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51.
An isolated-core-excitation (ICE) scheme and stepwise
excitation are employed to study the highly excited states of the
europium atom. The bound europium spectrum with odd parity in a
region of 42400--43500~cm^{ - 1} is measured, from which
spectral information on 38 transitions, such as level position
and relative intensity, can be deduced. Combined with information
about excitation calibration and the error estimation process, the
selection rules enable us to determine the possible values of total
angular momentum J for the observed states. The autoionization
spectra of atomic europium, belonging to the 4f^{7}6p{nl}
(l=0, 2) configurations, are systematically investigated by using
the three-step laser resonance ionization spectroscopy (RIS)
approach. With the ICE scheme, all the experimental spectra of the
autoionizing states have nearly symmetric profiles whose peak
positions and widths can be easily obtained. A comparison between
our results and those from the relevant literature shows that our
work not only confirms many reported states, but also discovers 14
bound states and 16 autoionizing states. 相似文献
52.
Two-colour stepwise excitation and photoionization schemes are adopted to study the spectra of high-lying states of the Sm atom. These bound even-parity states are excited with three different excitation paths from the 4f66s6p7DJ (J = 1, 2, 3) intermediate states, respectively. They are probed by photoionization process with an extra photon driving them to the continuum states. In this experiment, 270 states are detected in an energy range from 36160 cm-1 to 42250 cm-1, 109 of which are newly discovered, while the rest of them are confirmed to be the energy levels reported previously. Furthermore, based on the J-momentum selection rules of three excitation paths, a unique assignment of J-momentum for all observed states is determined, eliminating all remaining ambiguities in the literature. Finally, 53 single-colour transitions originating from the scanning laser are also identified. For all the relevant transitions, the information about their relative intensities is also given in the paper. 相似文献
53.
戴长建 《原子与分子物理学报》1999,16(4):587-591
采有耦合和非耦合表象,描述了超短脉冲激光与钾原子的相互作用。分析了进一步 激发光电离的过程,导出了跃迁终态随激光偏振组合的密切关键。 相似文献
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56.
利用拉曼光谱技术分别研究了植物油和动物脂肪油的光谱特性。通过自适应迭代惩罚最小二乘法的基线校正方法, 对所测得的拉曼光谱进行了数据处理,获得了它们的微观信息。进而通过选取其中部分油的拉曼光谱,进行了植物油的光谱、动物脂肪油的光谱以及动物脂肪油和植物油之间的光谱比较和分析,从而发现了多种植物油光谱(包括多个频移范围内的频移大小以及强度大小)的差异,也发现了动物脂肪油与植物油的拉曼光谱间的差异。不但提供了辨识不同食用油的光谱依据,也证明了拉曼光谱是一种识别不同油品的有效方法。 相似文献
57.
Branching ratio and angular distribution of ejected electrons from Eu 4f~76p_(1/2)nd auto-ionizing states
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The branching ratios of ions and the angular distributions of electrons ejected from the Eu 4f~76p_(1/2)nd auto-ionizing states are investigated with the velocity-map-imaging technique.To populate the above auto-ionizing states,the relevant bound Rydberg states have to be detected first.Two new bound Rydberg states are identified in the region between41150 cm~(-1)and 44580 cm~(-1),from which auto-ionization spectra of the Eu 4f~76p_(1/2)nd states are observed with isolated core excitation method.With all preparations above,the branching ratios from the above auto-ionizing states to different final ionic states and the angular distributions of electrons ejected from these processes are measured systematically.Energy dependence of branching ratios and anisotropy parameters within the auto-ionization spectra are carefully analyzed,followed by a qualitative interpretation. 相似文献
58.
建立了一种理论模型和实验方法, 可以有效地修正来自于环境和介质对测温结果的影响。这种修正方法通过计入测温环境对辐射体的衰减系数,可以显著改善以灰体辐射为基础的测温技术的精度和普适性。首先,利用多通道CCD图像光谱仪快速准确地获得给定辐射体在空气中的指纹光谱,并将其等效为一个标准的灰体模型;其次,将该辐射体放入未知的环境和介质中,重复测量该辐射体的辐射光谱,并建立包含待测介质对辐射体的衰减特征的灰体模型。最后,通过对比上述两种情况下的灰体模型,便可精确确定该辐射体在该环境和介质下的温度。通过对处于不同环境和介质下的相同辐射体的系统实验,检验了该测温技术和修正方法的普适性和准确性。 相似文献
59.
Two-step excitation and ionization processes are used to detect Sm atoms in many excited states populated with tunable lasers. The wavelength of the first laser is tuned to the resonances from the Sm 4f^6 6s^2 ^7FJ (J=0 6) states to many odd-parity states with different electronic configurations, where the atoms are detected by photoionization process using an ultraviolet laser with a wavelength of 355 nm. Precise measurements on the energy level and intensity for many Sm 4f^6 6s6p and 4f^5 5d6s^2 states have been carried out. In a theoretical analysis on the spectral data, such as peak position, relative intensity, many transitions can be identified as the resonances from the Sm 4f^6 6s^2 7FJ (J=0-6) states to the atomic states with 4f^6 6s6p and 4f^5 5d6s^2 electronic configurations. This work also reports many spectral data on the odd-parity states that cannot be found in the literature. 相似文献
60.
采用双色三步激发和光电离过程,对Sm原子的偶宇称高激发态的光谱进行了研究.先采用两条激发路线分别将Sm原子两步共振激发至待测的高激发态,然后利用光电离技术对其进行探测.分别将第一束激光的波长固定在627.50nm和624.41nm上,以便将Sm原子从亚稳态共振激发到由4f66s6p电子组态所构成的两个原子状态上.第二束激光在440-700nm的波段范围内扫描,不仅使Sm原子在30040-38065cm-1能域内的偶宇称高激发态上布居,将其进一步光电离,测量了其光谱.通过光谱定标和选择定则等分析手段,本工作不仅精确获得了136个态的能级位置,而且也唯一确定了其总角动量,并且给出了相关跃迁的相对谱线强度. 相似文献