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A. di Bona S.F. Contri G.C. Gazzadi S. Valeri P. Vavassori 《Journal of magnetism and magnetic materials》2007
Square magnetic elements with side in the 100–500 nm range have been fabricated using the focused ion beam (FIB) milling technique from a 10 nm thick, single-crystal Fe film, epitaxially grown on MgO(0 0 1). Thanks to the good crystal quality of the film, magnetic elements with well-defined magnetocrystalline anisotropy have been prepared, while the fine control of the size and shape of the magnets allows for the effective engineering of the anisotropic behavior of the magnetostatic energy that determines the so-called configurational anisotropy. Micromagnetic calculations and experiments show that the angular dependence of the transverse susceptibility has a strong dependence on the material parameters as well as on the static applied field. This allows the effective engineering of the total anisotropy of the magnets. 相似文献
84.
A new transient regime in the relaxation towards absolute equilibrium of the conservative and time-reversible 3D Euler equation with a high-wave-number spectral truncation is characterized. Large-scale dissipative effects, caused by the thermalized modes that spontaneously appear between a transition wave number and the maximum wave number, are calculated using fluctuation dissipation relations. The large-scale dynamics is found to be similar to that of high-Reynolds number Navier-Stokes equations and thus obeys (at least approximately) Kolmogorov scaling. 相似文献
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86.
Daniele Baboneau G. Di Bona P. Chelle M. Decroisette J. Martineau 《Physics letters. A》1976,57(3):247-249
Fast ions theoretical distribution functions deduced from ponderomotive force mechanism are computed and compared to those obtained in laser plasma experiments. Within the limit of validity of the calculations, experimental and theoretical results are in good agreement. 相似文献
87.
The general Hartree-Fock energy in the frontier orbital model in the terms of independent variables is given. The existence conditions for extrema of this expression are derived and their relation with various types of solutions of the HF problem as RHF, UHF and complex wavefunctions is shown. The connection between overall properties of the energy surface and the local properties i.e. the stability and instability conditions of various kinds is demonstrated. The conditions for the occurrence of strange HF solutions are expressed in terms of quantities characterizing the correlation effects. This shows explicitly that the lack of respecting the electronic correlation is the reason for the occurrence of the strange HF solutions for the molecular configurations which exhibit a certain amount of diradical character.The summary of the results has been presented at the 6th Jerusalem Symposium on Quantum Chemistry and Biochemistry and at the I. Congress of Quantum Chemistry, Menton, July 1973.On leave of absence from Institute Rudjer Bokovi, Zagreb, Yugoslavia. 相似文献
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Eulerian granular multiphase model with a drag coefficient correction based on the energy-minimization multi-scale (EMMS) model was used to simulate a semi-industry scale circulating fluidized bed (CFB). Three-dimensional (3D), time-dependent simulation of a full-loop CFB revealed that the axial profiles of cross-sectionally averaged solid volume fraction, and the radial profiles of solid axial velocity and solid volume fraction were in reasonable agreement with experimental data. Based on this agreement, database derived from experiments not yet accomplished was replenished with such simulations, and fluid regime diagrams and pressure balance around the CFB loop were derived accordingly. This work presents an integrated viewpoint on CFB and unfolds a fresh paradigm for CFB modeling, which can be expected to help resolve certain issues long in dispute but bard for experiments. 相似文献
90.
V. Bonačić-Koutecký M. Hartmann J. Pittner 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2001,16(1):133-138
We present the ultrafast multistate nuclear dynamics involving adiabatic and nonadiabatic excited states of non-stoichiometric
halide deficient clusters (NanFn-1) characterized by strong ionic bonding and one-excess electron for which the “frozen ionic bonds” approximation has been
justified allowing to consider the optical response of the single excess electron in the effective field of the other electrons.
We combined the Wigner-Moyal representation of the vibronic density matrix with the ab initio multi state molecular dynamics in the ground and excited electronic states including the nonadiabatic couplings calculated
“on the fly” at low computational demand. This method allows the simulation of femtosecond pump-probe and pump-dump signals
based on an analytical formulation, which utilizes temperature dependent ground state initial conditions, an ensemble of trajectories
carried out on the electronic excited state as well as on the ground state after the passage through the conical intersection
in the case of nonadiabatic dynamics and for probing either in the cationic state or in the ground state. The choice of the
systems we presented has been made in order to determine the timescales of the fast geometric relaxation leaving the bonding
frame intact as during the dynamics in the first excited state of Na4F3, and of the bond breaking processes leading to conical intersection between the first excited state and the ground state
as in Na3F2. The former is the smallest finite system prototype for an surface F-center of bulk color centers. The latter allows to study
the photo isomerization in full complexity taking into account all degrees of freedom. In the case of Na4F3 after the fast geometric relaxation in the excited state leading to deformed cuboidal structure without breaking of bonds,
different types of internal vibrational redistribution (IVR) processes have been identified in pump-dump signals by tuning
the dump laser. In contrast, from the analysis of the pump-probe signals of Na3F2 cluster, the timescales for the metallic and the ionic bond breaking, as well as for the passage through conical intersection
have been determined. Finally the conditions under which these processes can be experimentally observed have been identified.
Received 22 December 2000 相似文献