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151.
Olga Ordeig Craig E Banks Trevor J Davies F Javier del Campo Francesc Xavier Mu?oz Richard G Compton 《Analytical sciences》2006,22(5):679-683
Gold ultra-microelectrode arrays are used to explore the electrochemical oxidation of hydroxide ions and are shown to be analytical useful. Two types of ultra-microelectrode arrays are used; the first consist of 256 individual electrodes of 5 microm in radius, 170 of which are electrochemically active in a cubic arrangement which are separated from their nearest neighbour by a distance of 100 microm. The second array compromises 2597 electrodes of 2.5 microm in radius and of which 1550 of which are electrochemically active in a hexagonal arrangement separated by the nearest neighbour by 55 microm. Well defined voltammetric waves are found with peak currents proportional to the concentration of hydroxide ions in the range 50 microM to 1 mM. Detection limits of 20 microM using the 170 ultra-microelectrode and 10 microM with the 1550 ultra-microelectrode array are shown to be possible but with a higher sensitivity of 4 mA M(-1) observed using the 1550 ultra-microelectrode array compared to 1.2 mA M(-1) with the 170 ultra-microelectrode array. 相似文献
152.
Ivan Gutman Sabina Gojak Niko Radulovi? Boris Furtula 《Monatshefte für Chemie / Chemical Monthly》2006,46(2):277-284
In a recent work it was demonstrated that in linear hexagonal chains the distribution of π-electrons into rings (as computed
by means of the Randić–Balaban method) is uniform, irrespective of the nature of the terminal fragments. We now establish that an analogous, yet somewhat
more complex, uniformity in the π-electron distribution exists also in double linear hexagonal chains, as well as in some
other benzenoid systems. 相似文献
153.
J.-S. Kang G. Kim S.S. Lee S. Choi S. Cho S.W. Han H.J. Shin B.I. Min 《Journal of magnetism and magnetic materials》2006
The spatial concentration distribution and local electronic structure of ferromagnetic Ge1−xTx (T=Cr, Mn, Fe) DMS single crystals have been investigated by using scanning photoelectron microscopy (SPEM), X-ray absorption spectroscopy (XAS), and photoemission spectroscopy (PES). It is found that doped T ions in Ge1−xTx crystals are chemically phase-separated, suggesting that the observed ferromagnetism arises from the phase-separated T-rich phases in Ge1−xTx. 相似文献
154.
155.
Chang-Wan Kim 《Archiv der Mathematik》2007,88(4):378-384
We showed that any compact locally symmetric Finsler metric with positive flag curvature must be Riemannian.
Dedicated to Professor Karsten Grove on the occassion of his sixtieth birthday
Received: 8 May 2006 相似文献
156.
The energy level alignment between C60 and Al has been investigated by using ultraviolet photoelectron spectroscopy. To obtain the interfacial electronic structure between C60 and Al, C60 was deposited on a clean Al substrate in a stepwise manner. The valence-band spectra were measured immediately after each step of C60 deposition without breaking the vacuum. The measured onset of the highest occupied molecular orbital energy level was located at 1.59 eV from the Fermi level of Al. The vacuum level was shifted 0.68 eV toward lower binding energy with additional C60 layers. The observed vacuum level shift means that the interface dipole exists at the interface between C60 and Al. The barrier height of electron injection from Al to C60 is 0.11 eV, which is smaller value than that of hole injection. 相似文献
157.
Moments of claims in a Markovian environment 总被引:1,自引:1,他引:0
This paper considers discounted aggregate claims when the claim rates and sizes fluctuate according to the state of the risk business. We provide a system of differential equations for the Laplace–Stieltjes transform of the distribution of discounted aggregate claims under this assumption. Using the differential equations, we present the first two moments of discounted aggregate claims in a Markovian environment. We also derive simple expressions for the moments of discounted aggregate claims when the Markovian environment has two states. Numerical examples are illustrated when the claim sizes are specified. 相似文献
158.
I. S. Kim N. L. Krussanova I. V. Alekseeva R. N. Smartt 《Radiophysics and Quantum Electronics》1998,41(2):94-98
A new approach to investigating the statistical relationship between certain solar features and recurrent wind streams is
presented. This approach is based, on a comparative analysis of the distributions of lifetimes of a set of solar features,
recurrent geomagnetic disturbances, and geomagnetic “calms.” Correlation coefficients of 0.81, 0.85, 0.79, and 0.77 are found
for the distributions of several solar features—filaments, large-scale magnetic fields, coronal features, and coronal holes,
respectively—and recurrent geomagnetic disturbances. A correlation factor of 0.97 between the distributions of geomagnetic
“calms” and active regions is found. The combined evidence indicates that no specific type of solar feature is responsible
for the recurrent stream activity. Rather, the configuration of the large-scale magnetic field of the Sun appears to control
the permanently existing corpuscular activity. Since prominences trace polarity division lines of the large-scale magnetic
field structure of the Sun, they have been checked as a possible general predictor of recurrent corpuscular activity; their
parameters could present the most reliable indices that relate closely with trends in geomagnetic disturbances. A comparative
analysis of cyclic variations of sunspot numbers, the total number of prominences, the relative number of low-height (<-20″)
prominences, and recurrent geomagnetic storms is made for solar cycle N16. The relative number of low-height prominences is
found to correlate broadly (0.83) with recurrent wind streams.
P. K. Shternberg State Astronomical Institute, Moscow, Russia; National Solar Observatory, Sacramento Peak, U.S. Published
in Izvestiya Vysshikh Uchebnykh Zavedenii, Radiofizika, Vol. 41, No. 2, pp. 145–151, February, 1998. 相似文献
159.
160.