, P=.01). In conclusion, flow- and eddy-currents-induced imaging artifacts in coronary MRA using SSFP sequence can be markedly reduced with LCE acquisition of PE lines. 相似文献
130.
研究用于GaN基大功率倒装焊(Flip-chip)紫光LED(UV-LED)的高反射率p型欧姆接触的电学和光学性能。用磁控溅射的方法在GaN基LED外延片表面沉积了不同厚度Ag,Al,Au和Pd四种金属,测量了样品的反射率和透射率。结合同步辐射高强度X射线衍射和AFM对金属薄膜的晶体结构进行分析,并对表面形貌进行了观测,对由金属薄膜构成的多层膜结构及其对光反射率的作用机理进行了研究。测量结果表明,在入射光波长为400nm时,Ni/Au/Ag和Ni/Au/Al电极的反射率比Ni/Au的反射率提高了三倍。同时与p-GaN有良好的欧姆接触特性。 相似文献