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31.
32.
E. Wendehorst E. Knoche S. S. Nametkin E. A. Robinson M. J. Herbrich G. Egloff J. C. Morrell P. Truesdell O. C. Bridgeman J. C. Molitor T. H. Rogers V. Voorhees H. O. Ervin E. R. Gillis C. C. Minter und A. Dongescu 《Fresenius' Journal of Analytical Chemistry》1935,102(7-8):308-312
Ohne Zusammenfassung 相似文献
33.
Formation energies for Ge/Si(100) pyramidal islands are computed combining continuum calculations of strain energy with first-principles-computed strain-dependent surface energies. The strain dependence of surface energy is critically impacted by the presence of strain-induced changes in the Ge {100} surface reconstruction. The appreciable strain dependencies of rebonded-step {105} and dimer-vacancy-line-reconstructed {100} surface energies are estimated to give rise to a significant reduction in the surface contribution to island formation energies. 相似文献
34.
A single-component strained film is known to be unstable to the stress-driven morphological instability. Here, we determine how the instability is modified in an alloy film by considering the effect of compositional stresses due to an atomic size difference. We find that the coupling of composition to stress always makes the film more unstable to the formation of stress-driven surface undulations. The destabilization is greatest over a range of intermediate deposition rates. 相似文献
35.
36.
Burton Voorhees 《Journal of statistical physics》1992,66(5-6):1397-1414
One-dimensional nearest neighbor cellular automata defined over Z2 are characterized in terms of a set of eight nonadditive basis operators which act on the automaton state space. Every evolution rule for such automata can be expressed as an operator which is a direct sum of the basis operators. This approach allows decomposition of automata rules into additive and nonadditive parts. As a result, it is simple to determine fixed points (those states for which the rule reduces to the identity), and shift cycles (sets of states on which the rule reduces to a shift). Sets of states on which any given nearest neighbor automaton reduces to an identity or a shift are characterized. This allows us to obtain some results on the entropic properties of nonadditive automata, although these are not nearly so complete as results obtained for additive automata. 相似文献
37.
Kingery DA Pfund E Voorhees RM Okuda K Wohlgemuth I Kitchen DE Rodnina MV Strobel SA 《Chemistry & biology》2008,15(5):493-500
The ribosome has an active site comprised of RNA that catalyzes peptide bond formation. To understand how RNA promotes this reaction requires a detailed understanding of the chemical transition state. Here, we report the Br?nsted coefficient of the alpha-amino nucleophile with a series of puromycin derivatives. Both 50S subunit- and 70S ribosome-catalyzed reactions displayed linear free-energy relationships with slopes close to zero under conditions where chemistry is rate limiting. These results indicate that, at the transition state, the nucleophile is neutral in the ribosome-catalyzed reaction, in contrast to the substantial positive charge reported for typical uncatalyzed aminolysis reactions. This suggests that the ribosomal transition state involves deprotonation to a degree commensurate with nitrogen-carbon bond formation. Such a transition state is significantly different from that of uncatalyzed aminolysis reactions in solution. 相似文献
38.
Peter de B. Harrington Kent J. Voorhees Franco Basile Alan D. Hendricker 《Journal of the American Society for Mass Spectrometry》2002,13(1):10-21
Temperature constrained cascade correlation networks (TCCCNs) are computational neural networks that configure their own architecture, train rapidly, and give reproducible prediction results. TCCCN classification models were built using the Latin-partition method for five classes of pathogenic bacteria. Neural networks are problematic in that the relationships among the inputs (i.e., mass spectra) and the outputs (i.e., the bacterial identities) are not apparent. In this study, neural network models were constructed that successfully classified the targeted bacteria and the classification model was validated using sensitivity and target transformation factor analysis (TTFA). Without validation of the classification model, it is impossible to ascertain whether the bacteria are classified by peaks in the mass spectrum that have no causal relationships with the bacteria, but instead randomly correlate with the bacterial classes. Multiple single output network models did not offer any benefits when compared to single network models that had multiple outputs. A multiple output TCCCN model achieved classification accuracies of 96 +/- 2% and exhibited improved performance over multiple single output TCCCN models. Chemical ionization mass spectra were obtained from in situ thermal hydrolysis methylation of freeze-dried bacteria. Mass spectral peaks that pertain to the neural network classification model of the pathogenic bacterial classes were obtained by sensitivity analysis. A significant number of mass spectral peaks that had high sensitivity corresponded to known biomarkers, which is the first time that the significant peaks used by a neural network model to classify mass spectra have been divulged. Furthermore, TTFA furnishes a useful visual target as to which peaks in the mass spectrum correlate with the bacterial identities. 相似文献
39.
A procedure is explained to determined the amount of several pairs of diametrical loads applied to the outside boundary of
a ring when stresses at selected points of the inside or outside boundaries are known. Coefficients of influence are used,
following an approach similar to the one presented in a previous paper. Examples of application are given and the possible
increase in precision is shown when the number of points of measurements is larger than the number of loads to be determined. 相似文献
40.
Burton Voorhees 《Communications in Mathematical Physics》1988,117(3):431-439
This paper reports the solution of the problem of finding which inputs for a function of discrete variables will result in any specified output for the set of binomially determined nearest neighbor additive cellular automata defined on finite or half-infinite sequences. In computing the solution to this problem a process which is the discrete analog to backward integration is defined. This process is determined in terms of an operator which exhibits an interesting period multiplying property. 相似文献