两纠缠原子与光场相互作用系统原子的纠缠特性

研究了两纠缠原子与单模相干态光场相互作用系统中原子纠缠度的时间演化特性,运用全量子理论和数值计算的方法,应用Concurrence纠缠度量标准,讨论了原子初始时刻的纠缠状态和光场强度对两原子纠缠度的影响.结果表明：双原子系统初始纠缠度越大,两原子间的纠缠在演化过程中的峰值也越大;随着光场强度的增加,两原子纠缠度的振荡曲线逐渐表现出崩塌-回复现象,周期性也越来越明显.     

利用一个三粒子W态隐形传送N粒子GHZ态

杨洪钦等提出一个用两个三粒子W态作为量子信道将N粒子GHZ态从发送者传送给两个接收者中任意一个的量子隐形传送方案. 给出其理论分析,并提出了一个仅用一个三粒子W态作为量子信道将N粒子GHZ态传送给两个接收者之一的量子隐形传送的方案. 关键词： 隐形传态 GHZ态 W态量子信道     

An organoantimony nitrate complex with azastibocine framework as water tolerant Lewis acid catalyst for the synthesis of 1,2-disubstitued benzimidazoles

A novel organoantimony complex of 6-cyclohexyl-6,7-dihydrodibenzo[c,f] [1,5]azastibocin-12(5H)-yl nitrate ( 2 ) was synthesized and systematically characterized by techniques such as NMR spectra, TG-DSC, and X-ray diffraction. It was found that the complex 2 exhibits relatively strong Lewis acidity (3.3 < Ho ≤ 4.8) and could be employed as a water tolerant Lewis acid catalyst for the synthesis of synthetically valuable benzimidazole derivatives starting from aldehydes and arylenediamines. This catalytic system shows excellent tolerance toward a wide variety of functional groups, such as methyl, methoxyl, fluoro, chloro, bromo, nitro, cyan, trifluoromethyl, 1-naphthaldehyde, furfural and n-butyl, together with facile reusability in 5 times scale enlarged synthesis.     

Enhancement of Mass and Charge Transfer during Carbon Dioxide Photoreduction by Enhanced Surface Hydrophobicity without a Barrier Layer

The CO₂ reduction reaction (CRR) represents a promising route for the clean utilization of renewable resources. But mass-transfer limitations seriously hinder the forward step. Enhancing the surface hydrophobicity by using polymers has been proved to be one of the most efficient strategies. However, as macromolecular organics, polymers on the surface hinder the transfer of charge carriers from catalysts to reactants. Herein, we describe an in-situ surface fluorination strategy to enhance the surface hydrophobicity of TiO₂ without a barrier layer of organics, thus facilitating the mass transfer of CO₂ to catalysts and charge transfer. With less obstruction to charge transfer, a higher CO_2, and lower H⁺ surface concentration, the photocatalytic CRR generation rate of methanol (CH₃OH) is greatly enhanced to up to 247.15 μmol g⁻¹ h⁻¹. Furthermore, we investigated the overall defects; enhancing the surface hydrophobicity of catalysts provides a general and reliable method to improve the competitiveness of CRR.     

有机化学实验线上课程之扬长避短教学设计与实践篇

It has been two months since a boom of online education triggered by the epidemic in China. At present, we are keeping focus on how to optimize our online class. In the case of chemistry laboratory courses, there's not much that can be done to experimental operations through online teaching. While for the traditional teaching procedure, there is still room for improvement in terms of integrating research to teaching, interactivity, etc. This paper will present some design strategies for improving teaching the organic chemistry laboratory online. To be specific, it describes how teaching materials like the lesson plan and virtual lab were coordinated into the online teaching. And we will also discuss the holistic approach to a better outcome for students' active learning and integration research into teaching by redesigning multiple phases, such as the pre-laboratory preparation, live online class, experimental operations.     

The effects of adjusting pulse anodization parameters on the surface morphology and properties of a WO3 photoanode for photoelectrochemical water splitting

Journal of Solid State Electrochemistry - An ordered porous nanostructure provides a large reaction interface with an unusually high number of active sites, meaning that such a nanostructure is...     

Generalizations of Non-Commutative Neutrix Convolution Products of Functions

The non-commutative neutrix convolution product of the functions x ^r cos_–(x) and x ^s cos₊(x) is evaluated. Further similar non-commutative neutrix convolution products are evaluated and deduced.