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121.
Let k and m are positive integers with k ≥ m. The probability generating function of the waiting time for the first occurrence of consecutive k successes in a sequence of m-th order Markov dependent trials is given as a function of the conditional probability generating functions of the waiting
time for the first occurrence of consecutive m successes. This provides an efficient algorithm for obtaining the probability generating function when k is large. In particular, in the case of independent trials a simple relationship between the geometric distribution of order
k and the geometric distribution of order k−1 is obtained.
This research was partially supported by the ISM Cooperative Research Program(2004-ISM-CRP-2006) and by a Grant-in-Aid for
Scientific Research (C) of the JSPI (Grant Number 16500183) 相似文献
122.
Wataru Yoshida Aki Kezuka Yoshiyuki Murakami Jinhee Lee Koichi Abe Hiroaki Motoki Takafumi Matsuo Nobuaki Shimura Mamoru Noda Shizunobu Igimi Kazunori Ikebukuro 《Analytica chimica acta》2013
An automatic polymerase chain reaction (PCR) product detection system for food safety monitoring using zinc finger (ZF) protein fused to luciferase was developed. ZF protein fused to luciferase specifically binds to target double stranded DNA sequence and has luciferase enzymatic activity. Therefore, PCR products that comprise ZF protein recognition sequence can be detected by measuring the luciferase activity of the fusion protein. We previously reported that PCR products from Legionella pneumophila and Escherichia coli (E. coli) O157 genomic DNA were detected by Zif268, a natural ZF protein, fused to luciferase. In this study, Zif268–luciferase was applied to detect the presence of Salmonella and coliforms. Moreover, an artificial zinc finger protein (B2) fused to luciferase was constructed for a Norovirus detection system. In the luciferase activity detection assay, several bound/free separation process is required. Therefore, an analyzer that automatically performed the bound/free separation process was developed to detect PCR products using the ZF–luciferase fusion protein. By means of the automatic analyzer with ZF–luciferase fusion protein, target pathogenic genomes were specifically detected in the presence of other pathogenic genomes. Moreover, we succeeded in the detection of 10 copies of E. coli BL21 without extraction of genomic DNA by the automatic analyzer and E. coli was detected with a logarithmic dependency in the range of 1.0 × 10 to 1.0 × 106 copies. 相似文献
123.
Aki Pulkkinen Katariina Pussi 《The European Physical Journal B - Condensed Matter and Complex Systems》2017,90(10):184
We study atomic oxygen adsorption on a Pb(1 0 0) surface using density functional theory. The structures, binding energies, work function, and charge transfer of on-surface and subsurface adsorption are investigated at a range of coverages from 0.06 to 1.00 ML. The energetically favored adsorption site for on-surface adsorption is found to be a distorted hollow site for the whole coverage range studied. The distorted structures are stabilized by mixing of 6s and 6p states of lead mediated by the 2p states of oxygen. For subsurface adsorption, the sub-bridge site is found to be preferred to the sub-hollow site at low coverages, the two being nearly equal in energy at monolayer coverage. At 0.11 ML coverage, diffusion from an on-surface hollow site to a sub-bridge site is found to be barrierless, suggesting facile subsurface oxidation at low coverages. Combined on-surface and subsurface adsorption leads to the formation of a two-layer oxide structure resembling β-PbO. 相似文献
124.
125.
Yoshio Imai Kazuo Itoya Masami Kanamaru Masa‐Aki Kakimoto 《Journal of polymer science. Part A, Polymer chemistry》2002,40(11):1790-1795
New phenolic hydroxyl‐pendant aromatic polyimides were synthesized with the N‐silylated diamine method in two steps: the ring‐opening polyaddition of tetrakis(trimethylsilyl)‐substituted 4,4′‐diamino‐3,3′‐dihydroxybiphenyl to various aromatic tetracarboxylic dianhydrides, giving trimethylsiloxy‐pendant poly(amic acid) trimethylsilyl esters, and thermal imidization. The hydroxyl‐bearing polyimides were amorphous but insoluble in organic solvents. They had glass‐transition temperatures greater than 370 °C and temperatures of 10% weight loss greater than 415 °C in nitrogen. The hydroxyl‐pendant polypyromellitimide film had a high tensile strength and a high modulus of 310 MPa and 10 GPa, respectively. © 2002 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 40: 1790–1795, 2002 相似文献
126.
在线性压电陶瓷本构关系和裂纹边界绝缘的框架下,用超奇异积分方程的方法对椭圆类片状裂纹问题进行了重新研究.超奇异积分方程中的未知位移间断和电势间断近似地表示为基本密度函数与多项式之积,其中基本密度函数反映了椭圆片状裂纹前沿电弹性场的奇异性,而多项式在均布载荷作用下可用一个常数来表达.引入椭球坐标系后,得到了均布载荷作用下未知位移间断和电势间断的解析解.使用这些解析解和电弹性场强度的定义,得到了裂纹前沿Ⅰ型、Ⅱ型和Ⅲ型应力强度因子以及电位移强度因子的精确表达式.法向均布载荷作用下的结果与现有精确解完全一致,切向均布载荷作用下的结果则尚未见有其它报道. 相似文献
127.
128.
Tanaka T Inui H Kida H Kodama T Okamoto T Takeshima A Tachi Y Morimoto Y 《Chemical communications (Cambridge, England)》2011,47(10):2949-2951
The characteristic indeno-tetrahydropyridine core of cytotoxic haouamine B (2) was efficiently synthesized featuring the diastereoselective construction of a diaryl-substituted stereogenic quaternary center by an intramolecular Pd-catalyzed α-C-arylation and subsequent direct conversion of the vinylogous imide function into the C2-C25 double bond by TsNHNH(2). 相似文献
129.
Shingo Kimura Satoshi Kobayashi Takuya Kumamoto Aki Akagi Naomi Sato Tsutomu Ishikawa 《Helvetica chimica acta》2011,94(4):578-591
Towards total synthesis of a series of kinamycin and related antibiotics via common synthetic intermediates, total synthesis of prekinamycin was achieved via Suzuki coupling of naphthaleneboronic acid and bromobenzene derivative, intramolecular Friedel? Crafts reaction of 2‐(naphthalen‐2‐yl)benzoic acid, and diazotization in ten steps from 3,5‐dimethylphenol. Synthetic studies towards kinamycin antibiotics was also examined, and the tetracyclic quinone core for kinamycins was synthesized. Palladium‐catalyzed site‐selective hydroxylation of a benzoic acid derivative with the AB‐D ring part was successfully applied to the selective D‐ring functionalizations. 相似文献
130.
P. Surya Mohan Tanja Tarvainen Martin Schweiger Aki Pulkkinen Simon R. Arridge 《Journal of computational physics》2011,230(19):7364-7383
We propose the PN approximation based on a finite element framework for solving the radiative transport equation with optical tomography as the primary application area. The key idea is to employ a variable order spherical harmonic expansion for angular discretization based on the proximity to the source and the local scattering coefficient. The proposed scheme is shown to be computationally efficient compared to employing homogeneously high orders of expansion everywhere in the domain. In addition the numerical method is shown to accurately describe the void regions encountered in the forward modeling of real-life specimens such as infant brains. The accuracy of the method is demonstrated over three model problems where the PN approximation is compared against Monte Carlo simulations and other state-of-the-art methods. 相似文献