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21.
本文考虑由抛物型BMO函数和沿抛物线γ(t)=(t,t2)的Hilbert变换生成的交换子.通过局部化方法, Fourier变换估计和bootstrap讨论,得到了所考虑的交换子的Lp(1相似文献   
22.
Two types of quinoline scaffolds were constructed in a combinatorial format via the Ugi four-component reaction (U-4CR) and Pd-catalyzed intramolecular arylation reaction. The scope of this two-step synthetic sequence was examined from commercially available and synthetically accessible starting materials.  相似文献   
23.
Weijun Chen  Huajun Yang  Zhibo Li  Jin Li  Bin Zhu 《Optik》2010,121(24):2259-2261
On the basis of the electromagnetic field mode matching theory, the coupling efficiency ratio from spatial light to Bragg fiber is analyzed, which shows that the coupling efficiency ratio is related to the radius of focused facular, the core radius of Bragg fiber and wave number of the core. By optimizing the value of such parameters appropriately, the Bragg fiber coupling efficiency ratio can be improved. It is also important for the analysis of the coupling efficiency of Bragg fiber, which can be applied to the free optical communication system and laser radar system.  相似文献   
24.
In this paper, we first discuss some properties of the neutral operator with multiple variable coefficients $(Ax)(t):=x(t)-\sum\limits_{i=1}^{n}c_i(t)x(t-\delta_i)$. Afterwards, by using an extension of Mawhin''s continuation theorem, a kind of second order $p$-Laplacian neutral differential equation with multiple variable coefficients as follows $$\left(\phi_p\left(x(t)-\sum\limits_{i=1}^{n}c_i(t)x(t-\delta_i)\right)''\right)''=\tilde{f}(t,x(t),x''(t))$$ is studied. Finally, we consider the existence of periodic solutions for two kinds of second-order $p$-Laplacian neutral Rayleigh equations with singularity and without singularity. Some new results on the existence of periodic solutions are obtained. It is worth noting that $c_i$ ($i=1,\cdots,n$) are no longer constants which are different from the corresponding ones of past work.  相似文献   
25.
Sufficient conditions are presented for theexistence and stability of periodic solutions for a high-order differential system.Besides, an example is given to illustrate the result.  相似文献   
26.
Using Green's function for third‐order differential equation and some fixed‐point theorems, i.e., Leray‐Schauder alternative principle and Schauder's fixed point theorem, we establish three new existence results of periodic solutions for nonlinear third‐order singular differential equation, which extend and improve significantly existing results in the literature.  相似文献   
27.
A highly efficient bifunctional metal‐free catalyst was prepared by growth of three‐dimensional porous fluorographdiyne networks on carbon cloth (p‐FGDY/CC). Our experiments and density functional theory (DFT) calculations show the 3D p‐FGDY/CC network is highly active and it is a high potential metal‐free catalyst for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER), as well as overall water splitting (OWS) under both acidic and alkaline conditions. The experimental and theoretical results show very good consistency; for example, in the HER process, p‐FGDY/CC exhibits small overpotentials of 82 and 92 mV to achieve 10 mA cm?2 under alkaline and acidic conditions, respectively. This ensures an even higher selectivity for the adsorption/desorption of various O/H intermediate species. The essential key promotion accomplishes a bifunctional H2O redox performance application under pH‐universal electrochemical conditions.  相似文献   
28.
Organotrifluoroborates solvolyze in water at rates that vary over five orders of magnitude. The negative logarithm of the solvolytic rate constant, pk(B?F), correlates exceptionally well with the pKa of the analogous carboxylic acid (R2=0.984). This unforeseen correlation may be of predictive value for several applications including Suzuki–Miyaura cross‐coupling reactions and the design of 18F‐organotrifluoroborate radioprosthetic groups.  相似文献   
29.
Fragmentation of protonated RVYIHPF and RVYIHPF-OMe and the corresponding radical cations was studied using time- and collision energy-resolved surface-induced dissociation (SID) in a Fourier transform ion cyclotron resonance mass spectrometer (FT-ICR MS) specially equipped to perform SID experiments. Peptide radical cations were produced by gas-phase fragmentation of Co (III)(salen)-peptide complexes. Both the energetics and the mechanisms of dissociation of even-electron and odd-electron angiotensin III ions are quite different. Protonated molecules are much more stable toward fragmentation than the corresponding radical cations. RRKM modeling of the experimental data suggests that this stability is largely attributed to differences in threshold energies for dissociation, while activation entropies are very similar. Detailed analysis of the experimental data obtained for radical cations demonstrated the presence of two distinct structures separated by a high free-energy barrier. The two families of structures were ascribed to the canonical and zwitterionic forms of the radical cations produced in our experiments.  相似文献   
30.
Abdominal wall defect caused by surgical trauma, congenital rupture, or tumor resection may result in hernia formation or even death. Tension-free abdominal wall defect repair by using patches is the gold standard to solve such problems. However, adhesions following patch implantation remain one of the most challenging issues in surgical practice. The development of new kinds of barriers is key to addressing peritoneal adhesions and repairing abdominal wall defects. It is already well recognized that ideal barrier materials need to have good resistance to nonspecific protein adsorption, cell adhesion, and bacterial colonization for preventing the initial development of adhesion. Herein, electrospun poly(4-hydroxybutyrate) (P4HB) membranes infused with perfluorocarbon oil are used as physical barriers. The oil-infused P4HB membranes can greatly prevent protein attachment and reduce blood cell adhesion in vitro. It is further shown that the perfluorocarbon oil-infused P4HB membranes can reduce bacterial colonization. The in vivo study reveals that perfluoro(decahydronaphthalene)-infused P4HB membranes can significantly prevent peritoneal adhesions in the classic abdominal wall defects’ model and accelerate defect repair, as evidenced by gross examination and histological evaluation. This work provides a safe fluorinated lubricant-impregnated P4HB physical barrier to inhibit the formation of postoperative peritoneal adhesions and efficiently repair soft-tissue defects.  相似文献   
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