Two photon-induced fluorescence intensity and anisotropy decays of diphenylhexatriene in solvents and lipid bilayers

We measured the fluorescence intensity and anisotropy decays of 1,6-diphenyl-1,3,5-hexatriene (DPH)-labeled membranes resulting from simultaneous two-photon excitation of fluorescence. Comparison of these two-photon data with the more usual one-photon measurements revealed that DPH displayed identical intensity decays, anisotropy decays, and order parameters for one- and two-photon excitation. While the anisotropy data are numerically distinct, they can be compared by use of the factor 10/7, which accounts for the two-photon versus one-photon photoselection. The increased time 0 anisotropy of DPH can result in increased resolution of complex anisotropy decays. Global analysis of the one- and two-photon data reveals consistency with a single apparent angle between the absorption and the emission oscillators. The global anisotropy analysis also suggests that, except for the photoselection factor, the anisotropy decays are the same for one-and two-photon excitation. This ideal behavior of DPH as a two-photon absorber, and its high two-photon cross section, makes DPH a potential probe for confocal two-photon microscopy and other systems where it is advantageous to use long-wavelength (680- to 760-nm) excitation.     

Phenomenological nuclear-reaction description in deuterium-saturated palladium and synthesized structure in dense deuterium gas under γ-quanta irradiation

The observed phenomena of changes of chemical compositions in previous reports [1, 2] allowed us to develop a phenomenological nuclear fusion-fission model with taking into consideration the elastic and inelastic scattering of photoprotons and photoneutrons, heating of surrounding deuterium nuclei, following d-d fusion reactions and fission of middle-mass nuclei by “hot” protons, deuterons and various-energy neutrons. Such chain processes could produce the necessary number of neutrons, “hot” deuterons for explanation of observed experimental results [1, 2]. The developed approach can be a basis for creation of deuterated nuclear fission reactors (DNFR) with high-density deuterium gas and the so-called deuterated metals. Also, this approach can be used for the study of nuclear reactions in high-density deuterium or tritium gas and deuterated metals.     

Molecular transient effects in K-band spectroscopy

The time dependence of microwave transient absorption and emission was measured forJ=2←1 of the OCS molecule under on- and off-resonant conditions by the technique of Stark switching. The results are analyzed with the theory of a coherent electromagnetic wave interacting with a two-level quantum system through the electric dipole interaction to obtain the pressure dependence of the relaxation timesT ₂ and in consequence the pressure broadening parameterC _w=26.7±0.9 (μs·mTorr)^?1 has been obtained.     

Detailed infrared spectroscopic study of thermal transitions in new hybrid [(CH3)2CHNH3]4Cd3Cl10 crystal

Phase transitions of tetra(isopropylammonium)decachlorotricadmate(II) [(CH₃)₂CHNH₃]₄Cd₃Cl₁₀ crystal have been studied by infrared, far infrared and Raman measurements in wide temperature range, between 11 K and 388 K. The temperature changes of wavenumber, center of gravity, width and intensity of the bands were analyzed to clarify cationic and anionic contributions to the phase transitions mechanism. The results of investigation showed earlier by differential scanning calorimetry (DSC), thermal expansion and dielectric measurements clearly confirmed the sequence of phase transitions at T₁=353 K, T₂=294 K and T₃=260 K. The current results derived from DSC and infrared measurements revealed additional phase transition at T₄=120 K.     

Thickness dependence of the magnetic anisotropy of Fe layers separated by Al

Magnetic multilayers of ⁵⁷Fe with nominal thickness, T _nom, between 0.4 and 1.0 nm separated by 3.0 nm Al spacer layers were prepared by alternate deposition of the constituents in high vacuum. The samples were investigated at 4.2 K in external magnetic field. A fraction of Fe atoms corresponding to about 0.3 nm equivalent Fe-thickness was found to mix into the Al spacer. The extremely strong magnetic anisotropy observed for T _nom < 0.8 nm is attributed to Fe layers of approximately two atomic planes thick. The anisotropy decreases considerably after the building up of the third Fe atomic layer starts at T _nom = 0.8 nm, but full saturation was not achieved even for T _nom = 1 nm and 3 T magnetic field applied perpendicularly to the sample plane.     

Antenna length and polarization response of antenna-coupled MOM diode infrared detectors

This work focuses on the fabrication and response of dipole antenna-coupled metal–oxide–metal diode detectors to long-wave infrared radiation. The detectors are fabricated using a single electron beam lithography step and a shadow evaporation technique. The detector’s characteristics are presented, which include response as a function of incident infrared power and polarization angle. In addition, the effect of dipole antenna length on detection characteristics for 10.6 μm radiation has been measured to determine resonant lengths. The response of the detector shows a first resonance at a dipole length of 3.1 μm, a second resonance at 9.3 μm, and third at 15.5 μm. The zeros intermediate to the resonances are also evident.     

Nuclear stopping from 0.09A to 1.93A GeV and its correlation to flow

We present a complete systematics (excitation functions and system-size dependences) of global stopping and side flow for heavy ion reactions in the energy range between 0.09A and 1.93A GeV. For the heaviest system, Au+Au, we observe a plateau of maximal stopping extending from about 0.2A to 0.8A GeV with a fast drop on both sides. The degree of stopping, which is shown to remain significantly below the expectations of a full stopping scenario, is found to be highly correlated to the amount of side flow.     

Electron-electron interaction in strong electromagnetic fields: the two-electron contribution to the ground-state energy in He-like uranium

Radiative recombination transitions into the ground state of cooled bare and hydrogenlike uranium ions were measured at the storage ring ESR. By comparing the corresponding x-ray centroid energies, this technique allows for a direct measurement of the electron-electron contribution to the ionization potential in the heaviest He-like ions. For the two-electron contribution to the ionization potential of He-like uranium we obtain a value of 2248+/-9 eV. This represents the most accurate determination of two-electron effects in the domain of high-Z He-like ions, and the accuracy reaches already the size of the specific two-electron radiative QED corrections.     

A model for FL and R = FL/FT at low x and low Q2

A model for the longitudinal structure function F_L at low x and low Q² is presented, which includes the kinematical constraint F_L ～ Q⁴ as Q² → 0. It is based on the photon-gluon fusion mechanism suitably extrapolated to the region of low Q². The contribution of quarks having limited transverse momentum is treated phenomenologically assuming that it is described by the soft pomeron exchange mechanism. The ratio R = F_L/(F₂ ? F_L), with the F₂ appropriately extrapolated to the region of low Q², is also discussed.